UV-Induced Nonlinear Absorption in Lanthanum Calcium Borate Single Crystals

UV-Induced Nonlinear Absorption in Lanthanum Calcium Borate Single Crystals

It has been revealed that lanthanum calcium borate (La2CaB10O19) crystals show two-photon absorption (TPA) induced by a UV laser field. UV-induced TPA measurements were performed in the spectral range of 475−1130 nm using as fundamental beam the third harmonics of the 28 ps Nd−YAG pulsed laser as a...

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Veröffentlicht in:The journal of physical chemistry. B 2006-05, Vol.110 (18), p.9090-9094
Hauptverfasser: Kityk, I. V, Majchrowski, A, Michalski, E, Kasprowicz, D, Drozdowski, M, Kisielewski, J, Lukasiewicz, T, Sahraoui, B
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container_end_page 9094
container_issue 18
container_start_page 9090
container_title The journal of physical chemistry. B
container_volume 110
creator Kityk, I. V
Majchrowski, A
Michalski, E
Kasprowicz, D
Drozdowski, M
Kisielewski, J
Lukasiewicz, T
Sahraoui, B
description It has been revealed that lanthanum calcium borate (La2CaB10O19) crystals show two-photon absorption (TPA) induced by a UV laser field. UV-induced TPA measurements were performed in the spectral range of 475−1130 nm using as fundamental beam the third harmonics of the 28 ps Nd−YAG pulsed laser as a pumping beam for LiB3O5 optical parametrized generator using Z-scan method. Investigations performed by the Z-scan method were done during illumination by a Xe−F laser (λ = 217 nm) as a photoinducing (pumping) beam. The pumping laser beam created a thin surface layer (about 80−90 nm) that was the source of the observed photoinduced TPA. The highest values of the TPA β coefficients were achieved for polarization of the pumping light directed along the second-order crystallographic axis of the investigated crystals. The obtained values of the TPA coefficients were higher than those for the BiB3O6 crystals investigated earlier by us.
doi_str_mv 10.1021/jp060079f
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title UV-Induced Nonlinear Absorption in Lanthanum Calcium Borate Single Crystals
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