Picosecond time-resolved laser pump/X-ray probe experiments using a gated single-photon-counting area detector

The recent developments in X‐ray detectors have opened new possibilities in the area of time‐resolved pump/probe X‐ray experiments; this article presents the novel use of a PILATUS detector to achieve X‐ray pulse duration limited time‐resolution at the Advanced Photon Source (APS), USA. The capabili...

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Veröffentlicht in:Journal of synchrotron radiation 2009-05, Vol.16 (3), p.387-390
Hauptverfasser: Ejdrup, T., Lemke, H. T., Haldrup, K., Nielsen, T. N., Arms, D. A., Walko, D. A., Miceli, A., Landahl, E. C., Dufresne, E. M., Nielsen, M. M.
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container_end_page 390
container_issue 3
container_start_page 387
container_title Journal of synchrotron radiation
container_volume 16
creator Ejdrup, T.
Lemke, H. T.
Haldrup, K.
Nielsen, T. N.
Arms, D. A.
Walko, D. A.
Miceli, A.
Landahl, E. C.
Dufresne, E. M.
Nielsen, M. M.
description The recent developments in X‐ray detectors have opened new possibilities in the area of time‐resolved pump/probe X‐ray experiments; this article presents the novel use of a PILATUS detector to achieve X‐ray pulse duration limited time‐resolution at the Advanced Photon Source (APS), USA. The capability of the gated PILATUS detector to selectively detect the signal from a given X‐ray pulse in 24 bunch mode at the APS storage ring is demonstrated. A test experiment performed on polycrystalline organic thin films of α‐perylene illustrates the possibility of reaching an X‐ray pulse duration limited time‐resolution of 60 ps using the gated PILATUS detector. This is the first demonstration of X‐ray pulse duration limited data recorded using an area detector without the use of a mechanical chopper array at the beamline.
doi_str_mv 10.1107/S0909049509004658
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source Wiley Online Library Open Access
subjects Computer-Aided Design
Equipment Design
Equipment Failure Analysis
Lasers, Solid-State
Photometry - instrumentation
PILATUS
pixel detector
Radiation Dosage
Radiometry - instrumentation
Reproducibility of Results
Sensitivity and Specificity
time-resolved X-ray diffraction
Transducers
X-Ray Diffraction - instrumentation
α-perylene
title Picosecond time-resolved laser pump/X-ray probe experiments using a gated single-photon-counting area detector
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