Characterization and photocatalytic performance of cement mortars with incorporation of TiO2 and mineral admixtures
As the main components of the building envelope, construction materials have a straight relation with air contaminants from anthropogenic origins. Titanium dioxide has been recently applied in construction industry products since its photocatalytic properties can be used for pollutant degradation pu...
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| Veröffentlicht in: | Environmental science and pollution research international 2023-09, Vol.30 (42), p.95537-95549 |
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| creator | Lara, Rancés Castillo de Castro Xavier, Gustavo Canela, Maria C. Carvalho, Juliana Alves Alexandre, Jonas de Azevedo, Afonso Rangel Garcez |
| description | As the main components of the building envelope, construction materials have a straight relation with air contaminants from anthropogenic origins. Titanium dioxide has been recently applied in construction industry products since its photocatalytic properties can be used for pollutant degradation purposes. This study evaluated the performance of cement-based mortars with the incorporation of TiO
2
nanoparticles and mineral admixtures. Six mortar compositions were defined by considering two reference mixes (with and without TiO
2
incorporation), two mineral admixtures (bentonite and metakaolin) as partial cement replacement and one waste from ornamental stone processing in two levels of partial substitution of natural sand. Consistency index, density, and entrained air content of mixtures were investigated at fresh state. Compressive strength, water absorption, sorptivity, and micrographs from scanning electron microscopy were used to characterize mortars at hardened state. It was observed that incorporation of TiO
2
does not considerably change mortar’s properties at fresh and hardened state, despite a denser microstructure and improved interfacial transition zone. In general, the relation between the water-to-cement ratio and porosity on the performances of TiO
2
-added mortars was shown, which is strongly related to their photocatalytic efficiency. Metakaolin mixtures were more efficient to NO conversion, and high selectivity was observed for the bentonite mortars. |
| doi_str_mv | 10.1007/s11356-023-29084-6 |
| format | Article |
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2
nanoparticles and mineral admixtures. Six mortar compositions were defined by considering two reference mixes (with and without TiO
2
incorporation), two mineral admixtures (bentonite and metakaolin) as partial cement replacement and one waste from ornamental stone processing in two levels of partial substitution of natural sand. Consistency index, density, and entrained air content of mixtures were investigated at fresh state. Compressive strength, water absorption, sorptivity, and micrographs from scanning electron microscopy were used to characterize mortars at hardened state. It was observed that incorporation of TiO
2
does not considerably change mortar’s properties at fresh and hardened state, despite a denser microstructure and improved interfacial transition zone. In general, the relation between the water-to-cement ratio and porosity on the performances of TiO
2
-added mortars was shown, which is strongly related to their photocatalytic efficiency. Metakaolin mixtures were more efficient to NO conversion, and high selectivity was observed for the bentonite mortars.</description><identifier>ISSN: 1614-7499</identifier><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-023-29084-6</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Admixtures ; air ; Air Content ; Air entrainment ; air pollutants ; Air pollution ; Anthropogenic factors ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Bentonite ; Building envelopes ; Cement ; compression strength ; Compressive strength ; Construction industry ; Construction materials ; Contaminants ; Earth and Environmental Science ; Ecotoxicology ; electron microscopy ; Environment ; Environmental Chemistry ; Environmental Health ; Metakaolin ; Micrography ; microstructure ; Mortars (material) ; Nanoparticles ; Performance evaluation ; Photocatalysis ; Photomicrographs ; Porosity ; Research Article ; sand ; Scanning electron microscopy ; Titanium dioxide ; Transition zone ; Waste Water Technology ; wastes ; Water absorption ; Water Management ; Water Pollution Control ; water uptake ; Water-cement ratio</subject><ispartof>Environmental science and pollution research international, 2023-09, Vol.30 (42), p.95537-95549</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c429t-66ff1a84db13d2ee8edc71e49f9e4594b561325ac608d6d369b69aea4e7407d53</citedby><cites>FETCH-LOGICAL-c429t-66ff1a84db13d2ee8edc71e49f9e4594b561325ac608d6d369b69aea4e7407d53</cites><orcidid>0000-0001-8985-2936</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-023-29084-6$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-023-29084-6$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Lara, Rancés Castillo</creatorcontrib><creatorcontrib>de Castro Xavier, Gustavo</creatorcontrib><creatorcontrib>Canela, Maria C.</creatorcontrib><creatorcontrib>Carvalho, Juliana Alves</creatorcontrib><creatorcontrib>Alexandre, Jonas</creatorcontrib><creatorcontrib>de Azevedo, Afonso Rangel Garcez</creatorcontrib><title>Characterization and photocatalytic performance of cement mortars with incorporation of TiO2 and mineral admixtures</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><description>As the main components of the building envelope, construction materials have a straight relation with air contaminants from anthropogenic origins. Titanium dioxide has been recently applied in construction industry products since its photocatalytic properties can be used for pollutant degradation purposes. This study evaluated the performance of cement-based mortars with the incorporation of TiO
