Secondary nucleation in symmetric binary SALR mixtures
Monte Carlo simulation is used to study secondary nucleation, fissioning, or 'reproduction', of giant clusters in a symmetric binary model fluid with competing short-range (SA) and long-range (LR) interactions. Previous work [M. B. Sweatman, Mol. Phys. , 116 (15-16), 1945-1952] suggests th...
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| creator | Tan, Jiazheng Sweatman, Martin B |
| description | Monte Carlo simulation is used to study secondary nucleation, fissioning, or 'reproduction', of giant clusters in a symmetric binary model fluid with competing short-range (SA) and long-range (LR) interactions. Previous work [M. B. Sweatman,
Mol. Phys.
,
116
(15-16), 1945-1952] suggests that a pure SALR fluid can exhibit secondary nucleation if the solute concentration is slowly increased. We show this is also true for a binary symmetric SALR mixture where the cross-interactions can be tuned to generate clusters with three different kinds of structure; (i) independent clusters of each component, (ii) contact clusters of different components, and (iii) mixed clusters. In each case, the overall concentration of each component is identical. This binary model is an initial step towards using SALR fluids to model the intra-cellular space of biological cells that contain a wide range of membraneless organelles and the chemical 'soup' at the origin of life.
The cluster in symmetric binary SALR mixture can form
via
secondary nucleation. |
| doi_str_mv | 10.1039/d3cp05765h |
| format | Article |
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Mol. Phys.
,
116
(15-16), 1945-1952] suggests that a pure SALR fluid can exhibit secondary nucleation if the solute concentration is slowly increased. We show this is also true for a binary symmetric SALR mixture where the cross-interactions can be tuned to generate clusters with three different kinds of structure; (i) independent clusters of each component, (ii) contact clusters of different components, and (iii) mixed clusters. In each case, the overall concentration of each component is identical. This binary model is an initial step towards using SALR fluids to model the intra-cellular space of biological cells that contain a wide range of membraneless organelles and the chemical 'soup' at the origin of life.
The cluster in symmetric binary SALR mixture can form
via
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Mol. Phys.
,
116
(15-16), 1945-1952] suggests that a pure SALR fluid can exhibit secondary nucleation if the solute concentration is slowly increased. We show this is also true for a binary symmetric SALR mixture where the cross-interactions can be tuned to generate clusters with three different kinds of structure; (i) independent clusters of each component, (ii) contact clusters of different components, and (iii) mixed clusters. In each case, the overall concentration of each component is identical. This binary model is an initial step towards using SALR fluids to model the intra-cellular space of biological cells that contain a wide range of membraneless organelles and the chemical 'soup' at the origin of life.
The cluster in symmetric binary SALR mixture can form
via
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Mol. Phys.
,
116
(15-16), 1945-1952] suggests that a pure SALR fluid can exhibit secondary nucleation if the solute concentration is slowly increased. We show this is also true for a binary symmetric SALR mixture where the cross-interactions can be tuned to generate clusters with three different kinds of structure; (i) independent clusters of each component, (ii) contact clusters of different components, and (iii) mixed clusters. In each case, the overall concentration of each component is identical. This binary model is an initial step towards using SALR fluids to model the intra-cellular space of biological cells that contain a wide range of membraneless organelles and the chemical 'soup' at the origin of life.
The cluster in symmetric binary SALR mixture can form
via
secondary nucleation.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>38836847</pmid><doi>10.1039/d3cp05765h</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-4141-5670</orcidid><oa>free_for_read</oa></addata></record> |
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| ispartof | Physical chemistry chemical physics : PCCP, 2024-06, Vol.26 (24), p.1757-1764 |
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| language | eng |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Clusters Mixtures Monte Carlo simulation Nucleation Organelles |
| title | Secondary nucleation in symmetric binary SALR mixtures |
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