Comparative study on genesis mechanism of high arsenic groundwater in typical alluvial plain of the Upper and lower Yellow River, China

Groundwater with naturally high‑arsenic (As) concentrations is a pervasive issue across several major plains (basins) traversed by the Yellow River in China. The genesis of this high-As groundwater and its interrelationships among different plains (basins) have consistently been focal and challengin...

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Veröffentlicht in:The Science of the total environment 2024-12, Vol.957, p.177694, Article 177694
Hauptverfasser: Guo, Jiju, Cao, Wengeng, Li, Xiangzhi, Ren, Yu, Lu, Chongsheng, Wang, Yanyan, Song, Le, Liu, Yang, Sun, Xiaoyue
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container_title The Science of the total environment
container_volume 957
creator Guo, Jiju
Cao, Wengeng
Li, Xiangzhi
Ren, Yu
Lu, Chongsheng
Wang, Yanyan
Song, Le
Liu, Yang
Sun, Xiaoyue
description Groundwater with naturally high‑arsenic (As) concentrations is a pervasive issue across several major plains (basins) traversed by the Yellow River in China. The genesis of this high-As groundwater and its interrelationships among different plains (basins) have consistently been focal and challenging topics for domestic and international experts. The study focuses on the Hetao Basin in the upper Yellow River and the North Henan Plain in its lower reaches. Selecting typical profiles within the study area, a comparative analysis is performed based on the hydrochemical and isotopic signatures of these profiles. This analysis elucidates the distribution patterns, formation environments, and hydrogeochemical evolution models of high-As groundwater under the influence of different sedimentary environments. The results demonstrate that the shallow groundwater in the upper Yellow River is progressively salinizing, and conversely, the lower reaches are exhibiting a gradual alkalization. Redox conditions, the degree of evaporative concentration, and the intensity of groundwater recharge can influence the distribution disparities of high-As groundwater in the upper and lower reaches of the Yellow River. High-As groundwater in the Hetao Basin of the upper Yellow River is predominantly affected by the strength of groundwater reduction. Conversely, in the North Henan Plain of the lower Yellow River, the chemical conditions of the groundwater are more intricate, with As enrichment being influenced by a confluence of factors such as redox conditions, evaporative concentration, and the intensity of groundwater replenishment. [Display omitted] •Comparison of high arsenic groundwater in upper and lower Yellow River basins•Upstream groundwater salinizes, downstream alkalizes•High arsenic in upstream groundwater is largely due to reduction levels.•Downstream high arsenic groundwater is affected by many factors.
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The genesis of this high-As groundwater and its interrelationships among different plains (basins) have consistently been focal and challenging topics for domestic and international experts. The study focuses on the Hetao Basin in the upper Yellow River and the North Henan Plain in its lower reaches. Selecting typical profiles within the study area, a comparative analysis is performed based on the hydrochemical and isotopic signatures of these profiles. This analysis elucidates the distribution patterns, formation environments, and hydrogeochemical evolution models of high-As groundwater under the influence of different sedimentary environments. The results demonstrate that the shallow groundwater in the upper Yellow River is progressively salinizing, and conversely, the lower reaches are exhibiting a gradual alkalization. Redox conditions, the degree of evaporative concentration, and the intensity of groundwater recharge can influence the distribution disparities of high-As groundwater in the upper and lower reaches of the Yellow River. High-As groundwater in the Hetao Basin of the upper Yellow River is predominantly affected by the strength of groundwater reduction. Conversely, in the North Henan Plain of the lower Yellow River, the chemical conditions of the groundwater are more intricate, with As enrichment being influenced by a confluence of factors such as redox conditions, evaporative concentration, and the intensity of groundwater replenishment. 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Redox conditions, the degree of evaporative concentration, and the intensity of groundwater recharge can influence the distribution disparities of high-As groundwater in the upper and lower reaches of the Yellow River. High-As groundwater in the Hetao Basin of the upper Yellow River is predominantly affected by the strength of groundwater reduction. Conversely, in the North Henan Plain of the lower Yellow River, the chemical conditions of the groundwater are more intricate, with As enrichment being influenced by a confluence of factors such as redox conditions, evaporative concentration, and the intensity of groundwater replenishment. 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The genesis of this high-As groundwater and its interrelationships among different plains (basins) have consistently been focal and challenging topics for domestic and international experts. The study focuses on the Hetao Basin in the upper Yellow River and the North Henan Plain in its lower reaches. Selecting typical profiles within the study area, a comparative analysis is performed based on the hydrochemical and isotopic signatures of these profiles. This analysis elucidates the distribution patterns, formation environments, and hydrogeochemical evolution models of high-As groundwater under the influence of different sedimentary environments. The results demonstrate that the shallow groundwater in the upper Yellow River is progressively salinizing, and conversely, the lower reaches are exhibiting a gradual alkalization. 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subjects Hetao basin
High arsenic groundwater
North Henan Plain
Typical alluvial plain
Yellow River basin
title Comparative study on genesis mechanism of high arsenic groundwater in typical alluvial plain of the Upper and lower Yellow River, China
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