Selective Detection Method Derived from a Controlled Diffusion Process at Metal-Modified Diamond Electrodes

A novel, selective methodology is derived based on the difference between the diffusion processes at microelectrodes (i.e., hemispherical diffusion) and the macroelectrode (i.e., linear diffusion) in a metal-implanted boron-doped diamond electrode (metal-BDDs). As an example, the selective detection...

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Veröffentlicht in:Analytical chemistry (Washington) 2006-11, Vol.78 (22), p.7857-7860
Hauptverfasser: Watanabe, Takeshi, Ivandini, Tribidasari A, Makide, Yoshihiro, Fujishima, Akira, Einaga, Yasuaki
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container_end_page 7860
container_issue 22
container_start_page 7857
container_title Analytical chemistry (Washington)
container_volume 78
creator Watanabe, Takeshi
Ivandini, Tribidasari A
Makide, Yoshihiro
Fujishima, Akira
Einaga, Yasuaki
description A novel, selective methodology is derived based on the difference between the diffusion processes at microelectrodes (i.e., hemispherical diffusion) and the macroelectrode (i.e., linear diffusion) in a metal-implanted boron-doped diamond electrode (metal-BDDs). As an example, the selective detection of glucose in a solution containing interference species such as ascorbic acid and uric acid is demonstrated. The electrochemical properties of BDD, which are low background current, extremely high stability, and (especially) inactivity toward glucose, play an important role in realizing these differences in the diffusion characteristics. The present methodology can be applied not only to selective glucose detection by the metal-BDD system but also to other selective detection systems.
doi_str_mv 10.1021/ac060860j
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subjects Analytical chemistry
Ascorbic Acid - chemistry
Biosensing Techniques
Chemistry
Diamond - chemistry
Diamonds
Diffusion
Electrochemical methods
Electrochemistry
Electrodes
Exact sciences and technology
Glucose
Glucose - analysis
Metals - chemistry
Sensitivity and Specificity
Surface Properties
Time Factors
Uric Acid - chemistry
title Selective Detection Method Derived from a Controlled Diffusion Process at Metal-Modified Diamond Electrodes
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