On the reality of residual entropies of glasses and disordered crystals
We show that the hypothesis that the configurational entropy of a liquid disappears when it is kinetically frozen into a single glass state implies a spontaneous decrease of entropy. We show further that this is not an innocuous exception to the second law that requires a slight modification of that...
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| Veröffentlicht in: | The Journal of chemical physics 2008-04, Vol.128 (15), p.154510-154510-7 |
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| Format: | Artikel |
| Sprache: | eng |
| Online-Zugang: | Volltext |
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