Moiré superlattices in twisted two-dimensional halide perovskites
Moiré superlattices have emerged as a new platform for studying strongly correlated quantum phenomena, but these systems have been largely limited to van der Waals layer two-dimensional materials. Here we introduce moiré superlattices leveraging ultrathin, ligand-free halide perovskites, facilitated...
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| Veröffentlicht in: | Nature materials 2024-09, Vol.23 (9), p.1222-1229 |
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| creator | Zhang, Shuchen Jin, Linrui Lu, Yuan Zhang, Linghai Yang, Jiaqi Zhao, Qiuchen Sun, Dewei Thompson, Joshua J. P. Yuan, Biao Ma, Ke Akriti Park, Jee Yung Lee, Yoon Ho Wei, Zitang Finkenauer, Blake P. Blach, Daria D. Kumar, Sarath Peng, Hailin Mannodi-Kanakkithodi, Arun Yu, Yi Malic, Ermin Lu, Gang Dou, Letian Huang, Libai |
| description | Moiré superlattices have emerged as a new platform for studying strongly correlated quantum phenomena, but these systems have been largely limited to van der Waals layer two-dimensional materials. Here we introduce moiré superlattices leveraging ultrathin, ligand-free halide perovskites, facilitated by ionic interactions. Square moiré superlattices with varying periodic lengths are clearly visualized through high-resolution transmission electron microscopy. Twist-angle-dependent transient photoluminescence microscopy and electrical characterizations indicate the emergence of localized bright excitons and trapped charge carriers near a twist angle of ~10°. The localized excitons are accompanied by enhanced exciton emission, attributed to an increased oscillator strength by a theoretically predicted flat band. This research showcases the promise of two-dimensional perovskites as unique room-temperature moiré materials.
The emergence of moiré superlattices in twisted two-dimensional halide perovskites has been reported, revealing the emergence of localized bright excitons with enhanced emissions and trapped charge carriers. |
| doi_str_mv | 10.1038/s41563-024-01921-0 |
| format | Article |
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The emergence of moiré superlattices in twisted two-dimensional halide perovskites has been reported, revealing the emergence of localized bright excitons with enhanced emissions and trapped charge carriers.</description><identifier>ISSN: 1476-1122</identifier><identifier>ISSN: 1476-4660</identifier><identifier>EISSN: 1476-4660</identifier><identifier>DOI: 10.1038/s41563-024-01921-0</identifier><identifier>PMID: 38906993</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>140/125 ; 639/301/1019 ; 639/301/357/404 ; Biomaterials ; Charge materials ; Chemistry ; Chemistry and Materials Science ; Condensed Matter Physics ; Crystal lattices ; Current carriers ; Electrons ; Emissions ; Engineering ; Excitons ; High resolution electron microscopy ; Ionic interactions ; Ligands ; Materials Science ; Nanotechnology ; Optical and Electronic Materials ; Perovskites ; Photoluminescence ; Physics ; Quantum phenomena ; Room temperature ; Superlattices ; Temperature ; Transmission electron microscopy ; Trapped charge ; Two dimensional materials</subject><ispartof>Nature materials, 2024-09, Vol.23 (9), p.1222-1229</ispartof><rights>The Author(s), under exclusive licence to Springer Nature Limited 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>2024. The Author(s), under exclusive licence to Springer Nature Limited.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c256t-bd08badebc574f3e0a08f5b3e717f6251e8015cb1f3d07c5ff8c0e032b536c6e3</cites><orcidid>0000-0002-1416-786X ; 0000-0003-1434-9003 ; 0000-0001-8560-0045 ; 0000-0002-9814-6563 ; 0000-0003-4326-5992 ; 0000-0002-7391-0342 ; 0000-0001-6945-6207 ; 0000-0001-6411-8591 ; 0000-0003-0536-5765 ; 0000-0001-9975-3624 ; 0000-0003-0780-1583</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38906993$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhang, Shuchen</creatorcontrib><creatorcontrib>Jin, Linrui</creatorcontrib><creatorcontrib>Lu, Yuan</creatorcontrib><creatorcontrib>Zhang, Linghai</creatorcontrib><creatorcontrib>Yang, Jiaqi</creatorcontrib><creatorcontrib>Zhao, Qiuchen</creatorcontrib><creatorcontrib>Sun, Dewei</creatorcontrib><creatorcontrib>Thompson, Joshua J. P.