Stabilizing zinc anodes via engineering the active sites and pore structure of functional composite layers

Stabilizing zinc anodes via engineering the active sites and pore structure of functional composite layers

Functional composite layers composed of an amino-functionalized zirconium 1,4-dicarboxybenzene metal-organic framework were constructed on zinc anodes to mitigate the interface disturbances in aqueous batteries. These layers enable robust Zn adsorption and homogenized Zn transport and deposition kin...

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Veröffentlicht in:Chemical communications (Cambridge, England) England), 2024-09, Vol.60 (73), p.9962-9965
Hauptverfasser: Li, Kun, Chen, Jiahao, Xu, Wang, Yan, Zhongfu, Yang, Borui, Li, Ting, He, Miao, Liu, Jing, Hu, Anjun, Long, Jianping
Format: Artikel
Sprache:eng
Schlagworte:
Anodes
Metal-organic frameworks
Zinc
Zirconium
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Zusammenfassung:Functional composite layers composed of an amino-functionalized zirconium 1,4-dicarboxybenzene metal-organic framework were constructed on zinc anodes to mitigate the interface disturbances in aqueous batteries. These layers enable robust Zn adsorption and homogenized Zn transport and deposition kinetics, facilitating achieving high stability in a symmetric cell (3500 h) and a full cell (35 000 cycles, 96.7%).
ISSN:1359-7345
1364-548X
1364-548X
DOI:10.1039/d4cc03536d