Heterodyne analysis of high-order partial waves in attosecond photoionization of helium
Partial wave analysis is key to interpretation of the photoionization of atoms and molecules on the attosecond timescale. Here we propose a heterodyne analysis approach, based on the delay-resolved anisotropy parameters to reveal the role played by high-order partial waves during photoionization. Th...
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| Veröffentlicht in: | Nature communications 2025-01, Vol.16 (1), p.381-8, Article 381 |
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| creator | Jiang, Wenyu Roantree, Luke Han, Lulu Ji, Jiabao Xu, Yidan Zuo, Zitan Wörner, Hans Jakob Ueda, Kiyoshi Brown, Andrew C. van der Hart, Hugo W. Gong, Xiaochun Wu, Jian |
| description | Partial wave analysis is key to interpretation of the photoionization of atoms and molecules on the attosecond timescale. Here we propose a heterodyne analysis approach, based on the delay-resolved anisotropy parameters to reveal the role played by high-order partial waves during photoionization. This extends the Reconstruction of Attosecond Beating By Interference of Two-photon Transitions technique into the few-photon regime. We demonstrate that even for moderate ( ~ 1TW/cm
2
) intensities, near-infrared-assisted photoionization of helium through Rydberg states results in a tiny contribution from the
g
0
wave, which has a significant impact on the photoelectron angular distributions via interference with the
s
- and
d
0
-waves. This modulation also causes a substantial deviation in the angular distribution of the recovered spectral phase shift. Our analysis provides an efficient method to resolve isolated partial wave contributions beyond the perturbative regime, and paves the way towards understanding resonance-enhancement of partial waves.
Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a technique used to study photoionization of atoms occurring on attosecond timescales. Here the authors implement a heterodyne approach to detect higher-order partial-waves due to multi-photon transitions, opening a path towards analysis of the strong field regime. |
| doi_str_mv | 10.1038/s41467-024-55247-1 |
| format | Article |
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2
) intensities, near-infrared-assisted photoionization of helium through Rydberg states results in a tiny contribution from the
g
0
wave, which has a significant impact on the photoelectron angular distributions via interference with the
s
- and
d
0
-waves. This modulation also causes a substantial deviation in the angular distribution of the recovered spectral phase shift. Our analysis provides an efficient method to resolve isolated partial wave contributions beyond the perturbative regime, and paves the way towards understanding resonance-enhancement of partial waves.
Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a technique used to study photoionization of atoms occurring on attosecond timescales. Here the authors implement a heterodyne approach to detect higher-order partial-waves due to multi-photon transitions, opening a path towards analysis of the strong field regime.</description><identifier>ISSN: 2041-1723</identifier><identifier>EISSN: 2041-1723</identifier><identifier>DOI: 10.1038/s41467-024-55247-1</identifier><identifier>PMID: 39753550</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/624/400/584 ; 639/766/36/2796 ; Angular distribution ; Anisotropy ; Atoms & subatomic particles ; Electrons ; Fourier transforms ; Helium ; Humanities and Social Sciences ; Infrared analysis ; Lasers ; multidisciplinary ; Photoelectrons ; Photoionization ; Photons ; Reconstruction ; Rydberg states ; Science ; Science (multidisciplinary) ; Wave analysis</subject><ispartof>Nature communications, 2025-01, Vol.16 (1), p.381-8, Article 381</ispartof><rights>The Author(s) 2025</rights><rights>2025. The Author(s).</rights><rights>Copyright Nature Publishing Group 2025</rights><rights>The Author(s) 2025 2025</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c3371-20de325b07a4f30e8677877c7a83a261c5e1ddef49f7bece1f1f8f2a29c86d433</cites><orcidid>0000-0001-5652-1495 ; 0000-0003-3986-4490 ; 0000-0002-1318-2291 ; 0000-0001-8051-8966 ; 0000-0002-5088-9835 ; 0000-0001-8225-7544</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC11698836/pdf/$$EPDF$$P50$$Gpubmedcentral$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.ncbi.nlm.nih.gov/pmc/articles/PMC11698836/$$EHTML$$P50$$Gpubmedcentral$$Hfree_for_read</linktohtml><link.rule.ids>230,314,723,776,780,860,881,2095,27903,27904,41099,42168,51554,53769,53771</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/39753550$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Jiang, Wenyu</creatorcontrib><creatorcontrib>Roantree, Luke</creatorcontrib><creatorcontrib>Han, Lulu</creatorcontrib><creatorcontrib>Ji, Jiabao</creatorcontrib><creatorcontrib>Xu, Yidan</creatorcontrib><creatorcontrib>Zuo, Zitan</creatorcontrib><creatorcontrib>Wörner, Hans Jakob</creatorcontrib><creatorcontrib>Ueda, Kiyoshi</creatorcontrib><creatorcontrib>Brown, Andrew C.