Impact of low molecular weight organic acids on heavy metal(loid) desorption in biochar-amended paddy soil
Low molecular weight organic acids (LMWOAs) are important soil components and play a key role in regulating the geochemical behavior of heavy metal(loid)s. Biochar (BC) is a commonly used amendment that could change LMWOAs in soil. Here, four LMWOAs of oxalic acid (OA), tartaric acid (TA), malic aci...
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| Veröffentlicht in: | Environmental geochemistry and health 2024-08, Vol.46 (8), p.289-289, Article 289 |
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| creator | Huang, Qiuxiang Chen, Wenzhe Gao, Jinyan Meng, Fande Cai, Yongbing Wang, Yan Yuan, Guodong |
| description | Low molecular weight organic acids (LMWOAs) are important soil components and play a key role in regulating the geochemical behavior of heavy metal(loid)s. Biochar (BC) is a commonly used amendment that could change LMWOAs in soil. Here, four LMWOAs of oxalic acid (OA), tartaric acid (TA), malic acid (MA), and citric acid (CA) were evaluated for their roles in changing Cd and SB desorption behavior in contaminated soil with (S1-BC) or without BC (S1) produced from
Paulownia
biowaste. The results showed that OA, TA, MA, and CA reduced soil pH with rising concentrations, and biochar partially offset the pH reduction by LMWOAs. The LMWOAs reduced Cd desorption from the soil at low concentrations but increased Cd desorption at high concentrations, and CA was the most powerful in this regard. The LMWOAs had a similar effect on Sb desorption, and CA was the most effective species of LMWOAs. Adding BC to the soil affects Cd and Sb dynamics by reducing the Cd desorption but increasing Sb desorption from the soil and increasing the distribution coefficient (
K
d
) values of Cd but lowering the
K
d
values of Sb. This study helped understand the effects of LMWOAs on the geochemical behavior of Cd and Sb in the presence of biochar, as well as the potential risks of biochar amendment in enhancing Sb desorption from contaminated soil. |
| doi_str_mv | 10.1007/s10653-024-02064-6 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_3153665025</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>3076422714</sourcerecordid><originalsourceid>FETCH-LOGICAL-c289t-e462daa677142546dc9578071673253a4fdbb5483a2afa691da04fa5abe457273</originalsourceid><addsrcrecordid>eNqFkU1v1DAQhi1ERZfCH-CALHEphxR_OzmiCmilSr2UszWxnV2vnDjYCdX-e9xuoRIHOFgjeZ557dGD0DtKLigh-lOhREneECbqIUo06gXaUKl5w7qWv0QbwlTXCCLYKXpdyp4Q0mnRvkKnvO00UV27QfvrcQa74DTgmO7xmKK3a4SM733Y7up93sIULAYbXMFpwjsPPw949AvE85iC-4idLynPS6jNMOE-JLuD3MDoJ-cdnsG5Ay4pxDfoZIBY_Nuneoa-f_1yd3nV3Nx-u778fNNY1nZL44ViDkBpTQWTQjnbSd0STZXmTHIQg-t7KVoODAZQHXVAxAASei-kZpqfofNj7pzTj9WXxYyhWB8jTD6txXAquVKS1LD_okQrwVj9SUU__IXu05qnusgjxYngVFWKHSmbUynZD2bOYYR8MJSYB2nmKM1UaeZRmnkYev8Uvfajd39GfluqAD8Cpbamrc_Pb_8j9hcHpaDi</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>3076304316</pqid></control><display><type>article</type><title>Impact of low molecular weight organic acids on heavy metal(loid) desorption in biochar-amended paddy soil</title><source>MEDLINE</source><source>SpringerLink Journals - AutoHoldings</source><creator>Huang, Qiuxiang ; Chen, Wenzhe ; Gao, Jinyan ; Meng, Fande ; Cai, Yongbing ; Wang, Yan ; Yuan, Guodong</creator><creatorcontrib>Huang, Qiuxiang ; Chen, Wenzhe ; Gao, Jinyan ; Meng, Fande ; Cai, Yongbing ; Wang, Yan ; Yuan, Guodong</creatorcontrib><description>Low molecular weight organic acids (LMWOAs) are important soil components and play a key role in regulating the geochemical behavior of heavy metal(loid)s. Biochar (BC) is a commonly used amendment that could change LMWOAs in soil. Here, four LMWOAs of oxalic acid (OA), tartaric acid (TA), malic acid (MA), and citric acid (CA) were evaluated for their roles in changing Cd and SB desorption behavior in contaminated soil with (S1-BC) or without BC (S1) produced from
Paulownia
biowaste. The results showed that OA, TA, MA, and CA reduced soil pH with rising concentrations, and biochar partially offset the pH reduction by LMWOAs. The LMWOAs reduced Cd desorption from the soil at low concentrations but increased Cd desorption at high concentrations, and CA was the most powerful in this regard. The LMWOAs had a similar effect on Sb desorption, and CA was the most effective species of LMWOAs. Adding BC to the soil affects Cd and Sb dynamics by reducing the Cd desorption but increasing Sb desorption from the soil and increasing the distribution coefficient (
