A Plastic‐Crystal Electrolyte Layer Promotes Interfacial Stability of Ni‐Rich Oxide Cathode in Li6PS5Cl‐Based All‐Solid‐State Rechargeable Li Batteries

Unfavorable parasitic reactions between the Ni‐rich layered oxide cathode and the sulfide solid electrolyte have plagued the realization of all‐solid‐state rechargeable Li batteries. The accumulation of inactive by‐products (P2Sx, S, POxn− and SOxn−) at the cathode‐sulfide interface impedes fast Li‐...

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Veröffentlicht in:	ChemSusChem 2024-12, Vol.17 (24), p.e202400840-n/a
Hauptverfasser:	Ma, Ruojian, Liu, Yaning, Fang, Ruyi, Zhang, Jun, Wang, Ya‐Hui, Huang, Hui, Gan, Yongping, He, Xinping, Xia, Xinhui, Zhang, Wenkui, Xia, Yang, Xin, Sen
Format:	Artikel
Sprache:	eng
Schlagworte:	all-solid-state rechargeable Li batteries Cathodes Crystal lattices Cycle ratio Electrochemistry Electrode materials Electrolytes interface chemistry nickel-rich layered oxide cathode Phase transitions plastic-crystal electrolyte Reaction kinetics Rechargeable batteries Solid electrolytes Succinonitrile sulfide solid electrolyte
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