Driving Multi-electron Reactions with Photons: Dinuclear Ruthenium Complexes Capable of Stepwise and Concerted Multi-electron Reduction

Using biological precedents, it is expected that concerted, multi-electron reduction processes will play a significant role in the development of efficient artificial photosynthetic systems. We have found that the dinuclear ruthenium complexes [(phen)₂Ru(tatpp)Ru(phen)₂]⁴⁺ (P) and [(phen)₂Ru(tatpq)...

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Veröffentlicht in:	Photosynthesis research 2006, Vol.87 (1), p.41-55
Hauptverfasser:	Wouters, Kelly L, de Tacconi, Norma R, Konduri, Rama, Lezna, Reynaldo O, MacDonnell, Frederick M
Format:	Artikel
Sprache:	eng
Schlagworte:	Atoms & subatomic particles Dimerization Electrochemistry Electrons energy Kinetics ligands Oxidation-Reduction photocatalyst Photons Photosynthesis reducing agents ruthenium Ruthenium - chemistry spectroscopy
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