Application of several advanced oxidation processes for the destruction of terephthalic acid (TPA)
Terephthalic acid (TPA) is widely applied as a raw material in making polyester fiber, polyethylene terephthalate (PET) bottles, polyester films, etc. TPA is toxic and is known to act as endocrine disruptor. TPA wastewater is traditionally treated by biological process and this study aims to evaluat...
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| Veröffentlicht in: | Journal of hazardous materials 2007-04, Vol.142 (1), p.308-314 |
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| creator | Thiruvenkatachari, Ramesh Kwon, Tae Ouk Jun, Jung Chul Balaji, Subramanian Matheswaran, Manickam Moon, Il Shik |
| description | Terephthalic acid (TPA) is widely applied as a raw material in making polyester fiber, polyethylene terephthalate (PET) bottles, polyester films, etc. TPA is toxic and is known to act as endocrine disruptor. TPA wastewater is traditionally treated by biological process and this study aims to evaluate the effectiveness of several advanced oxidation processes on TPA removal. The oxidation processes studied were: UV–TiO
2, UV–H
2O
2, UV–H
2O
2–Fe, O
3, O
3/Fe, O
3/TiO
2, UV–O
3–H
2O
2–Fe and UV–O
3–H
2O
2–Fe–TiO
2. The results indicate that the time required for the complete destruction of 50
ppm of TPA can be minimized from 10
h using UV–TiO
2 system, to less than 10
min by UV–H
2O
2–Fe–O
3 system. Some of the likely organic intermediates identified during TPA destruction include, benzoquinone, benzene, maleic acid and oxalic acid. Possible destruction pathway of TPA has been proposed. TPA degradation by various systems was also analyzed based on the reaction kinetics and operating costs. |
| doi_str_mv | 10.1016/j.jhazmat.2006.08.023 |
| format | Article |
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2, UV–H
2O
2, UV–H
2O
2–Fe, O
3, O
3/Fe, O
3/TiO
2, UV–O
3–H
2O
2–Fe and UV–O
3–H
2O
2–Fe–TiO
2. The results indicate that the time required for the complete destruction of 50
ppm of TPA can be minimized from 10
h using UV–TiO
2 system, to less than 10
min by UV–H
2O
2–Fe–O
3 system. Some of the likely organic intermediates identified during TPA destruction include, benzoquinone, benzene, maleic acid and oxalic acid. Possible destruction pathway of TPA has been proposed. TPA degradation by various systems was also analyzed based on the reaction kinetics and operating costs.</description><identifier>ISSN: 0304-3894</identifier><identifier>EISSN: 1873-3336</identifier><identifier>DOI: 10.1016/j.jhazmat.2006.08.023</identifier><identifier>PMID: 17023113</identifier><identifier>CODEN: JHMAD9</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Advanced oxidation process ; Applied sciences ; Catalysis ; Catalytic ozonation ; Catalytic reactions ; Chemical engineering ; Chemistry ; Endocrine Disruptors - chemistry ; Exact sciences and technology ; Ferric Compounds - chemistry ; General and physical chemistry ; General purification processes ; Hydrogen Peroxide - chemistry ; Kinetics ; Oxidation-Reduction ; Ozone - chemistry ; Photofenton oxidation ; Phthalic Acids - chemistry ; Pollution ; Reactors ; Terephthalic acid ; Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry ; Titanium - chemistry ; Titanium dioxide (TiO 2) ; Ultraviolet Rays ; Wastewaters ; Water Pollutants, Chemical ; Water treatment and pollution</subject><ispartof>Journal of hazardous materials, 2007-04, Vol.142 (1), p.308-314</ispartof><rights>2006</rights><rights>2008 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c496t-186d47959cfcde32dd0ad7f27b896af9054a549a8829661357c52722ebc871443</citedby><cites>FETCH-LOGICAL-c496t-186d47959cfcde32dd0ad7f27b896af9054a549a8829661357c52722ebc871443</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.jhazmat.2006.08.023$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=18639694$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/17023113$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Thiruvenkatachari, Ramesh</creatorcontrib><creatorcontrib>Kwon, Tae Ouk</creatorcontrib><creatorcontrib>Jun, Jung