K
d
) values of Cd but lowering the
K
d
values of Sb. This study helped understand the effects of LMWOAs on the geochemical behavior of Cd and Sb in the presence of biochar, as well as the potential risks of biochar amendment in enhancing Sb desorption from contaminated soil.</description><identifier>ISSN: 0269-4042</identifier><identifier>ISSN: 1573-2983</identifier><identifier>EISSN: 1573-2983</identifier><identifier>DOI: 10.1007/s10653-024-02064-6</identifier><identifier>PMID: 38970698</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Acidic soils ; Acids ; Adsorption ; biochar ; Cadmium ; Cadmium - chemistry ; Charcoal ; Charcoal - chemistry ; Citric acid ; Citric Acid - chemistry ; Desorption ; Earth and Environmental Science ; Effectiveness ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental Restoration and Remediation - methods ; Geochemistry ; Geographical distribution ; Heavy metals ; Hydrogen-Ion Concentration ; Low concentrations ; Low molecular weights ; Malates - chemistry ; Malic acid ; Metals, Heavy - chemistry ; Molecular Weight ; Organic acids ; Organic soils ; Original Paper ; Oryza - chemistry ; Oxalic acid ; Oxalic Acid - chemistry ; paddy soils ; Paulownia ; polluted soils ; Public Health ; Soil ; Soil - chemistry ; Soil amendment ; Soil contamination ; Soil pH ; Soil Pollutants - chemistry ; Soil pollution ; Soil Science & Conservation ; species ; Tartaric acid ; Tartrates - chemistry ; Terrestrial Pollution ; wastes</subject><ispartof>Environmental geochemistry and health, 2024-08, Vol.46 (8), p.289-289, Article 289</ispartof><rights>The Author(s), under exclusive licence to Springer Nature B.V. 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>2024. The Author(s), under exclusive licence to Springer Nature B.V.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c289t-e462daa677142546dc9578071673253a4fdbb5483a2afa691da04fa5abe457273</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10653-024-02064-6$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10653-024-02064-6$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51297</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38970698$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Huang, Qiuxiang</creatorcontrib><creatorcontrib>Chen, Wenzhe</creatorcontrib><creatorcontrib>Gao, Jinyan</creatorcontrib><creatorcontrib>Meng, Fande</creatorcontrib><creatorcontrib>Cai, Yongbing</creatorcontrib><creatorcontrib>Wang, Yan</creatorcontrib><creatorcontrib>Yuan, Guodong</creatorcontrib><title>Impact of low molecular weight organic acids on heavy metal(loid) desorption in biochar-amended paddy soil</title><title>Environmental geochemistry and health</title><addtitle>Environ Geochem Health</addtitle><addtitle>Environ Geochem Health</addtitle><description>Low molecular weight organic acids (LMWOAs) are important soil components and play a key role in regulating the geochemical behavior of heavy metal(loid)s. Biochar (BC) is a commonly used amendment that could change LMWOAs in soil. Here, four LMWOAs of oxalic acid (OA), tartaric acid (TA), malic acid (MA), and citric acid (CA) were evaluated for their roles in changing Cd and SB desorption behavior in contaminated soil with (S1-BC) or without BC (S1) produced from
Paulownia
biowaste. The results showed that OA, TA, MA, and CA reduced soil pH with rising concentrations, and biochar partially offset the pH reduction by LMWOAs. The LMWOAs reduced Cd desorption from the soil at low concentrations but increased Cd desorption at high concentrations, and CA was the most powerful in this regard. The LMWOAs had a similar effect on Sb desorption, and CA was the most effective species of LMWOAs. Adding BC to the soil affects Cd and Sb dynamics by reducing the Cd desorption but increasing Sb desorption from the soil and increasing the distribution coefficient (
K
d
) values of Cd but lowering the
K
d
