Zr-based multivariate metal-organic framework for rapid extraction of sulfonamide antibiotics from water and food samples
Based on multiple ligands strategy, a series of multivariate metal organic frameworks (MTV-MOFs) named as PCN-224-DCDPSx were prepared using one-pot solvothermal method to extract and remove sulfonamide antibiotics (SAs). The pore structure and adsorption performance can be further regulated by modu...
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creator | Gao, Yanmei Tian, Xiao Wang, Youmei Zhu, Jiawen Lou, Xuejing Qin, Mengjie Lu, Minghua Cai, Zongwei |
description | Based on multiple ligands strategy, a series of multivariate metal organic frameworks (MTV-MOFs) named as PCN-224-DCDPSx were prepared using one-pot solvothermal method to extract and remove sulfonamide antibiotics (SAs). The pore structure and adsorption performance can be further regulated by modulating the doping ratios of medium-tetra(4-carboxylphenyl) porphyrin and 4,4′-dicarboxydiphenyl sulfones. The MTV-MOFs of PCN-224-DCDPS1.0 possesses very large specific surface area (1625 m2/g). Using PCN-224-DCDPS1.0 as sorbent, a dispersive solid-phase extraction method was developed to extract and preconcentrate SAs from water, eggs, and milk prior to high performance liquid chromatography analysis. The limits of detection of method were determined between 0.17 and 0.27 ng/mL with enrichment factors ranging 214–327. The adsorption can be finished within 30 s, and the recovery rate remains above 80 % after 10 repeated uses. The adsorption capacities of sorbent were determined from 300 to 621 mg/g for sulfadiazine, sulphapyridine, sulfamethoxydiazine, sulfachlorpyridazine, sulfabenzamide, and sulfadimethoxine. The adsorption mechanisms were investigated and can be attributed to π-π interactions, hydrogen bonds, and electrostatic interactions. This work represents a method for preparation of MTV-MOFs and uses as sorbent for extraction and enrichment of trace pollutants from complex samples.
[Display omitted]
•Zr-based multivariate MOF (PCN-224-DCDPS1.0) was prepared by multiple ligands strategy.•PCN-224-DCDPS1.0 was used as sorbent for adsorption of sulfonamide antibiotics (SAs).•The sorbent has excellent crystal structure stability and adsorption performance.•The adsorption of SAs with PCN-224-DCDPS1.0 can be finished within 30 s. |
doi_str_mv | 10.1016/j.jhazmat.2024.135019 |
format | Article |
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[Display omitted]
•Zr-based multivariate MOF (PCN-224-DCDPS1.0) was prepared by multiple ligands strategy.•PCN-224-DCDPS1.0 was used as sorbent for adsorption of sulfonamide antibiotics (SAs).•The sorbent has excellent crystal structure stability and adsorption performance.•The adsorption of SAs with PCN-224-DCDPS1.0 can be finished within 30 s.</description><identifier>ISSN: 0304-3894</identifier><identifier>ISSN: 1873-3336</identifier><identifier>EISSN: 1873-3336</identifier><identifier>DOI: 10.1016/j.jhazmat.2024.135019</identifier><identifier>PMID: 38925054</identifier><language>eng</language><publisher>Netherlands: Elsevier B.V</publisher><subject>Adsorption ; Animals ; Anti-Bacterial Agents - analysis ; Anti-Bacterial Agents - chemistry ; Anti-Bacterial Agents - isolation & purification ; Chromatography, High Pressure Liquid ; Dispersive solid phase extraction ; Eggs - analysis ; Food Contamination - analysis ; Metal-Organic Frameworks - chemistry ; Milk - chemistry ; Mixed-linkers ; MTV-MOFs ; PCN-224 ; Sample pretreatment ; Solid Phase Extraction - methods ; Sulfonamide antibiotics (SAs) ; Sulfonamides - analysis ; Sulfonamides - chemistry ; Sulfonamides - isolation & purification ; Water Pollutants, Chemical - analysis ; Water Pollutants, Chemical - chemistry ; Zirconium - chemistry</subject><ispartof>Journal of hazardous materials, 2024-09, Vol.476, p.135019, Article 135019</ispartof><rights>2024 Elsevier B.V.</rights><rights>Copyright © 2024 Elsevier B.V. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c243t-c5db9896244abcbe2185b3a2c2b28b3068d60082e99e2aa25893b60c62e19e903</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.jhazmat.2024.135019$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38925054$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Gao, Yanmei</creatorcontrib><creatorcontrib>Tian, Xiao</creatorcontrib><creatorcontrib>Wang, Youmei</creatorcontrib><creatorcontrib>Zhu, Jiawen</creatorcontrib><creatorcontrib>Lou, Xuejing</creatorcontrib><creatorcontrib>Qin, Mengjie</creatorcontrib><creatorcontrib>Lu, Minghua</creatorcontrib><creatorcontrib>Cai, Zongwei</creatorcontrib><title>Zr-based multivariate metal-organic framework for rapid extraction of sulfonamide antibiotics from water and food samples</title><title>Journal of hazardous materials</title><addtitle>J Hazard Mater</addtitle><description>Based on multiple ligands strategy, a series of multivariate metal organic frameworks (MTV-MOFs) named as PCN-224-DCDPSx were prepared using one-pot solvothermal method to extract and remove sulfonamide antibiotics (SAs). The pore structure and adsorption performance can be further regulated by modulating the doping ratios of medium-tetra(4-carboxylphenyl) porphyrin and 4,4′-dicarboxydiphenyl sulfones. The MTV-MOFs of PCN-224-DCDPS1.0 possesses very large specific surface area (1625 m2/g). Using PCN-224-DCDPS1.0 as sorbent, a dispersive solid-phase extraction method was developed to extract and preconcentrate SAs from water, eggs, and milk prior to high performance liquid chromatography analysis. The limits of detection of method were determined between 0.17 and 0.27 ng/mL with enrichment factors ranging 214–327. The adsorption can be finished within 30 s, and the recovery rate remains above 80 % after 10 repeated uses. The adsorption capacities of sorbent were determined from 300 to 621 mg/g for sulfadiazine, sulphapyridine, sulfamethoxydiazine, sulfachlorpyridazine, sulfabenzamide, and sulfadimethoxine. The adsorption mechanisms were investigated and can be attributed to π-π interactions, hydrogen bonds, and electrostatic interactions. This work represents a method for preparation of MTV-MOFs and uses as sorbent for extraction and enrichment of trace pollutants from complex samples.