Chul</creatorcontrib><creatorcontrib>Balaji, Subramanian</creatorcontrib><creatorcontrib>Matheswaran, Manickam</creatorcontrib><creatorcontrib>Moon, Il Shik</creatorcontrib><title>Application of several advanced oxidation processes for the destruction of terephthalic acid (TPA)</title><title>Journal of hazardous materials</title><addtitle>J Hazard Mater</addtitle><description>Terephthalic acid (TPA) is widely applied as a raw material in making polyester fiber, polyethylene terephthalate (PET) bottles, polyester films, etc. TPA is toxic and is known to act as endocrine disruptor. TPA wastewater is traditionally treated by biological process and this study aims to evaluate the effectiveness of several advanced oxidation processes on TPA removal. The oxidation processes studied were: UV–TiO
2, UV–H
2O
2, UV–H
2O
2–Fe, O
3, O
3/Fe, O
3/TiO
2, UV–O
3–H
2O
2–Fe and UV–O
3–H
2O
2–Fe–TiO
2. The results indicate that the time required for the complete destruction of 50
ppm of TPA can be minimized from 10
h using UV–TiO
2 system, to less than 10
min by UV–H
2O
2–Fe–O
3 system. Some of the likely organic intermediates identified during TPA destruction include, benzoquinone, benzene, maleic acid and oxalic acid. Possible destruction pathway of TPA has been proposed. TPA degradation by various systems was also analyzed based on the reaction kinetics and operating costs.</description><subject>Advanced oxidation process</subject><subject>Applied sciences</subject><subject>Catalysis</subject><subject>Catalytic ozonation</subject><subject>Catalytic reactions</subject><subject>Chemical engineering</subject><subject>Chemistry</subject><subject>Endocrine Disruptors - chemistry</subject><subject>Exact sciences and technology</subject><subject>Ferric Compounds - chemistry</subject><subject>General and physical chemistry</subject><subject>General purification processes</subject><subject>Hydrogen Peroxide - chemistry</subject><subject>Kinetics</subject><subject>Oxidation-Reduction</subject><subject>Ozone - chemistry</subject><subject>Photofenton oxidation</subject><subject>Phthalic Acids - chemistry</subject><subject>Pollution</subject><subject>Reactors</subject><subject>Terephthalic acid</subject><subject>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><subject>Titanium - chemistry</subject><subject>Titanium dioxide (TiO 2)</subject><subject>Ultraviolet Rays</subject><subject>Wastewaters</subject><subject>Water Pollutants, Chemical</subject><subject>Water treatment and pollution</subject><issn>0304-3894</issn><issn>1873-3336</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2007</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkU1P3DAYhK2qVVlofwKVL0VwSOqv-OOEVghoJaT2QM-W136j9Sq7Se3sCvrrcbRBHDn58D4zHs0gdE5JTQmVPzb1Zu3-b91YM0JkTXRNGP-AFlQrXnHO5Ue0IJyIimsjTtBpzhtCCFWN-IxOqCowpXyBVsth6KJ3Y-x3uG9xhgMk12EXDm7nIeD-KYbjdUi9h5wh47ZPeFwDDpDHtPev2hESDOtx7Yohdj4GfPn4Z3n1BX1qXZfh6_yeob93t483P6uH3_e_bpYPlRdGjhXVMghlGuNbH4CzEIgLqmVqpY10rSGNcI0wTmtmpKS8Ub5hijFYea2oEPwMXRx9S9B_-xLNbmP20HVuB_0-W2a0Vo3m74LUSM0VmRybI-hTn3OC1g4pbl16tpTYaQW7sfMKdlrBEm1LsUX3bf5gv9pCeFPNtRfg-wy47F3XptJ1zG-cltxIMwW4PnJQejtESDb7CNMuMYEfbejjO1FeADJmqBY</recordid><startdate>20070402</startdate><enddate>20070402</enddate><creator>Thiruvenkatachari, Ramesh</creator><creator>Kwon, Tae Ouk</creator><creator>Jun, Jung Chul</creator><creator>Balaji, Subramanian</creator><creator>Matheswaran, Manickam</creator><creator>Moon, Il Shik</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7U7</scope><scope>C1K</scope><scope>8FD</scope><scope>FR3</scope><scope>KR7</scope></search><sort><creationdate>20070402</creationdate><title>Application of several advanced oxidation processes for the destruction of terephthalic acid (TPA)</title><author>Thiruvenkatachari, Ramesh ; Kwon, Tae Ouk ; Jun, Jung Chul ; Balaji, Subramanian ; Matheswaran, Manickam ; Moon, Il Shik</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c496t-186d47959cfcde32dd0ad7f27b896af9054a549a8829661357c52722ebc871443</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2007</creationdate><topic>Advanced oxidation process</topic><topic>Applied sciences</topic><topic>Catalysis</topic><topic>Catalytic ozonation</topic><topic>Catalytic reactions</topic><topic>Chemical