Porous polymers embedded with iron carbon enhanced densified activated sludge formation and wastewater treatment

[Display omitted] •The filler of iron carbon inserted porous polymers was innovatively constructed.•Combining mesh granulation and iron carbon expedited the formation of DAS.•The DAS with small particle size and good sedimentation was cultivated.•Nitrogen and phosphorus removal were significantly en...

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Veröffentlicht in:Bioresource technology 2024-12, Vol.418, p.131924, Article 131924
Hauptverfasser: Feng, Hongbo, Jin, Linyi, Yao, Yunbo, Yu, Xiaobing, Li, Lincong, Rousseau, Diederik P.L., Li, Jun
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container_start_page 131924
container_title Bioresource technology
container_volume 418
creator Feng, Hongbo
Jin, Linyi
Yao, Yunbo
Yu, Xiaobing
Li, Lincong
Rousseau, Diederik P.L.
Li, Jun
description [Display omitted] •The filler of iron carbon inserted porous polymers was innovatively constructed.•Combining mesh granulation and iron carbon expedited the formation of DAS.•The DAS with small particle size and good sedimentation was cultivated.•Nitrogen and phosphorus removal were significantly enhanced. Municipal wastewater treatment plants in China face significant challenges in effectively removing pollutants from low-strength wastewater with a low carbon-to-nitrogen (COD/N) ratio. This study proposes a novel approach incorporating porous polymers embedded with iron-carbon (PP-IC) into an activated sludge system to enhance treatment. The PP-IC accelerated the formation of densified activated sludge (DAS), characterized by small particle sizes (
doi_str_mv 10.1016/j.biortech.2024.131924
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Municipal wastewater treatment plants in China face significant challenges in effectively removing pollutants from low-strength wastewater with a low carbon-to-nitrogen (COD/N) ratio. This study proposes a novel approach incorporating porous polymers embedded with iron-carbon (PP-IC) into an activated sludge system to enhance treatment. The PP-IC accelerated the formation of densified activated sludge (DAS), characterized by small particle sizes (&lt;200 μm), excellent settleability (sludge volume index: 61 mL/g), and improved pollutant removal efficiency, with total nitrogen and total phosphorus removal rates increasing by 14.4 % and 57.4 %, respectively. DAS formation was achieved within 7 days and stabilized after 42 days. The enrichment of microorganisms, including unclassified_f_Caldilineaceae, Dechloromonas, and Candidatus Accumulibacter, further enhanced pollutant removal. Additionally, Fe2+, Fe3+ and hydroxyl radical (·OH) produced by iron-carbon micro-electrolysis supported DAS formation. Microbial interactions with the iron shavings sustained the long-term stability of the micro-electrolysis process. This synergistic mechanism significantly improved pollutant removal in wastewater treatment.</description><identifier>ISSN: 0960-8524</identifier><identifier>ISSN: 1873-2976</identifier><identifier>EISSN: 1873-2976</identifier><identifier>DOI: 10.1016/j.biortech.2024.131924</identifier><identifier>PMID: 39626807</identifier><language>eng</language><publisher>England: Elsevier Ltd</publisher><subject>Densified activated sludge ; Iron carbon ; Micro-electrolysis ; Nitrogen removal ; Phosphorus removal</subject><ispartof>Bioresource technology, 2024-12, Vol.418, p.131924, Article 131924</ispartof><rights>2024</rights><rights>Copyright © 2024. 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Municipal wastewater treatment plants in China face significant challenges in effectively removing pollutants from low-strength wastewater with a low carbon-to-nitrogen (COD/N) ratio. This study proposes a novel approach incorporating porous polymers embedded with iron-carbon (PP-IC) into an activated sludge system to enhance treatment. The PP-IC accelerated the formation of densified activated sludge (DAS), characterized by small particle sizes (&lt;200 μm), excellent settleability (sludge volume index: 61 mL/g), and improved pollutant removal efficiency, with total nitrogen and total phosphorus removal rates increasing by 14.4 % and 57.4 %, respectively. DAS formation was achieved within 7 days and stabilized after 42 days. The enrichment of microorganisms, including unclassified_f_Caldilineaceae, Dechloromonas, and Candidatus Accumulibacter, further enhanced pollutant removal. 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Municipal wastewater treatment plants in China face significant challenges in effectively removing pollutants from low-strength wastewater with a low carbon-to-nitrogen (COD/N) ratio. This study proposes a novel approach incorporating porous polymers embedded with iron-carbon (PP-IC) into an activated sludge system to enhance treatment. The PP-IC accelerated the formation of densified activated sludge (DAS), characterized by small particle sizes (&lt;200 μm), excellent settleability (sludge volume index: 61 mL/g), and improved pollutant removal efficiency, with total nitrogen and total phosphorus removal rates increasing by 14.4 % and 57.4 %, respectively. DAS formation was achieved within 7 days and stabilized after 42 days. The enrichment of microorganisms, including unclassified_f_Caldilineaceae, Dechloromonas, and Candidatus Accumulibacter, further enhanced pollutant removal. Additionally, Fe2+, Fe3+ and hydroxyl radical (·OH) produced by iron-carbon micro-electrolysis supported DAS formation. Microbial interactions with the iron shavings sustained the long-term stability of the micro-electrolysis process. This synergistic mechanism significantly improved pollutant removal in wastewater treatment.</abstract><cop>England</cop><pub>Elsevier Ltd</pub><pmid>39626807</pmid><doi>10.1016/j.biortech.2024.131924</doi><orcidid>https://orcid.org/0000-0002-9492-3601</orcidid></addata></record>
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subjects Densified activated sludge
Iron carbon
Micro-electrolysis
Nitrogen removal
Phosphorus removal
title Porous polymers embedded with iron carbon enhanced densified activated sludge formation and wastewater treatment
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