</creatorcontrib><creatorcontrib>Yuan, Biao</creatorcontrib><creatorcontrib>Ma, Ke</creatorcontrib><creatorcontrib>Akriti</creatorcontrib><creatorcontrib>Park, Jee Yung</creatorcontrib><creatorcontrib>Lee, Yoon Ho</creatorcontrib><creatorcontrib>Wei, Zitang</creatorcontrib><creatorcontrib>Finkenauer, Blake P.</creatorcontrib><creatorcontrib>Blach, Daria D.</creatorcontrib><creatorcontrib>Kumar, Sarath</creatorcontrib><creatorcontrib>Peng, Hailin</creatorcontrib><creatorcontrib>Mannodi-Kanakkithodi, Arun</creatorcontrib><creatorcontrib>Yu, Yi</creatorcontrib><creatorcontrib>Malic, Ermin</creatorcontrib><creatorcontrib>Lu, Gang</creatorcontrib><creatorcontrib>Dou, Letian</creatorcontrib><creatorcontrib>Huang, Libai</creatorcontrib><title>Moiré superlattices in twisted two-dimensional halide perovskites</title><title>Nature materials</title><addtitle>Nat. Mater</addtitle><addtitle>Nat Mater</addtitle><description>Moiré superlattices have emerged as a new platform for studying strongly correlated quantum phenomena, but these systems have been largely limited to van der Waals layer two-dimensional materials. Here we introduce moiré superlattices leveraging ultrathin, ligand-free halide perovskites, facilitated by ionic interactions. Square moiré superlattices with varying periodic lengths are clearly visualized through high-resolution transmission electron microscopy. Twist-angle-dependent transient photoluminescence microscopy and electrical characterizations indicate the emergence of localized bright excitons and trapped charge carriers near a twist angle of ~10°. The localized excitons are accompanied by enhanced exciton emission, attributed to an increased oscillator strength by a theoretically predicted flat band. This research showcases the promise of two-dimensional perovskites as unique room-temperature moiré materials.
The emergence of moiré superlattices in twisted two-dimensional halide perovskites has been reported, revealing the emergence of localized bright excitons with enhanced emissions and trapped charge carriers.</description><subject>140/125</subject><subject>639/301/1019</subject><subject>639/301/357/404</subject><subject>Biomaterials</subject><subject>Charge materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Condensed Matter Physics</subject><subject>Crystal lattices</subject><subject>Current carriers</subject><subject>Electrons</subject><subject>Emissions</subject><subject>Engineering</subject><subject>Excitons</subject><subject>High resolution electron microscopy</subject><subject>Ionic interactions</subject><subject>Ligands</subject><subject>Materials Science</subject><subject>Nanotechnology</subject><subject>Optical and Electronic Materials</subject><subject>Perovskites</subject><subject>Photoluminescence</subject><subject>Physics</subject><subject>Quantum phenomena</subject><subject>Room temperature</subject><subject>Superlattices</subject><subject>Temperature</subject><subject>Transmission electron microscopy</subject><subject>Trapped charge</subject><subject>Two dimensional materials</subject><issn>1476-1122</issn><issn>1476-4660</issn><issn>1476-4660</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kEtOxDAMhiME4n0BFqgSGzYFO2nSdAkjXhKIDayjNnUh0GmHpAVxJM7BxQjMABILVrbkz7-tj7EdhAMEoQ9DhlKJFHiWAhYcU1hi65jlKs2UguVFj8j5GtsI4QGAo5Rqla0JXYAqCrHOjq9659_fkjDOyLflMDhLIXFdMry4MFAda5_WbkpdcH1Xtsl92bqakkj3z-HRDRS22EpTtoG2F3WT3Z6e3EzO08vrs4vJ0WVquVRDWtWgq7Kmyso8awRBCbqRlaAc80ZxiaQBpa2wETXkVjaNtkAgeCWFsorEJtuf5858_zRSGMzUBUttW3bUj8EIyBG0zJFHdO8P-tCPPr7_SRW6kBlyHSk-p6zvQ_DUmJl309K_GgTzadjMDZto2HwZNhCXdhfRYzWl-mflW2kExBwIcdTdkf-9_U_sByOah0A</recordid><startdate>20240901</startdate><enddate>20240901</enddate><creator>Zhang, Shuchen</creator><creator>Jin, Linrui</creator><creator>Lu, Yuan</creator><creator>Zhang, Linghai</creator><creator>Yang, Jiaqi</creator><creator>Zhao, Qiuchen</creator><creator>Sun, Dewei</creator><creator>Thompson, Joshua J. 