High-performance multifunctional porous iron Acetylacetonate/N, O-doped carbon nanospheres for electromagnetic wave absorption at 2–18 GHz and methyl orange absorption
[Display omitted] Nowadays, multifunction is regarded as an advanced development direction of new-generation electromagnetic wave absorption (EMWA) materials to fulfill the ever-growing demands in complex environment and situation. Environmental pollution and electromagnetic pollution are all diffic...
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Veröffentlicht in: | Journal of colloid and interface science 2023-09, Vol.646, p.54-66 |
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creator | He, Enhui Xue, Liying Wang, Zheng Yan, Xuefeng Yu, Liangmin |
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Nowadays, multifunction is regarded as an advanced development direction of new-generation electromagnetic wave absorption (EMWA) materials to fulfill the ever-growing demands in complex environment and situation. Environmental pollution and electromagnetic pollution are all difficult problems for human beings all the time. Now, there is no multifunctional materials for collaborative treatment of environmental and electromagnetic pollution. Herein, We synthesized nanospheres with divinyl benzene (DVB) and N-[3-(dimethylamino)propyl]methacrylamide (DMAPMA), using a simple one-pot method. After calcination at 800 ℃ in N2, porous N, O-doped porous carbon materials were prepared. By regulating the mole ratio of DVB and DMAPMA, the ratio was 5:1 reached excellent EMWA property. Remarkably, the introduction of iron acetylacetonate into the reaction of DVB and DMAPMA was effective in enhancing the absorption bandwidth to 8.00 GHz at a 3.74 mm thickness, which depended on the synergistic effects from dielectric and magnetic losses. Simultaneously, the Fe-doped carbon materials had a methyl orange adsorption capacity. The adsorption isotherm conformed to the Freundlich model. After methyl orange absorption, the EMWA property did not greatly change. Thus, this research paves the way for the creation of multifunctional materials to solve environmental pollution and electromagnetic pollution together. |
doi_str_mv | 10.1016/j.jcis.2023.05.027 |
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Nowadays, multifunction is regarded as an advanced development direction of new-generation electromagnetic wave absorption (EMWA) materials to fulfill the ever-growing demands in complex environment and situation. Environmental pollution and electromagnetic pollution are all difficult problems for human beings all the time. Now, there is no multifunctional materials for collaborative treatment of environmental and electromagnetic pollution. Herein, We synthesized nanospheres with divinyl benzene (DVB) and N-[3-(dimethylamino)propyl]methacrylamide (DMAPMA), using a simple one-pot method. After calcination at 800 ℃ in N2, porous N, O-doped porous carbon materials were prepared. By regulating the mole ratio of DVB and DMAPMA, the ratio was 5:1 reached excellent EMWA property. Remarkably, the introduction of iron acetylacetonate into the reaction of DVB and DMAPMA was effective in enhancing the absorption bandwidth to 8.00 GHz at a 3.74 mm thickness, which depended on the synergistic effects from dielectric and magnetic losses. Simultaneously, the Fe-doped carbon materials had a methyl orange adsorption capacity. The adsorption isotherm conformed to the Freundlich model. After methyl orange absorption, the EMWA property did not greatly change. Thus, this research paves the way for the creation of multifunctional materials to solve environmental pollution and electromagnetic pollution together.</description><identifier>ISSN: 0021-9797</identifier><identifier>EISSN: 1095-7103</identifier><identifier>DOI: 10.1016/j.jcis.2023.05.027</identifier><identifier>PMID: 37182259</identifier><language>eng</language><publisher>United States: Elsevier Inc</publisher><subject>absorption ; adsorption ; carbon ; Electrical properties ; electromagnetic radiation ; humans ; iron ; Magnetic properties ; magnetism ; methyl orange ; Multifunctional composites ; Nanoparticles ; nanospheres ; pollution ; sorption isotherms</subject><ispartof>Journal of colloid and interface science, 2023-09, Vol.646, p.54-66</ispartof><rights>2023 Elsevier Inc.