Morphology does not matter: WSe2 luminescence nanothermometry unravelled

Transition metal dichalcogenides, including WSe2, have gained significant attention as promising nanomaterials for various applications due to their unique properties. In this study, we explore the temperature-dependent photoluminescent properties of WSe2 nanomaterials to investigate their potential...

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Veröffentlicht in:Nanoscale 2024-05, Vol.16 (17), p.8470-8478
Hauptverfasser: Martínez-Merino, Paloma, Hernández-Rodríguez, Miguel A, Piñero, José C, Brites, Carlos D S, Alcántara, Rodrigo, Navas, Javier
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container_end_page 8478
container_issue 17
container_start_page 8470
container_title Nanoscale
container_volume 16
creator Martínez-Merino, Paloma
Hernández-Rodríguez, Miguel A
Piñero, José C
Brites, Carlos D S
Alcántara, Rodrigo
Navas, Javier
description Transition metal dichalcogenides, including WSe2, have gained significant attention as promising nanomaterials for various applications due to their unique properties. In this study, we explore the temperature-dependent photoluminescent properties of WSe2 nanomaterials to investigate their potential as luminescent nanothermometers. We compare the performance of WSe2 quantum dots and nanorods synthesized using sonication synthesis and hot injection methods. Our results show a distinct temperature dependence of the photoluminescence, and conventional ratiometric luminescence thermometry demonstrates comparable relative thermal sensitivity (0.68–0.80% K−1) and temperature uncertainty (1.3–1.5 K), irrespective of the morphology of the nanomaterials. By applying multiple linear regression to WSe2 quantum dots, we achieve enhanced thermal sensitivity (30% K−1) and reduced temperature uncertainty (0.1 K), highlighting the potential of WSe2 as a versatile nanothermometer for microfluidics, nanofluidics, and biomedical assays.
doi_str_mv 10.1039/d4nr00014e
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source Royal Society Of Chemistry Journals 2008-
subjects Fluidics
Luminescence
Microfluidics
Morphology
Nanofluids
Nanomaterials
Nanorods
Photoluminescence
Quantum dots
Sensitivity enhancement
Temperature dependence
Transition metal compounds
Uncertainty
title Morphology does not matter: WSe2 luminescence nanothermometry unravelled
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