Methane pyrolysis in packed bed reactors: Kinetic modeling, numerical simulations, and experimental insights

[Display omitted] •CH4 pyrolysis in a packed bed reactor yields over 98 % H2 and captures carbon.•Coupling of models for carbon deposition, soot formation, and gas-phase microkinetics.•Model captures H2 inhibition effect and formation of by-products.•Numerical simulations of lab-scale reactor behavi...

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Veröffentlicht in:	Chemical engineering journal (Lausanne, Switzerland : 1996) Switzerland : 1996), 2024-04, Vol.485, p.149684, Article 149684
Hauptverfasser:	Mokashi, Manas, Shirsath, Akash Bhimrao, Çelik, Ahmet, Lott, Patrick, Müller, Heinz, Tischer, Steffen, Maier, Lubow, Bode, Johannes, Schlereth, David, Scheiff, Frederik, Flick, Dieter, Bender, Michael, Ehrhardt, Kai, Deutschmann, Olaf
Format:	Artikel
Sprache:	eng
Schlagworte:	carbon Carbon deposition Fixed bed reactor High temperature kinetics hydrogen Hydrogen production methane Methane pyrolysis natural gas polycyclic aromatic hydrocarbons pyrolysis reaction mechanisms soot Soot formation temperature
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