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P. ; Yuan, Biao ; Ma, Ke ; Akriti ; Park, Jee Yung ; Lee, Yoon Ho ; Wei, Zitang ; Finkenauer, Blake P. ; Blach, Daria D. ; Kumar, Sarath ; Peng, Hailin ; Mannodi-Kanakkithodi, Arun ; Yu, Yi ; Malic, Ermin ; Lu, Gang ; Dou, Letian ; Huang, Libai</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c256t-bd08badebc574f3e0a08f5b3e717f6251e8015cb1f3d07c5ff8c0e032b536c6e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>140/125</topic><topic>639/301/1019</topic><topic>639/301/357/404</topic><topic>Biomaterials</topic><topic>Charge materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Condensed Matter Physics</topic><topic>Crystal lattices</topic><topic>Current carriers</topic><topic>Electrons</topic><topic>Emissions</topic><topic>Engineering</topic><topic>Excitons</topic><topic>High resolution electron microscopy</topic><topic>Ionic interactions</topic><topic>Ligands</topic><topic>Materials Science</topic><topic>Nanotechnology</topic><topic>Optical and Electronic Materials</topic><topic>Perovskites</topic><topic>Photoluminescence</topic><topic>Physics</topic><topic>Quantum phenomena</topic><topic>Room temperature</topic><topic>Superlattices</topic><topic>Temperature</topic><topic>Transmission electron microscopy</topic><topic>Trapped charge</topic><topic>Two dimensional materials</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Shuchen</creatorcontrib><creatorcontrib>Jin, Linrui</creatorcontrib><creatorcontrib>Lu, Yuan</creatorcontrib><creatorcontrib>Zhang, Linghai</creatorcontrib><creatorcontrib>Yang, Jiaqi</creatorcontrib><creatorcontrib>Zhao, Qiuchen</creatorcontrib><creatorcontrib>Sun, Dewei</creatorcontrib><creatorcontrib>Thompson, Joshua J. 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Mater</stitle><addtitle>Nat Mater</addtitle><date>2024-09-01</date><risdate>2024</risdate><volume>23</volume><issue>9</issue><spage>1222</spage><epage>1229</epage><pages>1222-1229</pages><issn>1476-1122</issn><issn>1476-4660</issn><eissn>1476-4660</eissn><abstract>Moiré superlattices have emerged as a new platform for studying strongly correlated quantum phenomena, but these systems have been largely limited to van der Waals layer two-dimensional materials. Here we introduce moiré superlattices leveraging ultrathin, ligand-free halide perovskites, facilitated by ionic interactions. Square moiré superlattices with varying periodic lengths are clearly visualized through high-resolution transmission electron microscopy. Twist-angle-dependent transient photoluminescence microscopy and electrical characterizations indicate the emergence of localized bright excitons and trapped charge carriers near a twist angle of ~10°. The localized excitons are accompanied by enhanced exciton emission, attributed to an increased oscillator strength by a theoretically predicted flat band. This research showcases the promise of two-dimensional perovskites as unique room-temperature moiré materials.
The emergence of moiré superlattices in twisted two-dimensional halide perovskites has been reported, revealing the emergence of localized bright excitons with enhanced emissions and trapped charge carriers.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>38906993</pmid><doi>10.1038/s41563-024-01921-0</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-1416-786X</orcidid><orcidid>https://orcid.org/0000-0003-1434-9003</orcidid><orcidid>https://orcid.org/0000-0001-8560-0045</orcidid><orcidid>https://orcid.org/0000-0002-9814-6563</orcidid><orcidid>https://orcid.org/0000-0003-4326-5992</orcidid><orcidid>https://orcid.org/0000-0002-7391-0342</orcidid><orcidid>https://orcid.org/0000-0001-6945-6207</orcidid><orcidid>https://orcid.org/0000-0001-6411-8591</orcidid><orcidid>https://orcid.org/0000-0003-0536-5765</orcidid><orcidid>https://orcid.org/0000-0001-9975-3624</orcidid><orcidid>https://orcid.org/0000-0003-0780-1583</orcidid></addata></record> |
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| subjects | 140/125 639/301/1019 639/301/357/404 Biomaterials Charge materials Chemistry Chemistry and Materials Science Condensed Matter Physics Crystal lattices Current carriers Electrons Emissions Engineering Excitons High resolution electron microscopy Ionic interactions Ligands Materials Science Nanotechnology Optical and Electronic Materials Perovskites Photoluminescence Physics Quantum phenomena Room temperature Superlattices Temperature Transmission electron microscopy Trapped charge Two dimensional materials |
| title | Moiré superlattices in twisted two-dimensional halide perovskites |
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