Optical second harmonic generation from Pt nanowires

We have measured optical second harmonic intensity from arrays of Pt nanowires of 20 nm and 9 nm average widths, as a function of the incident and output light polarizations, the azimuthal angle, and the excitation photon energy. The nanowires were fabricated through shadow deposition on self-organi...

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Veröffentlicht in:Applied surface science 2007-09, Vol.253 (22), p.8933-8938
Hauptverfasser: Hayashi, N., Aratake, K., Okushio, R., Iwai, T., Sugawara, A., Sano, H., Mizutani, G.
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container_end_page 8938
container_issue 22
container_start_page 8933
container_title Applied surface science
container_volume 253
creator Hayashi, N.
Aratake, K.
Okushio, R.
Iwai, T.
Sugawara, A.
Sano, H.
Mizutani, G.
description We have measured optical second harmonic intensity from arrays of Pt nanowires of 20 nm and 9 nm average widths, as a function of the incident and output light polarizations, the azimuthal angle, and the excitation photon energy. The nanowires were fabricated through shadow deposition on self-organized NaCl(1 1 0) faceted templates. The anisotropy of the SH intensity from the Pt nanowires was found to be stronger than that from the Au nanowires reported previously. The effective nonlinear susceptibility element χ 222 ( 2 ) , with the suffix 2 indicating the direction [ 1   1 ¯   0 ] , was observed for Pt nanowires, although it was not observed for Au nanowires. This difference is suggested to be due to the weaker suppression of the incident fundamental fields by the depolarization field in the Pt nanowires and the larger anisotropy in the nonlinearity of Pt nanowires due to the thinner widths.
doi_str_mv 10.1016/j.apsusc.2007.05.007
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The nanowires were fabricated through shadow deposition on self-organized NaCl(1 1 0) faceted templates. The anisotropy of the SH intensity from the Pt nanowires was found to be stronger than that from the Au nanowires reported previously. The effective nonlinear susceptibility element χ 222 ( 2 ) , with the suffix 2 indicating the direction [ 1   1 ¯   0 ] , was observed for Pt nanowires, although it was not observed for Au nanowires. 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source Elsevier ScienceDirect Journals
subjects Condensed matter: electronic structure, electrical, magnetic, and optical properties
Exact sciences and technology
Frequency conversion
harmonic generation, including high-order harmonic generation
Fundamental areas of phenomenology (including applications)
Harmonic generation, frequency conversion
NaCl
Nanowire
Nonlinear optics
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures
Optical properties of nanoscale materials and structures
Optical second harmonic generation
Optics
Physics
title Optical second harmonic generation from Pt nanowires
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