</rights><rights>Copyright © 2023 Elsevier Inc. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c389t-75e121c54f554788dc8006624beba763df87eefd3c83a6b4212899093a0431af3</citedby><cites>FETCH-LOGICAL-c389t-75e121c54f554788dc8006624beba763df87eefd3c83a6b4212899093a0431af3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0021979723008093$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65534</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/37182259$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>He, Enhui</creatorcontrib><creatorcontrib>Xue, Liying</creatorcontrib><creatorcontrib>Wang, Zheng</creatorcontrib><creatorcontrib>Yan, Xuefeng</creatorcontrib><creatorcontrib>Yu, Liangmin</creatorcontrib><title>High-performance multifunctional porous iron Acetylacetonate/N, O-doped carbon nanospheres for electromagnetic wave absorption at 2–18 GHz and methyl orange absorption</title><title>Journal of colloid and interface science</title><addtitle>J Colloid Interface Sci</addtitle><description>[Display omitted]
Nowadays, multifunction is regarded as an advanced development direction of new-generation electromagnetic wave absorption (EMWA) materials to fulfill the ever-growing demands in complex environment and situation. Environmental pollution and electromagnetic pollution are all difficult problems for human beings all the time. Now, there is no multifunctional materials for collaborative treatment of environmental and electromagnetic pollution. Herein, We synthesized nanospheres with divinyl benzene (DVB) and N-[3-(dimethylamino)propyl]methacrylamide (DMAPMA), using a simple one-pot method. After calcination at 800 ℃ in N2, porous N, O-doped porous carbon materials were prepared. By regulating the mole ratio of DVB and DMAPMA, the ratio was 5:1 reached excellent EMWA property. Remarkably, the introduction of iron acetylacetonate into the reaction of DVB and DMAPMA was effective in enhancing the absorption bandwidth to 8.00 GHz at a 3.74 mm thickness, which depended on the synergistic effects from dielectric and magnetic losses. Simultaneously, the Fe-doped carbon materials had a methyl orange adsorption capacity. The adsorption isotherm conformed to the Freundlich model. After methyl orange absorption, the EMWA property did not greatly change. Thus, this research paves the way for the creation of multifunctional materials to solve environmental pollution and electromagnetic pollution together.</description><subject>absorption</subject><subject>adsorption</subject><subject>carbon</subject><subject>Electrical properties</subject><subject>electromagnetic radiation</subject><subject>humans</subject><subject>iron</subject><subject>Magnetic properties</subject><subject>magnetism</subject><subject>methyl orange</subject><subject>Multifunctional composites</subject><subject>Nanoparticles</subject><subject>nanospheres</subject><subject>pollution</subject><subject>sorption isotherms</subject><issn>0021-9797</issn><issn>1095-7103</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNqFkU9u1DAUhy0EokPhAiyQlyxI6j9x4khsqgo6SBXdwNpynJcZjxI72E6rYcUduABrjsFRepJ6NAWxgs17i_e93-L3IfSSkpISWp_typ2xsWSE8ZKIkrDmEVpR0oqioYQ_RitCGC3apm1O0LMYd4RQKkT7FJ3whkrGRLtCP9d2sy1mCIMPk3YG8LSMyQ6LM8l6p0c8--CXiG3wDp8bSPtR55lPCc4-vsHXRe9n6LHRocuE087HeQsBIs6RGEYwKfhJbxwka_CtvgGsu-jDfMjHOmF29-07lb9-XK6_Yu16PEHa7kfsg3abv9nn6MmgxwgvHvYp-vz-3aeLdXF1ffnh4vyqMFy2qWgEUEaNqAYhqkbK3khC6ppVHXS6qXk_yAZg6LmRXNddxSiTbUtarknFqR74KXp9zJ2D_7JATGqy0cA4age5CcWp4LJipCb_RZmkXEop6jqj7Iia4GMMMKg52EmHvaJEHXSqnTroVAedigiVdeanVw_5SzdB_-flt78MvD0CkAu5sRBUNBayxt6GXLzqvf1X_j08r7WX</recordid><startdate>20230915</startdate><enddate>20230915</enddate><creator>He, Enhui</creator><creator>Xue, Liying</creator><creator>Wang, Zheng</creator><creator>Yan, Xuefeng</creator><creator>Yu, Liangmin</creator><general>Elsevier