[Display omitted]
•Zr-based multivariate MOF (PCN-224-DCDPS1.0) was prepared by multiple ligands strategy.•PCN-224-DCDPS1.0 was used as sorbent for adsorption of sulfonamide antibiotics (SAs).•The sorbent has excellent crystal structure stability and adsorption performance.•The adsorption of SAs with PCN-224-DCDPS1.0 can be finished within 30 s.</description><subject>Adsorption</subject><subject>Animals</subject><subject>Anti-Bacterial Agents - analysis</subject><subject>Anti-Bacterial Agents - chemistry</subject><subject>Anti-Bacterial Agents - isolation & purification</subject><subject>Chromatography, High Pressure Liquid</subject><subject>Dispersive solid phase extraction</subject><subject>Eggs - analysis</subject><subject>Food Contamination - analysis</subject><subject>Metal-Organic Frameworks - chemistry</subject><subject>Milk - chemistry</subject><subject>Mixed-linkers</subject><subject>MTV-MOFs</subject><subject>PCN-224</subject><subject>Sample pretreatment</subject><subject>Solid Phase Extraction - methods</subject><subject>Sulfonamide antibiotics (SAs)</subject><subject>Sulfonamides - analysis</subject><subject>Sulfonamides - chemistry</subject><subject>Sulfonamides - isolation & purification</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>Zirconium - chemistry</subject><issn>0304-3894</issn><issn>1873-3336</issn><issn>1873-3336</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkE1v1DAQhi0EokvhJ4B85JJlbCfZ5IRQxZdUqZdy6cUa2xPwEseL7bS0vx5Xu3DlNNKr90PzMPZawFaA6N_tt_sf-BCwbCXIditUB2J8wjZi2KlGKdU_ZRtQ0DZqGNsz9iLnPQCIXdc-Z2dVkx107Ybd36TGYCbHwzoXf4vJYyEeqODcxPQdF2_5lDDQXUw_-RQTT3jwjtPvktAWHxceJ57XeYoLBu-I41K88bF4m2syBn5XG1OVXY1HxzOGw0z5JXs24Zzp1emes2-fPl5ffGkurz5_vfhw2VjZqtLYzplxGHvZtmisISmGziiUVho5GAX94HqAQdI4kkSU3TAq04PtJYmRRlDn7O2x95Dir5Vy0cFnS_OMC8U1awU7OQC0sKvW7mi1KeacaNKH5AOmey1AP1LXe32irh-p6yP1mntzmlhNIPcv9RdzNbw_Gqg-eusp6Ww9LZacT2SLdtH_Z-IPzqyYBA</recordid><startdate>20240905</startdate><enddate>20240905</enddate><creator>Gao, Yanmei</creator><creator>Tian, Xiao</creator><creator>Wang, Youmei</creator><creator>Zhu, Jiawen</creator><creator>Lou, Xuejing</creator><creator>Qin, Mengjie</creator><creator>Lu, Minghua</creator><creator>Cai, Zongwei</creator><general>Elsevier B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>20240905</creationdate><title>Zr-based multivariate metal-organic framework for rapid extraction of sulfonamide antibiotics from water and food samples</title><author>Gao, Yanmei ; Tian, Xiao ; Wang, Youmei ; Zhu, Jiawen ; Lou, Xuejing ; Qin, Mengjie ; Lu, Minghua ; Cai, Zongwei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c243t-c5db9896244abcbe2185b3a2c2b28b3068d60082e99e2aa25893b60c62e19e903</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Adsorption</topic><topic>Animals</topic><topic>Anti-Bacterial Agents - analysis</topic><topic>Anti-Bacterial Agents - chemistry</topic><topic>Anti-Bacterial Agents - isolation & purification</topic><topic>Chromatography, High Pressure Liquid</topic><topic>Dispersive solid phase extraction</topic><topic>Eggs - analysis</topic><topic>Food Contamination - analysis</topic><topic>Metal-Organic Frameworks - chemistry</topic><topic>Milk - chemistry</topic><topic>Mixed-linkers</topic><topic>MTV-MOFs</topic><topic>PCN-224</topic><topic>Sample pretreatment</topic><topic>Solid Phase Extraction - methods</topic><topic>Sulfonamide antibiotics (SAs)</topic><topic>Sulfonamides - analysis</topic><topic>Sulfonamides - chemistry</topic><topic>Sulfonamides - isolation & purification</topic><topic>Water Pollutants, Chemical - analysis</topic><topic>Water Pollutants, Chemical - chemistry</topic><topic>Zirconium - chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gao, Yanmei</creatorcontrib><creatorcontrib>Tian, Xiao</creatorcontrib><creatorcontrib>Wang, Youmei</creatorcontrib><creatorcontrib>Zhu, Jiawen</creatorcontrib><creatorcontrib>Lou, Xuejing</creatorcontrib><creatorcontrib>Qin, Mengjie</creatorcontrib><creatorcontrib>Lu, Minghua</creatorcontrib><creatorcontrib>Cai, Zongwei</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Journal of hazardous materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gao, Yanmei</au><au>Tian, Xiao</au><au>Wang, Youmei</au><au>Zhu, Jiawen</au><au>Lou, Xuejing</au><au>Qin, Mengjie</au><au>Lu, Minghua</au><au>Cai, Zongwei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Zr-based multivariate metal-organic framework for rapid extraction of sulfonamide antibiotics from water and food samples</atitle><jtitle>Journal of hazardous materials</jtitle><addtitle>J Hazard Mater</addtitle><date>2024-09-05</date><risdate>2024</risdate><volume>476</volume><spage>135019</spage><pages>135019-</pages><artnum>135019</artnum><issn>0304-3894</issn><issn>1873-3336</issn><eissn>1873-3336</eissn><abstract>Based on multiple ligands strategy, a series of multivariate metal organic frameworks (MTV-MOFs) named as PCN-224-DCDPSx were prepared using one-pot solvothermal method to extract and remove sulfonamide antibiotics (SAs). The pore structure and adsorption performance can be further regulated by modulating the doping ratios of medium-tetra(4-carboxylphenyl) porphyrin and 4,4′-dicarboxydiphenyl sulfones. The MTV-MOFs of PCN-224-DCDPS1.0 possesses very large specific surface area (1625 m2/g). Using PCN-224-DCDPS1.0 as sorbent, a dispersive solid-phase extraction method was developed to extract and preconcentrate SAs from water, eggs, and milk prior to high performance liquid chromatography analysis. The limits of detection of method were determined between 0.17 and 0.27 ng/mL with enrichment factors ranging 214–327. The adsorption can be finished within 30 s, and the recovery rate remains above 80 % after 10 repeated uses. The adsorption capacities of sorbent were determined from 300 to 621 mg/g for sulfadiazine, sulphapyridine, sulfamethoxydiazine, sulfachlorpyridazine, sulfabenzamide, and sulfadimethoxine. The adsorption mechanisms were investigated and can be attributed to π-π interactions, hydrogen bonds, and electrostatic interactions. This work represents a method for preparation of MTV-MOFs and uses as sorbent for extraction and enrichment of trace pollutants from complex samples.
[Display omitted]
•Zr-based multivariate MOF (PCN-224-DCDPS1.0) was prepared by multiple ligands strategy.•PCN-224-DCDPS1.0 was used as sorbent for adsorption of sulfonamide antibiotics (SAs).•The sorbent has excellent crystal structure stability and adsorption performance.•The adsorption of SAs with PCN-224-DCDPS1.0 can be finished within 30 s.</abstract><cop>Netherlands</cop><pub>Elsevier B.V</pub><pmid>38925054</pmid><doi>10.1016/j.jhazmat.2024.135019</doi></addata></record> |
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subjects | Adsorption Animals Anti-Bacterial Agents - analysis Anti-Bacterial Agents - chemistry Anti-Bacterial Agents - isolation & purification Chromatography, High Pressure Liquid Dispersive solid phase extraction Eggs - analysis Food Contamination - analysis Metal-Organic Frameworks - chemistry Milk - chemistry Mixed-linkers MTV-MOFs PCN-224 Sample pretreatment Solid Phase Extraction - methods Sulfonamide antibiotics (SAs) Sulfonamides - analysis Sulfonamides - chemistry Sulfonamides - isolation & purification Water Pollutants, Chemical - analysis Water Pollutants, Chemical - chemistry Zirconium - chemistry |
title | Zr-based multivariate metal-organic framework for rapid extraction of sulfonamide antibiotics from water and food samples |
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