Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance
Cesium lead iodide bromide (CsPbIBr2) perovskite solar cells (PSCs) have improved stability compared to other perovskite compositions. However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (P...
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| Veröffentlicht in: | Materials horizons 2024-09, Vol.11 (18), p.4329-4337 |
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| creator | Mohammad Ismail Hossain Shahiduzzaman, Md Junayed Hossain Rafij Asman Tamang Akhtaruzzaman, Md Hamad, Almohamadi Uddin, Jamal Amin, Nowshad Nunzi, Jean-Michel Taima, Tetsuya |
| description | Cesium lead iodide bromide (CsPbIBr2) perovskite solar cells (PSCs) have improved stability compared to other perovskite compositions. However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (PCEs). This study proposes a novel device design to tailor the potential of CsPbIBr2 PSCs by improving their optoelectronic properties. An advanced 3D multiphysics approach was rigorously used to investigate the optics and electrical properties of the proposed CsPbIBr2 PSCs. This approach combines finite-difference time-domain (FDTD) and finite element method (FEM) techniques with the particle swarm optimization (PSO) algorithm. The outcome from the adapted numerical approach is in good agreement with the experimental results. The optimized CsPbIBr2 PSC demonstrates a promising power conversion efficiency (PCE) of over 16.4%, associated VOC of 1.53 V, FF of 80.6%, and JSC of 13.4 mA cm−2. Therefore, the potential of CsPbIBr2 perovskites could be further explored with continued research and development in material science and device physics. |
| doi_str_mv | 10.1039/d4mh00323c |
| format | Article |
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However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (PCEs). This study proposes a novel device design to tailor the potential of CsPbIBr2 PSCs by improving their optoelectronic properties. An advanced 3D multiphysics approach was rigorously used to investigate the optics and electrical properties of the proposed CsPbIBr2 PSCs. This approach combines finite-difference time-domain (FDTD) and finite element method (FEM) techniques with the particle swarm optimization (PSO) algorithm. The outcome from the adapted numerical approach is in good agreement with the experimental results. The optimized CsPbIBr2 PSC demonstrates a promising power conversion efficiency (PCE) of over 16.4%, associated VOC of 1.53 V, FF of 80.6%, and JSC of 13.4 mA cm−2. 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However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (PCEs). This study proposes a novel device design to tailor the potential of CsPbIBr2 PSCs by improving their optoelectronic properties. An advanced 3D multiphysics approach was rigorously used to investigate the optics and electrical properties of the proposed CsPbIBr2 PSCs. This approach combines finite-difference time-domain (FDTD) and finite element method (FEM) techniques with the particle swarm optimization (PSO) algorithm. The outcome from the adapted numerical approach is in good agreement with the experimental results. The optimized CsPbIBr2 PSC demonstrates a promising power conversion efficiency (PCE) of over 16.4%, associated VOC of 1.53 V, FF of 80.6%, and JSC of 13.4 mA cm−2. Therefore, the potential of CsPbIBr2 perovskites could be further explored with continued research and development in material science and device physics.</description><subject>Algorithms</subject><subject>Cesium</subject><subject>Electrical properties</subject><subject>Energy conversion efficiency</subject><subject>Finite element method</subject><subject>Optoelectronic devices</subject><subject>Particle swarm optimization</subject><subject>Performance enhancement</subject><subject>Perovskites</subject><subject>Photovoltaic cells</subject><subject>R&D</subject><subject>Research & development</subject><subject>Solar cells</subject><subject>Time domain analysis</subject><issn>2051-6347</issn><issn>2051-6355</issn><issn>2051-6355</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNpdjktLw0AUhQdRsNRu_AUDbtxE55F5udNitVBQRNdlMrljUyeZmEnq3zdBcSF3ce69nO9wEDqn5IoSbq7LvN4Rwhl3R2jGiKCZ5EIc_-25OkWLlPaEEMpzQTSZof0LHMCGqnnH_Q6wH0LAbeyh6SsbcPR4mZ6L9V3HcAtdPKSPqgecYrAddhBCusG2PNjGQT0iCffxy3ZlwtDspmc5UT529XScoRNvQ4LFr87R2-r-dfmYbZ4e1svbTdYyKvvMFkILpXkppZCEysIxcNp5V3hpPGitlORE5UYy6VUOVFnLKXHKKWOpyfkcXf7ktl38HCD127pKU1nbQBzSdoQZM1yPM0cX_6z7OHTN2G47RgqujTCSfwNEYWhr</recordid><startdate>20240916</startdate><enddate>20240916</enddate><creator>Mohammad Ismail Hossain</creator><creator>Shahiduzzaman, Md</creator><creator>Junayed Hossain Rafij</creator><creator>Asman Tamang</creator><creator>Akhtaruzzaman, Md</creator><creator>Hamad, Almohamadi</creator><creator>Uddin, Jamal</creator><creator>Amin, Nowshad</creator><creator>Nunzi, Jean-Michel</creator><creator>Taima, Tetsuya</creator><general>Royal Society of Chemistry</general><scope>7SR</scope><scope>7TB</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>F28</scope><scope>FR3</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope></search><sort><creationdate>20240916</creationdate><title>Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance</title><author>Mohammad Ismail Hossain ; 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However, they still face significant challenges due to their poor photovoltaic performance parameters, which limit the devices' power conversion efficiencies (PCEs). This study proposes a novel device design to tailor the potential of CsPbIBr2 PSCs by improving their optoelectronic properties. An advanced 3D multiphysics approach was rigorously used to investigate the optics and electrical properties of the proposed CsPbIBr2 PSCs. This approach combines finite-difference time-domain (FDTD) and finite element method (FEM) techniques with the particle swarm optimization (PSO) algorithm. The outcome from the adapted numerical approach is in good agreement with the experimental results. The optimized CsPbIBr2 PSC demonstrates a promising power conversion efficiency (PCE) of over 16.4%, associated VOC of 1.53 V, FF of 80.6%, and JSC of 13.4 mA cm−2. Therefore, the potential of CsPbIBr2 perovskites could be further explored with continued research and development in material science and device physics.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/d4mh00323c</doi><tpages>9</tpages></addata></record> |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Algorithms Cesium Electrical properties Energy conversion efficiency Finite element method Optoelectronic devices Particle swarm optimization Performance enhancement Perovskites Photovoltaic cells R&D Research & development Solar cells Time domain analysis |
| title | Revealing the full potential of CsPbIBr2 perovskite solar cells: advancements towards enhanced performance |
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