values of Sb. This study helped understand the effects of LMWOAs on the geochemical behavior of Cd and Sb in the presence of biochar, as well as the potential risks of biochar amendment in enhancing Sb desorption from contaminated soil.</description><subject>Acidic soils</subject><subject>Acids</subject><subject>Adsorption</subject><subject>biochar</subject><subject>Cadmium</subject><subject>Cadmium - chemistry</subject><subject>Charcoal</subject><subject>Charcoal - chemistry</subject><subject>Citric acid</subject><subject>Citric Acid - chemistry</subject><subject>Desorption</subject><subject>Earth and Environmental Science</subject><subject>Effectiveness</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental Restoration and Remediation - methods</subject><subject>Geochemistry</subject><subject>Geographical distribution</subject><subject>Heavy metals</subject><subject>Hydrogen-Ion Concentration</subject><subject>Low concentrations</subject><subject>Low molecular weights</subject><subject>Malates - chemistry</subject><subject>Malic acid</subject><subject>Metals, Heavy - chemistry</subject><subject>Molecular Weight</subject><subject>Organic acids</subject><subject>Organic soils</subject><subject>Original Paper</subject><subject>Oryza - chemistry</subject><subject>Oxalic acid</subject><subject>Oxalic Acid - chemistry</subject><subject>paddy soils</subject><subject>Paulownia</subject><subject>polluted soils</subject><subject>Public Health</subject><subject>Soil</subject><subject>Soil - chemistry</subject><subject>Soil amendment</subject><subject>Soil contamination</subject><subject>Soil pH</subject><subject>Soil Pollutants - chemistry</subject><subject>Soil pollution</subject><subject>Soil Science & Conservation</subject><subject>species</subject><subject>Tartaric acid</subject><subject>Tartrates - chemistry</subject><subject>Terrestrial Pollution</subject><subject>wastes</subject><issn>0269-4042</issn><issn>1573-2983</issn><issn>1573-2983</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkU1v1DAQhi1ERZfCH-CALHEphxR_OzmiCmilSr2UszWxnV2vnDjYCdX-e9xuoRIHOFgjeZ557dGD0DtKLigh-lOhREneECbqIUo06gXaUKl5w7qWv0QbwlTXCCLYKXpdyp4Q0mnRvkKnvO00UV27QfvrcQa74DTgmO7xmKK3a4SM733Y7up93sIULAYbXMFpwjsPPw949AvE85iC-4idLynPS6jNMOE-JLuD3MDoJ-cdnsG5Ay4pxDfoZIBY_Nuneoa-f_1yd3nV3Nx-u778fNNY1nZL44ViDkBpTQWTQjnbSd0STZXmTHIQg-t7KVoODAZQHXVAxAASei-kZpqfofNj7pzTj9WXxYyhWB8jTD6txXAquVKS1LD_okQrwVj9SUU__IXu05qnusgjxYngVFWKHSmbUynZD2bOYYR8MJSYB2nmKM1UaeZRmnkYev8Uvfajd39GfluqAD8Cpbamrc_Pb_8j9hcHpaDi</recordid><startdate>20240801</startdate><enddate>20240801</enddate><creator>Huang, Qiuxiang</creator><creator>Chen, Wenzhe</creator><creator>Gao, Jinyan</creator><creator>Meng, Fande</creator><creator>Cai, Yongbing</creator><creator>Wang, Yan</creator><creator>Yuan, Guodong</creator><general>Springer Netherlands</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>7UA</scope><scope>C1K</scope><scope>F1W</scope><scope>H97</scope><scope>K9.</scope><scope>L.G</scope><scope>SOI</scope><scope>7X8</scope><scope>7S9</scope><scope>L.6</scope></search><sort><creationdate>20240801</creationdate><title>Impact of low molecular weight organic acids on heavy metal(loid) desorption in biochar-amended paddy soil</title><author>Huang, Qiuxiang ; Chen, Wenzhe ; Gao, Jinyan ; Meng, Fande ; Cai, Yongbing ; Wang, Yan ; Yuan, Guodong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c289t-e462daa677142546dc9578071673253a4fdbb5483a2afa691da04fa5abe457273</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Acidic soils</topic><topic>Acids</topic><topic>Adsorption</topic><topic>biochar</topic><topic>Cadmium</topic><topic>Cadmium - chemistry</topic><topic>Charcoal</topic><topic>Charcoal - chemistry</topic><topic>Citric acid</topic><topic>Citric Acid - chemistry</topic><topic>Desorption</topic><topic>Earth and Environmental Science</topic><topic>Effectiveness</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental Restoration and Remediation - methods</topic><topic>Geochemistry</topic><topic>Geographical distribution</topic><topic>Heavy metals</topic><topic>Hydrogen-Ion Concentration</topic><topic>Low concentrations</topic><topic>Low molecular weights</topic><topic>Malates - chemistry</topic><topic>Malic acid</topic><topic>Metals, Heavy - chemistry</topic><topic>Molecular Weight</topic><topic>Organic acids</topic><topic>Organic soils</topic><topic>Original Paper</topic><topic>Oryza - chemistry</topic><topic>Oxalic acid</topic><topic>Oxalic Acid - chemistry</topic><topic>paddy soils</topic><topic>Paulownia</topic><topic>polluted soils</topic><topic>Public Health</topic><topic>Soil</topic><topic>Soil - chemistry</topic><topic>Soil amendment</topic><topic>Soil