Towards atomic site-selective sensitivity in tip-enhanced Raman spectroscopy

Towards atomic site-selective sensitivity in tip-enhanced Raman spectroscopy

Depending on each nitrogen atom of adenine molecule to which a silver atom of a metallic tip approaches, tip-enhanced near-field Raman spectroscopy may show a potential to achieve atomic site-selective detection sensitivity. Molecular vibrational calculations show that silver atoms and adenine molec...

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Veröffentlicht in:The Journal of chemical physics 2006-12, Vol.125 (24), p.244706-244706
Hauptverfasser: Hayazawa, Norihiko, Watanabe, Hiroyuki, Saito, Yuika, Kawata, Satoshi
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container_issue 24
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container_title The Journal of chemical physics
container_volume 125
creator Hayazawa, Norihiko
Watanabe, Hiroyuki
Saito, Yuika
Kawata, Satoshi
description Depending on each nitrogen atom of adenine molecule to which a silver atom of a metallic tip approaches, tip-enhanced near-field Raman spectroscopy may show a potential to achieve atomic site-selective detection sensitivity. Molecular vibrational calculations show that silver atoms and adenine molecule create several isomers generating specific vibrational modes of each isomer that are shifted or not observable in isolated adenine molecule itself. Here, the authors observe the specific vibrational modes and spectral shifts of isomers experimentally and are in good agreement with their calculations.
doi_str_mv 10.1063/1.2423015
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title Towards atomic site-selective sensitivity in tip-enhanced Raman spectroscopy
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