How to measure Χ(3) of a nanoparticle

Most of the known methods to measure the nonlinear optical properties of materials deal with the bulk properties, but there are many demanding applications that require those measurements to be done on a single particle or a single molecule. We report a novel application of nonlinear optics to measu...

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Veröffentlicht in:Optics letters 2006-05, Vol.31 (10), p.1486-1488
Hauptverfasser: SHCHESLAVSKIY, Vladislav I, SALTIEL, Solomon M, FAUSTOV, Alexey R, PETROV, Georgi I, YAKOVLEV, Vladislav V
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container_end_page 1488
container_issue 10
container_start_page 1486
container_title Optics letters
container_volume 31
creator SHCHESLAVSKIY, Vladislav I
SALTIEL, Solomon M
FAUSTOV, Alexey R
PETROV, Georgi I
YAKOVLEV, Vladislav V
description Most of the known methods to measure the nonlinear optical properties of materials deal with the bulk properties, but there are many demanding applications that require those measurements to be done on a single particle or a single molecule. We report a novel application of nonlinear optics to measure the third-order nonlinear optical susceptibility of nanoparticles in solutions. By measuring the power of the third harmonic generated in a diluted solution of nanoparticles, both the size and chi(3) can be extracted from a simple set of measurements.
doi_str_mv 10.1364/OL.31.001486
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source MEDLINE; Optica Publishing Group Journals
subjects Algorithms
Crystallography - methods
Exact sciences and technology
Fundamental areas of phenomenology (including applications)
Image Enhancement - methods
Image Interpretation, Computer-Assisted - methods
Imaging, Three-Dimensional - methods
Information Storage and Retrieval - methods
Molecular Conformation
Nanostructures - chemistry
Nanostructures - ultrastructure
Nephelometry and Turbidimetry - methods
Nonlinear optics
Optics
Physics
Reproducibility of Results
Scattering, Radiation
Sensitivity and Specificity
Ultrafast processes
optical pulse generation and pulse compression
title How to measure Χ(3) of a nanoparticle
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