contamination</topic><topic>Soil pH</topic><topic>Soil Pollutants - chemistry</topic><topic>Soil pollution</topic><topic>Soil Science & Conservation</topic><topic>species</topic><topic>Tartaric acid</topic><topic>Tartrates - chemistry</topic><topic>Terrestrial Pollution</topic><topic>wastes</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Huang, Qiuxiang</creatorcontrib><creatorcontrib>Chen, Wenzhe</creatorcontrib><creatorcontrib>Gao, Jinyan</creatorcontrib><creatorcontrib>Meng, Fande</creatorcontrib><creatorcontrib>Cai, Yongbing</creatorcontrib><creatorcontrib>Wang, Yan</creatorcontrib><creatorcontrib>Yuan, Guodong</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Water Resources Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 3: Aquatic Pollution & Environmental Quality</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Environment Abstracts</collection><collection>MEDLINE - Academic</collection><collection>AGRICOLA</collection><collection>AGRICOLA - Academic</collection><jtitle>Environmental geochemistry and health</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Huang, Qiuxiang</au><au>Chen, Wenzhe</au><au>Gao, Jinyan</au><au>Meng, Fande</au><au>Cai, Yongbing</au><au>Wang, Yan</au><au>Yuan, Guodong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Impact of low molecular weight organic acids on heavy metal(loid) desorption in biochar-amended paddy soil</atitle><jtitle>Environmental geochemistry and health</jtitle><stitle>Environ Geochem Health</stitle><addtitle>Environ Geochem Health</addtitle><date>2024-08-01</date><risdate>2024</risdate><volume>46</volume><issue>8</issue><spage>289</spage><epage>289</epage><pages>289-289</pages><artnum>289</artnum><issn>0269-4042</issn><issn>1573-2983</issn><eissn>1573-2983</eissn><abstract>Low molecular weight organic acids (LMWOAs) are important soil components and play a key role in regulating the geochemical behavior of heavy metal(loid)s. Biochar (BC) is a commonly used amendment that could change LMWOAs in soil. Here, four LMWOAs of oxalic acid (OA), tartaric acid (TA), malic acid (MA), and citric acid (CA) were evaluated for their roles in changing Cd and SB desorption behavior in contaminated soil with (S1-BC) or without BC (S1) produced from
Paulownia
biowaste. The results showed that OA, TA, MA, and CA reduced soil pH with rising concentrations, and biochar partially offset the pH reduction by LMWOAs. The LMWOAs reduced Cd desorption from the soil at low concentrations but increased Cd desorption at high concentrations, and CA was the most powerful in this regard. The LMWOAs had a similar effect on Sb desorption, and CA was the most effective species of LMWOAs. Adding BC to the soil affects Cd and Sb dynamics by reducing the Cd desorption but increasing Sb desorption from the soil and increasing the distribution coefficient (
K
d
) values of Cd but lowering the
K
d
values of Sb. This study helped understand the effects of LMWOAs on the geochemical behavior of Cd and Sb in the presence of biochar, as well as the potential risks of biochar amendment in enhancing Sb desorption from contaminated soil.</abstract><cop>Dordrecht</cop><pub>Springer Netherlands</pub><pmid>38970698</pmid><doi>10.1007/s10653-024-02064-6</doi><tpages>1</tpages></addata></record> |
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| subjects | Acidic soils Acids Adsorption biochar Cadmium Cadmium - chemistry Charcoal Charcoal - chemistry Citric acid Citric Acid - chemistry Desorption Earth and Environmental Science Effectiveness Environment Environmental Chemistry Environmental Health Environmental Restoration and Remediation - methods Geochemistry Geographical distribution Heavy metals Hydrogen-Ion Concentration Low concentrations Low molecular weights Malates - chemistry Malic acid Metals, Heavy - chemistry Molecular Weight Organic acids Organic soils Original Paper Oryza - chemistry Oxalic acid Oxalic Acid - chemistry paddy soils Paulownia polluted soils Public Health Soil Soil - chemistry Soil amendment Soil contamination Soil pH Soil Pollutants - chemistry Soil pollution Soil Science & Conservation species Tartaric acid Tartrates - chemistry Terrestrial Pollution wastes |
| title | Impact of low molecular weight organic acids on heavy metal(loid) desorption in biochar-amended paddy soil |
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