Electron injection and defect passivation for high-efficiency mesoporous perovskite solar cells
Printable mesoscopic perovskite solar cells (p-MPSCs) do not require the added hole-transport layer needed in traditional p-n junctions but have also exhibited lower power conversion efficiencies of about 19%. We performed device simulation and carrier dynamics analysis to design a p-MPSC with mesop...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2024-03, Vol.383 (6688), p.1198-1204 |
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| creator | Liu, Jiale Chen, Xiayan Chen, Kaizhong Tian, Wenming Sheng, Yusong She, Bin Jiang, Youyu Zhang, Deyi Liu, Yang Qi, Jianhang Chen, Kai Ma, Yongmin Qiu, Zexiong Wang, Chaoyang Yin, Yanfeng Zhao, Shengli Leng, Jing Jin, Shengye Zhao, Wenshan Qin, Yanyang Su, Yaqiong Li, Xiaoyu Li, Xiaojiang Zhou, Yang Zhou, Yinhua Ling, Furi Mei, Anyi Han, Hongwei |
| description | Printable mesoscopic perovskite solar cells (p-MPSCs) do not require the added hole-transport layer needed in traditional p-n junctions but have also exhibited lower power conversion efficiencies of about 19%. We performed device simulation and carrier dynamics analysis to design a p-MPSC with mesoporous layers of semiconducting titanium dioxide, insulating zirconium dioxide, and conducting carbon infiltrated with perovskite that enabled three-dimensional injection of photoexcited electrons into titanium dioxide for collection at a transparent conductor layer. Holes underwent long-distance diffusion toward the carbon back electrode, and this carrier separation reduced recombination at the back contact. Nonradiative recombination at the bulk titanium dioxide/perovskite interface was reduced by ammonium phosphate modification. The resulting p-MPSCs achieved a power conversion efficiency of 22.2% and maintained 97% of their initial efficiency after 750 hours of maximum power point tracking at 55 ± 5°C. |
| doi_str_mv | 10.1126/science.adk9089 |
| format | Article |
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We performed device simulation and carrier dynamics analysis to design a p-MPSC with mesoporous layers of semiconducting titanium dioxide, insulating zirconium dioxide, and conducting carbon infiltrated with perovskite that enabled three-dimensional injection of photoexcited electrons into titanium dioxide for collection at a transparent conductor layer. Holes underwent long-distance diffusion toward the carbon back electrode, and this carrier separation reduced recombination at the back contact. Nonradiative recombination at the bulk titanium dioxide/perovskite interface was reduced by ammonium phosphate modification. The resulting p-MPSCs achieved a power conversion efficiency of 22.2% and maintained 97% of their initial efficiency after 750 hours of maximum power point tracking at 55 ± 5°C.</description><identifier>ISSN: 0036-8075</identifier><identifier>EISSN: 1095-9203</identifier><identifier>DOI: 10.1126/science.adk9089</identifier><identifier>PMID: 38484055</identifier><language>eng</language><publisher>United States: The American Association for the Advancement of Science</publisher><subject>Ammonium ; Ammonium phosphates ; Defects ; Energy conversion efficiency ; Injection ; Maximum power tracking ; Passivity ; Perovskites ; Photovoltaic cells ; Solar cells ; Titanium dioxide ; Titanium oxide ; Titanium oxides ; Zirconium ; Zirconium dioxide</subject><ispartof>Science (American Association for the Advancement of Science), 2024-03, Vol.383 (6688), p.1198-1204</ispartof><rights>Copyright © 2024 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c325t-c47fdf511e93b30fd4200bf8612b344dc78f2df0db93af1923417f94c4d8472a3</citedby><cites>FETCH-LOGICAL-c325t-c47fdf511e93b30fd4200bf8612b344dc78f2df0db93af1923417f94c4d8472a3</cites><orcidid>0000-0002-8142-853X ; 0009-0002-6871-2007 ; 0000-0002-3738-6766 ; 0009-0007-7615-833X ; 0009-0006-1347-8654 ; 0000-0002-8454-4835 ; 0000-0003-1114-8943 ; 0000-0002-5259-7027 ; 0000-0002-8345-1178 ; 0000-0001-6424-9962 ; 0000-0001-5581-5352 ; 0000-0003-0235-6652</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,778,782,2873,2874,27907,27908</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38484055$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liu, Jiale</creatorcontrib><creatorcontrib>Chen, Xiayan</creatorcontrib><creatorcontrib>Chen, Kaizhong</creatorcontrib><creatorcontrib>Tian, Wenming</creatorcontrib><creatorcontrib>Sheng, Yusong</creatorcontrib><creatorcontrib>She, Bin</creatorcontrib><creatorcontrib>Jiang, Youyu</creatorcontrib><creatorcontrib>Zhang, Deyi</creatorcontrib><creatorcontrib>Liu, Yang</creatorcontrib><creatorcontrib>Qi, Jianhang</creatorcontrib><creatorcontrib>Chen, Kai</creatorcontrib><creatorcontrib>Ma, Yongmin</creatorcontrib><creatorcontrib>Qiu, Zexiong</creatorcontrib><creatorcontrib>Wang, Chaoyang</creatorcontrib><creatorcontrib>Yin, Yanfeng</creatorcontrib><creatorcontrib>Zhao, Shengli</creatorcontrib><creatorcontrib>Leng, Jing</creatorcontrib><creatorcontrib>Jin, Shengye</creatorcontrib><creatorcontrib>Zhao, Wenshan</creatorcontrib><creatorcontrib>Qin, Yanyang</creatorcontrib><creatorcontrib>Su, Yaqiong</creatorcontrib><creatorcontrib>Li, Xiaoyu</creatorcontrib><creatorcontrib>Li, Xiaojiang</creatorcontrib><creatorcontrib>Zhou, Yang</creatorcontrib><creatorcontrib>Zhou, Yinhua</creatorcontrib><creatorcontrib>Ling, Furi</creatorcontrib><creatorcontrib>Mei, Anyi</creatorcontrib><creatorcontrib>Han, Hongwei</creatorcontrib><title>Electron injection and defect passivation for high-efficiency mesoporous perovskite solar cells</title><title>Science (American Association for the Advancement of Science)</title><addtitle>Science</addtitle><description>Printable mesoscopic perovskite solar cells (p-MPSCs) do not require the added hole-transport layer needed in traditional p-n junctions but have also exhibited lower power conversion efficiencies of about 19%. We performed device simulation and carrier dynamics analysis to design a p-MPSC with mesoporous layers of semiconducting titanium dioxide, insulating zirconium dioxide, and conducting carbon infiltrated with perovskite that enabled three-dimensional injection of photoexcited electrons into titanium dioxide for collection at a transparent conductor layer. Holes underwent long-distance diffusion toward the carbon back electrode, and this carrier separation reduced recombination at the back contact. Nonradiative recombination at the bulk titanium dioxide/perovskite interface was reduced by ammonium phosphate modification. The resulting p-MPSCs achieved a power conversion efficiency of 22.2% and maintained 97% of their initial efficiency after 750 hours of maximum power point tracking at 55 ± 5°C.</description><subject>Ammonium</subject><subject>Ammonium phosphates</subject><subject>Defects</subject><subject>Energy conversion efficiency</subject><subject>Injection</subject><subject>Maximum power tracking</subject><subject>Passivity</subject><subject>Perovskites</subject><subject>Photovoltaic cells</subject><subject>Solar cells</subject><subject>Titanium dioxide</subject><subject>Titanium oxide</subject><subject>Titanium oxides</subject><subject>Zirconium</subject><subject>Zirconium 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injection and defect passivation for high-efficiency mesoporous perovskite solar cells</title><author>Liu, Jiale ; Chen, Xiayan ; Chen, Kaizhong ; Tian, Wenming ; Sheng, Yusong ; She, Bin ; Jiang, Youyu ; Zhang, Deyi ; Liu, Yang ; Qi, Jianhang ; Chen, Kai ; Ma, Yongmin ; Qiu, Zexiong ; Wang, Chaoyang ; Yin, Yanfeng ; Zhao, Shengli ; Leng, Jing ; Jin, Shengye ; Zhao, Wenshan ; Qin, Yanyang ; Su, Yaqiong ; Li, Xiaoyu ; Li, Xiaojiang ; Zhou, Yang ; Zhou, Yinhua ; Ling, Furi ; Mei, Anyi ; Han, Hongwei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c325t-c47fdf511e93b30fd4200bf8612b344dc78f2df0db93af1923417f94c4d8472a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Ammonium</topic><topic>Ammonium phosphates</topic><topic>Defects</topic><topic>Energy conversion efficiency</topic><topic>Injection</topic><topic>Maximum power 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We performed device simulation and carrier dynamics analysis to design a p-MPSC with mesoporous layers of semiconducting titanium dioxide, insulating zirconium dioxide, and conducting carbon infiltrated with perovskite that enabled three-dimensional injection of photoexcited electrons into titanium dioxide for collection at a transparent conductor layer. Holes underwent long-distance diffusion toward the carbon back electrode, and this carrier separation reduced recombination at the back contact. Nonradiative recombination at the bulk titanium dioxide/perovskite interface was reduced by ammonium phosphate modification. 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| ispartof | Science (American Association for the Advancement of Science), 2024-03, Vol.383 (6688), p.1198-1204 |
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| language | eng |
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| source | American Association for the Advancement of Science |
| subjects | Ammonium Ammonium phosphates Defects Energy conversion efficiency Injection Maximum power tracking Passivity Perovskites Photovoltaic cells Solar cells Titanium dioxide Titanium oxide Titanium oxides Zirconium Zirconium dioxide |
| title | Electron injection and defect passivation for high-efficiency mesoporous perovskite solar cells |
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