Strong exciton-photon coupling and exciton hybridization in a thermally evaporated polycrystalline film of an organic small molecule
We demonstrate strong exciton-photon coupling in an optical microcavity containing a thermally evaporated polycrystalline organic thin film. Microcavity polaritons result from coupling between the 0-0 excitonic transition of 3,4,7,8 napthalenetetracarboxylic dianhydride and a cavity photon. For thic...
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| Veröffentlicht in: | Physical review letters 2004-10, Vol.93 (18), p.186404.1-186404.4, Article 186404 |
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| container_end_page | 186404.4 |
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| container_issue | 18 |
| container_start_page | 186404.1 |
| container_title | Physical review letters |
| container_volume | 93 |
| creator | HOLMES, R. J FORREST, S. R |
| description | We demonstrate strong exciton-photon coupling in an optical microcavity containing a thermally evaporated polycrystalline organic thin film. Microcavity polaritons result from coupling between the 0-0 excitonic transition of 3,4,7,8 napthalenetetracarboxylic dianhydride and a cavity photon. For thicker films, the 0-1 transition also couples to the cavity mode, as vibronic relaxation is overcome by the short Rabi period for strong coupling. To our knowledge, this is the first report of strong coupling between a cavity photon and multiple vibronic transitions in a single material, made possible by the pronounced vibronic absorption features characteristic of crystalline organic materials. |
| doi_str_mv | 10.1103/physrevlett.93.186404 |
| format | Article |
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To our knowledge, this is the first report of strong coupling between a cavity photon and multiple vibronic transitions in a single material, made possible by the pronounced vibronic absorption features characteristic of crystalline organic materials.</description><subject>Condensed matter: electronic structure, electrical, magnetic, and optical properties</subject><subject>Exact sciences and technology</subject><subject>Fundamental areas of phenomenology (including applications)</subject><subject>Optical materials</subject><subject>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</subject><subject>Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures</subject><subject>Optical properties of nanoscale materials and structures</subject><subject>Optics</subject><subject>Physics</subject><subject>Polymers and organics</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><recordid>eNpFkMuO1DAQRS0EYpqBTwB5A7s05diO4yUaDQ-pJRCPdeQ4lWkjJw620yKs-XA86kazKtn33CrpEPKSwZ4x4G-X45YinjzmvNd8z9pGgHhEdgyUrhRj4jHZAXBWaQB1RZ6l9BMAWN20T8kVk7KWrG135O-3HMN8R_G3dTnM1XIMZVAb1sW78m_m4X9Gj1sf3eD-mOzKy83U0HzEOBnvN4ons4RoMg50CX6zcUu5BG5GOjo_0TCWXTTEOzM7S9N9iU7Bo109PidPRuMTvrjMa_Lj_e33m4_V4fOHTzfvDpUVUuaKqQE4cqkH2WvDrWhkK20tlAFt1CiEVVKiRlRGjiXpRV83tQTeWK0HJfg1eXPeu8Twa8WUu8kli96bGcOaukYBVxpYAeUZtDGkonnslugmE7eOQXevv_tS9H_F06Ho7zTvzvpL79XlwNpPODy0Lr4L8PoCmGSNH6OZrUsPXFO3WrSC_wMS-ZSf</recordid><startdate>20041029</startdate><enddate>20041029</enddate><creator>HOLMES, R. 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R</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c455t-17d03e359d5b9a3c46585c247a09a7f44c755e9ee7a5f85cb4b2625036c99d743</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2004</creationdate><topic>Condensed matter: electronic structure, electrical, magnetic, and optical properties</topic><topic>Exact sciences and technology</topic><topic>Fundamental areas of phenomenology (including applications)</topic><topic>Optical materials</topic><topic>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</topic><topic>Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures</topic><topic>Optical properties of nanoscale materials and structures</topic><topic>Optics</topic><topic>Physics</topic><topic>Polymers and organics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>HOLMES, R. 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R</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Strong exciton-photon coupling and exciton hybridization in a thermally evaporated polycrystalline film of an organic small molecule</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2004-10-29</date><risdate>2004</risdate><volume>93</volume><issue>18</issue><spage>186404.1</spage><epage>186404.4</epage><pages>186404.1-186404.4</pages><artnum>186404</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><coden>PRLTAO</coden><abstract>We demonstrate strong exciton-photon coupling in an optical microcavity containing a thermally evaporated polycrystalline organic thin film. Microcavity polaritons result from coupling between the 0-0 excitonic transition of 3,4,7,8 napthalenetetracarboxylic dianhydride and a cavity photon. 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| ispartof | Physical review letters, 2004-10, Vol.93 (18), p.186404.1-186404.4, Article 186404 |
| issn | 0031-9007 1079-7114 |
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| source | American Physical Society Journals |
| subjects | Condensed matter: electronic structure, electrical, magnetic, and optical properties Exact sciences and technology Fundamental areas of phenomenology (including applications) Optical materials Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures Optical properties of nanoscale materials and structures Optics Physics Polymers and organics |
| title | Strong exciton-photon coupling and exciton hybridization in a thermally evaporated polycrystalline film of an organic small molecule |
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