Molecular Design of Solid Polymer Electrolytes with Enthalpy–Entropy Manipulation for Li Metal Batteries with Aggressive Cathode Chemistry

Solid polymer electrolytes (SPEs) with high ion conductivity, high Li+ transference number, and a wide electrochemical window are promising for the next-generation high-energy Li metal batteries (LMBs). Here we describe an enthalpy–entropy manipulation strategy enabling a class of polycarbonate-base...

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