On the nature of Cu-carbon interaction through N-modification for enhanced ethanol synthesis from syngas and methanol

Direct conversion of syngas into ethanol is an attractive process because of its short route and high-added value, but remains an enormous challenge due to the low selectivity caused by unclear active sites. Here, the Cu(111) supported N-modified graphene fragments C N /Cu(111) ( = 0-2) are demonstr...

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Veröffentlicht in:	Physical chemistry chemical physics : PCCP 2024-07, Vol.26 (30), p.20470-20482
Hauptverfasser:	Yang, Mingxue, Bai, Bing, Bai, Hui, Wei, Zhongzeng, Cao, Haojie, Zuo, Zhijun, Gao, Zhihua, Vinokurov, Vladimir A, Zuo, Jianping, Wang, Qiang, Huang, Wei
Format:	Artikel
Sprache:	eng
Schlagworte:	Carbon Catalysts Copper Direct conversion Doping Electron transfer Ethanol Graphene Hydrogenation Methanol Molecular orbitals Reaction mechanisms Synthesis gas
Online-Zugang:	Volltext
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