</creatorcontrib><creatorcontrib>van der Hart, Hugo W.</creatorcontrib><creatorcontrib>Gong, Xiaochun</creatorcontrib><creatorcontrib>Wu, Jian</creatorcontrib><title>Heterodyne analysis of high-order partial waves in attosecond photoionization of helium</title><title>Nature communications</title><addtitle>Nat Commun</addtitle><addtitle>Nat Commun</addtitle><description>Partial wave analysis is key to interpretation of the photoionization of atoms and molecules on the attosecond timescale. Here we propose a heterodyne analysis approach, based on the delay-resolved anisotropy parameters to reveal the role played by high-order partial waves during photoionization. This extends the Reconstruction of Attosecond Beating By Interference of Two-photon Transitions technique into the few-photon regime. We demonstrate that even for moderate ( ~ 1TW/cm
2
) intensities, near-infrared-assisted photoionization of helium through Rydberg states results in a tiny contribution from the
g
0
wave, which has a significant impact on the photoelectron angular distributions via interference with the
s
- and
d
0
-waves. This modulation also causes a substantial deviation in the angular distribution of the recovered spectral phase shift. Our analysis provides an efficient method to resolve isolated partial wave contributions beyond the perturbative regime, and paves the way towards understanding resonance-enhancement of partial waves.
Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a technique used to study photoionization of atoms occurring on attosecond timescales. 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waves in attosecond photoionization of helium</atitle><jtitle>Nature communications</jtitle><stitle>Nat Commun</stitle><addtitle>Nat Commun</addtitle><date>2025-01-03</date><risdate>2025</risdate><volume>16</volume><issue>1</issue><spage>381</spage><epage>8</epage><pages>381-8</pages><artnum>381</artnum><issn>2041-1723</issn><eissn>2041-1723</eissn><abstract>Partial wave analysis is key to interpretation of the photoionization of atoms and molecules on the attosecond timescale. Here we propose a heterodyne analysis approach, based on the delay-resolved anisotropy parameters to reveal the role played by high-order partial waves during photoionization. This extends the Reconstruction of Attosecond Beating By Interference of Two-photon Transitions technique into the few-photon regime. We demonstrate that even for moderate ( ~ 1TW/cm
2
) intensities, near-infrared-assisted photoionization of helium through Rydberg states results in a tiny contribution from the
g
0
wave, which has a significant impact on the photoelectron angular distributions via interference with the
s
- and
d
0
-waves. This modulation also causes a substantial deviation in the angular distribution of the recovered spectral phase shift. Our analysis provides an efficient method to resolve isolated partial wave contributions beyond the perturbative regime, and paves the way towards understanding resonance-enhancement of partial waves.
Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a technique used to study photoionization of atoms occurring on attosecond timescales. Here the authors implement a heterodyne approach to detect higher-order partial-waves due to multi-photon transitions, opening a path towards analysis of the strong field regime.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>39753550</pmid><doi>10.1038/s41467-024-55247-1</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0001-5652-1495</orcidid><orcidid>https://orcid.org/0000-0003-3986-4490</orcidid><orcidid>https://orcid.org/0000-0002-1318-2291</orcidid><orcidid>https://orcid.org/0000-0001-8051-8966</orcidid><orcidid>https://orcid.org/0000-0002-5088-9835</orcidid><orcidid>https://orcid.org/0000-0001-8225-7544</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | 639/624/400/584 639/766/36/2796 Angular distribution Anisotropy Atoms & subatomic particles Electrons Fourier transforms Helium Humanities and Social Sciences Infrared analysis Lasers multidisciplinary Photoelectrons Photoionization Photons Reconstruction Rydberg states Science Science (multidisciplinary) Wave analysis |
| title | Heterodyne analysis of high-order partial waves in attosecond photoionization of helium |
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