Inc</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7S9</scope><scope>L.6</scope></search><sort><creationdate>20230915</creationdate><title>High-performance multifunctional porous iron Acetylacetonate/N, O-doped carbon nanospheres for electromagnetic wave absorption at 2–18 GHz and methyl orange absorption</title><author>He, Enhui ; Xue, Liying ; Wang, Zheng ; Yan, Xuefeng ; Yu, Liangmin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c389t-75e121c54f554788dc8006624beba763df87eefd3c83a6b4212899093a0431af3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>absorption</topic><topic>adsorption</topic><topic>carbon</topic><topic>Electrical properties</topic><topic>electromagnetic radiation</topic><topic>humans</topic><topic>iron</topic><topic>Magnetic properties</topic><topic>magnetism</topic><topic>methyl orange</topic><topic>Multifunctional composites</topic><topic>Nanoparticles</topic><topic>nanospheres</topic><topic>pollution</topic><topic>sorption isotherms</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>He, Enhui</creatorcontrib><creatorcontrib>Xue, Liying</creatorcontrib><creatorcontrib>Wang, Zheng</creatorcontrib><creatorcontrib>Yan, Xuefeng</creatorcontrib><creatorcontrib>Yu, Liangmin</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>AGRICOLA</collection><collection>AGRICOLA - Academic</collection><jtitle>Journal of colloid and interface science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>He, Enhui</au><au>Xue, Liying</au><au>Wang, Zheng</au><au>Yan, Xuefeng</au><au>Yu, Liangmin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>High-performance multifunctional porous iron Acetylacetonate/N, O-doped carbon nanospheres for electromagnetic wave absorption at 2–18 GHz and methyl orange absorption</atitle><jtitle>Journal of colloid and interface science</jtitle><addtitle>J Colloid Interface Sci</addtitle><date>2023-09-15</date><risdate>2023</risdate><volume>646</volume><spage>54</spage><epage>66</epage><pages>54-66</pages><issn>0021-9797</issn><eissn>1095-7103</eissn><abstract>[Display omitted]
Nowadays, multifunction is regarded as an advanced development direction of new-generation electromagnetic wave absorption (EMWA) materials to fulfill the ever-growing demands in complex environment and situation. Environmental pollution and electromagnetic pollution are all difficult problems for human beings all the time. Now, there is no multifunctional materials for collaborative treatment of environmental and electromagnetic pollution. Herein, We synthesized nanospheres with divinyl benzene (DVB) and N-[3-(dimethylamino)propyl]methacrylamide (DMAPMA), using a simple one-pot method. After calcination at 800 ℃ in N2, porous N, O-doped porous carbon materials were prepared. By regulating the mole ratio of DVB and DMAPMA, the ratio was 5:1 reached excellent EMWA property. Remarkably, the introduction of iron acetylacetonate into the reaction of DVB and DMAPMA was effective in enhancing the absorption bandwidth to 8.00 GHz at a 3.74 mm thickness, which depended on the synergistic effects from dielectric and magnetic losses. Simultaneously, the Fe-doped carbon materials had a methyl orange adsorption capacity. The adsorption isotherm conformed to the Freundlich model. After methyl orange absorption, the EMWA property did not greatly change. Thus, this research paves the way for the creation of multifunctional materials to solve environmental pollution and electromagnetic pollution together.</abstract><cop>United States</cop><pub>Elsevier Inc</pub><pmid>37182259</pmid><doi>10.1016/j.jcis.2023.05.027</doi><tpages>13</tpages></addata></record> |
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subjects | absorption adsorption carbon Electrical properties electromagnetic radiation humans iron Magnetic properties magnetism methyl orange Multifunctional composites Nanoparticles nanospheres pollution sorption isotherms |
title | High-performance multifunctional porous iron Acetylacetonate/N, O-doped carbon nanospheres for electromagnetic wave absorption at 2–18 GHz and methyl orange absorption |
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