2
nanoparticles and mineral admixtures. Six mortar compositions were defined by considering two reference mixes (with and without TiO
2
incorporation), two mineral admixtures (bentonite and metakaolin) as partial cement replacement and one waste from ornamental stone processing in two levels of partial substitution of natural sand. Consistency index, density, and entrained air content of mixtures were investigated at fresh state. Compressive strength, water absorption, sorptivity, and micrographs from scanning electron microscopy were used to characterize mortars at hardened state. It was observed that incorporation of TiO
2
does not considerably change mortar’s properties at fresh and hardened state, despite a denser microstructure and improved interfacial transition zone. In general, the relation between the water-to-cement ratio and porosity on the performances of TiO
2
-added mortars was shown, which is strongly related to their photocatalytic efficiency. Metakaolin mixtures were more efficient to NO conversion, and high selectivity was observed for the bentonite mortars.</description><subject>Admixtures</subject><subject>air</subject><subject>Air Content</subject><subject>Air entrainment</subject><subject>air pollutants</subject><subject>Air pollution</subject><subject>Anthropogenic factors</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Bentonite</subject><subject>Building envelopes</subject><subject>Cement</subject><subject>compression strength</subject><subject>Compressive strength</subject><subject>Construction industry</subject><subject>Construction materials</subject><subject>Contaminants</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>electron microscopy</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Metakaolin</subject><subject>Micrography</subject><subject>microstructure</subject><subject>Mortars (material)</subject><subject>Nanoparticles</subject><subject>Performance evaluation</subject><subject>Photocatalysis</subject><subject>Photomicrographs</subject><subject>Porosity</subject><subject>Research Article</subject><subject>sand</subject><subject>Scanning electron microscopy</subject><subject>Titanium dioxide</subject><subject>Transition zone</subject><subject>Waste Water Technology</subject><subject>wastes</subject><subject>Water absorption</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><subject>water uptake</subject><subject>Water-cement 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Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lara, Rancés Castillo</au><au>de Castro Xavier, Gustavo</au><au>Canela, Maria C.</au><au>Carvalho, Juliana Alves</au><au>Alexandre, Jonas</au><au>de Azevedo, Afonso Rangel Garcez</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Characterization and photocatalytic performance of cement mortars with incorporation of TiO2 and mineral admixtures</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><date>2023-09-01</date><risdate>2023</risdate><volume>30</volume><issue>42</issue><spage>95537</spage><epage>95549</epage><pages>95537-95549</pages><issn>1614-7499</issn><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>As the main components of the building envelope, construction materials have a straight relation with air contaminants from anthropogenic origins. Titanium dioxide has been recently applied in construction industry products since its photocatalytic properties can be used for pollutant degradation purposes. This study evaluated the performance of cement-based mortars with the incorporation of TiO
2
nanoparticles and mineral admixtures. Six mortar compositions were defined by considering two reference mixes (with and without TiO
2
incorporation), two mineral admixtures (bentonite and metakaolin) as partial cement replacement and one waste from ornamental stone processing in two levels of partial substitution of natural sand. Consistency index, density, and entrained air content of mixtures were investigated at fresh state. Compressive strength, water absorption, sorptivity, and micrographs from scanning electron microscopy were used to characterize mortars at hardened state. It was observed that incorporation of TiO
2
does not considerably change mortar’s properties at fresh and hardened state, despite a denser microstructure and improved interfacial transition zone. In general, the relation between the water-to-cement ratio and porosity on the performances of TiO
2
-added mortars was shown, which is strongly related to their photocatalytic efficiency. Metakaolin mixtures were more efficient to NO conversion, and high selectivity was observed for the bentonite mortars.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s11356-023-29084-6</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0001-8985-2936</orcidid><oa>free_for_read</oa></addata></record> |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Admixtures air Air Content Air entrainment air pollutants Air pollution Anthropogenic factors Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Bentonite Building envelopes Cement compression strength Compressive strength Construction industry Construction materials Contaminants Earth and Environmental Science Ecotoxicology electron microscopy Environment Environmental Chemistry Environmental Health Metakaolin Micrography microstructure Mortars (material) Nanoparticles Performance evaluation Photocatalysis Photomicrographs Porosity Research Article sand Scanning electron microscopy Titanium dioxide Transition zone Waste Water Technology wastes Water absorption Water Management Water Pollution Control water uptake Water-cement ratio |
| title | Characterization and photocatalytic performance of cement mortars with incorporation of TiO2 and mineral admixtures |
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