Distribution dynamics and descriptive statistical analysis of radionuclides in the farmland soils near mining areas in Southwestern Nigeria

Human exposure to ionizing radiation in the environment is mainly due to naturally occurring radionuclides in the soils, building materials and rocks, but the level may vary depending on the anthropogenic activities prevalent in each location. Presently, in Nigeria, there are concerns due to environ...

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Veröffentlicht in:Environmental geochemistry and health 2023-06, Vol.45 (6), p.3617-3636
Hauptverfasser: Njinga, Raymond L., Ogundele, Tunde L., Adebayo, Adebiyi S., Olatunji, Michael A., Olufemi, Ayodele P., Olowookere, Christopher J., Aladeniyi, Kehinde, Pereira, Alcides, Arogunjo, Muyiwa A., Tshivhase, Victor M.
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container_issue 6
container_start_page 3617
container_title Environmental geochemistry and health
container_volume 45
creator Njinga, Raymond L.
Ogundele, Tunde L.
Adebayo, Adebiyi S.
Olatunji, Michael A.
Olufemi, Ayodele P.
Olowookere, Christopher J.
Aladeniyi, Kehinde
Pereira, Alcides
Arogunjo, Muyiwa A.
Tshivhase, Victor M.
description Human exposure to ionizing radiation in the environment is mainly due to naturally occurring radionuclides in the soils, building materials and rocks, but the level may vary depending on the anthropogenic activities prevalent in each location. Presently, in Nigeria, there are concerns due to environmental health implications of all sorts of mineral mining and processing spreading across the southwestern states of the country. This work determines the activity concentrations of naturally occurring radionuclide materials (NORMs) in the farmland soil with the aim of evaluating the radiation hazards. A total of 200 composite soil samples were taken from five states in the southwest of Nigeria, close to active mining sites at the root (0.2 m) and at deep planting zones (0.5 m) for analysis by gamma-ray spectrometry using NaI(Tl) detector. The activity concentrations of natural radionuclides in the composite soil samples were determined to vary in the order of 40  K >  232 Th >  226 Ra/ 238 U for all locations. In contrast to the other locations, Olode and Igbokoda had average radium equivalent activities (Ra eq ) to be 1.6 and 1.8 times, respectively, higher than the reference limit of 370 Bqkg −1 . The estimated excess life cancer risk values were lower than the 0.29 × 10 −3 global average value for soil by United Nations on Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) and International Commission on Radiological Protection (ICRP). Negative and low skewness values of 0.61 and 1.20 were obtained for 40  K in Itagunmodi, and also 0.47 and 0.66 for 232 Th were obtained in Sagamu. The kurtosis analysis of the activity concentrations was low and negative for soil at Itagunmodi for 40  K and 226 Ra/ 238 U; Olode for 40  K and 232 Th; and Igbokoda for 226 Ra/ 238 U and 232 Th where mining activities are commonly practiced. The variation in the results has been attributed to different agriculture practices and artisanal mining operations in each location.
doi_str_mv 10.1007/s10653-022-01440-4
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identifier ISSN: 0269-4042
ispartof Environmental geochemistry and health, 2023-06, Vol.45 (6), p.3617-3636
issn 0269-4042
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source MEDLINE; SpringerLink Journals - AutoHoldings
subjects Agricultural land
Agricultural practices
agricultural soils
Analysis
Anthropogenic factors
Building materials
Construction materials
Earth and Environmental Science
Environment
Environmental Chemistry
Environmental Health
Farms
Gamma rays
Geochemistry
Health risks
Humans
International organizations
Ionizing radiation
Kurtosis
Mining
Nigeria
Norms
Original Paper
Potassium Radioisotopes - analysis
Public Health
Radiation
Radiation hazards
Radiation Monitoring
Radiation protection
Radioisotopes
Radioisotopes - analysis
Radionuclide kinetics
Radium
Radium - analysis
Radium 226
Radium isotopes
Radium radioisotopes
risk
Skewness
Soil
Soil - chemistry
Soil dynamics
Soil Pollutants, Radioactive - analysis
Soil Science & Conservation
Soils
Spectrometry
spectroscopy
Statistical analysis
Statistical methods
Terrestrial Pollution
Thorium - analysis
traditional technology
title Distribution dynamics and descriptive statistical analysis of radionuclides in the farmland soils near mining areas in Southwestern Nigeria
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