engineering</topic><topic>Chemistry</topic><topic>Endocrine Disruptors - chemistry</topic><topic>Exact sciences and technology</topic><topic>Ferric Compounds - chemistry</topic><topic>General and physical chemistry</topic><topic>General purification processes</topic><topic>Hydrogen Peroxide - chemistry</topic><topic>Kinetics</topic><topic>Oxidation-Reduction</topic><topic>Ozone - chemistry</topic><topic>Photofenton oxidation</topic><topic>Phthalic Acids - chemistry</topic><topic>Pollution</topic><topic>Reactors</topic><topic>Terephthalic acid</topic><topic>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</topic><topic>Titanium - chemistry</topic><topic>Titanium dioxide (TiO 2)</topic><topic>Ultraviolet Rays</topic><topic>Wastewaters</topic><topic>Water Pollutants, Chemical</topic><topic>Water treatment and pollution</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Thiruvenkatachari, Ramesh</creatorcontrib><creatorcontrib>Kwon, Tae Ouk</creatorcontrib><creatorcontrib>Jun, Jung Chul</creatorcontrib><creatorcontrib>Balaji, Subramanian</creatorcontrib><creatorcontrib>Matheswaran, Manickam</creatorcontrib><creatorcontrib>Moon, Il Shik</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Toxicology Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><jtitle>Journal of hazardous materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Thiruvenkatachari, Ramesh</au><au>Kwon, Tae Ouk</au><au>Jun, Jung Chul</au><au>Balaji, Subramanian</au><au>Matheswaran, Manickam</au><au>Moon, Il Shik</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Application of several advanced oxidation processes for the destruction of terephthalic acid (TPA)</atitle><jtitle>Journal of hazardous materials</jtitle><addtitle>J Hazard Mater</addtitle><date>2007-04-02</date><risdate>2007</risdate><volume>142</volume><issue>1</issue><spage>308</spage><epage>314</epage><pages>308-314</pages><issn>0304-3894</issn><eissn>1873-3336</eissn><coden>JHMAD9</coden><abstract>Terephthalic acid (TPA) is widely applied as a raw material in making polyester fiber, polyethylene terephthalate (PET) bottles, polyester films, etc. TPA is toxic and is known to act as endocrine disruptor. TPA wastewater is traditionally treated by biological process and this study aims to evaluate the effectiveness of several advanced oxidation processes on TPA removal. The oxidation processes studied were: UV–TiO
2, UV–H
2O
2, UV–H
2O
2–Fe, O
3, O
3/Fe, O
3/TiO
2, UV–O
3–H
2O
2–Fe and UV–O
3–H
2O
2–Fe–TiO
2. The results indicate that the time required for the complete destruction of 50
ppm of TPA can be minimized from 10
h using UV–TiO
2 system, to less than 10
min by UV–H
2O
2–Fe–O
3 system. Some of the likely organic intermediates identified during TPA destruction include, benzoquinone, benzene, maleic acid and oxalic acid. Possible destruction pathway of TPA has been proposed. TPA degradation by various systems was also analyzed based on the reaction kinetics and operating costs.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><pmid>17023113</pmid><doi>10.1016/j.jhazmat.2006.08.023</doi><tpages>7</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0304-3894 |
| ispartof | Journal of hazardous materials, 2007-04, Vol.142 (1), p.308-314 |
| issn | 0304-3894 1873-3336 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_29887583 |
| source | MEDLINE; Access via ScienceDirect (Elsevier) |
| subjects | Advanced oxidation process Applied sciences Catalysis Catalytic ozonation Catalytic reactions Chemical engineering Chemistry Endocrine Disruptors - chemistry Exact sciences and technology Ferric Compounds - chemistry General and physical chemistry General purification processes Hydrogen Peroxide - chemistry Kinetics Oxidation-Reduction Ozone - chemistry Photofenton oxidation Phthalic Acids - chemistry Pollution Reactors Terephthalic acid Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry Titanium - chemistry Titanium dioxide (TiO 2) Ultraviolet Rays Wastewaters Water Pollutants, Chemical Water treatment and pollution |
| title | Application of several advanced oxidation processes for the destruction of terephthalic acid (TPA) |
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