Femtosecond Imaging of Surface Plasmon Dynamics in a Nanostructured Silver Film

Light interacting with nanostructured metals excites the collective charge density fluctuations known as surface plasmons (SP). Through excitation of the localized SP eigenmodes incident light is trapped on the nanometer spatial and femtosecond temporal scales and its field is enhanced. Here we demo...

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Veröffentlicht in:Nano letters 2005-06, Vol.5 (6), p.1123-1127
Hauptverfasser: Kubo, Atsushi, Onda, Ken, Petek, Hrvoje, Sun, Zhijun, Jung, Yun S, Kim, Hong Koo
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container_end_page 1127
container_issue 6
container_start_page 1123
container_title Nano letters
container_volume 5
creator Kubo, Atsushi
Onda, Ken
Petek, Hrvoje
Sun, Zhijun
Jung, Yun S
Kim, Hong Koo
description Light interacting with nanostructured metals excites the collective charge density fluctuations known as surface plasmons (SP). Through excitation of the localized SP eigenmodes incident light is trapped on the nanometer spatial and femtosecond temporal scales and its field is enhanced. Here we demonstrate the imaging and quantum control of SP dynamics in a nanostructured silver film. By inducing and imaging the nonlinear two-photon photoemission from the sample with a pair of identical 10-fs laser pulses while scanning the pulse delay, we record a movie of SP fields at a rate of 330-attoseconds/frame.
doi_str_mv 10.1021/nl0506655
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subjects Applied sciences
Condensed matter: structure, mechanical and thermal properties
Electronics
Electrons
Exact sciences and technology
Kinetics
Lasers
Light
Microelectronic fabrication (materials and surfaces technology)
Microscopy, Electron
Microscopy, Electron, Scanning
Nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals
Nanotechnology - methods
Oscillometry
Photons
Physics
Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices
Silver - chemistry
Spectrophotometry
Structure of solids and liquids
crystallography
Surface Plasmon Resonance - methods
Time Factors
title Femtosecond Imaging of Surface Plasmon Dynamics in a Nanostructured Silver Film
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