Room-Temperature Optical Spin Polarization of an Electron Spin Qudit in a Vanadyl-Free Base Porphyrin Dimer

Photoexcited organic chromophores appended to molecular qubits can serve as a source of spin initialization or multilevel qudit generation for quantum information applications. So far, this approach has been primarily investigated in chromophore-stable radical systems. Here, we extend this concept t...

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Veröffentlicht in:	Journal of the American Chemical Society 2024-12
Hauptverfasser:	Privitera, Alberto, Chiesa, Alessandro, Santanni, Fabio, Carella, Angelo, Ranieri, Davide, Caneschi, Andrea, Krzyaniak, Matthew D, Young, Ryan M, Wasielewski, Michael R, Carretta, Stefano, Sessoli, Roberta
Format:	Artikel
Sprache:	eng
Online-Zugang:	Volltext
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