Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis
A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al 2O 3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the select...
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Veröffentlicht in: | Applied catalysis. A, General General, 2005-04, Vol.283 (1), p.39-46 |
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container_title | Applied catalysis. A, General |
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creator | Bradford, Michael C.J. Te, Mure Pollack, Allen |
description | A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al
2O
3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al
2O
3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors. |
doi_str_mv | 10.1016/j.apcata.2004.12.032 |
format | Article |
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2O
3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al
2O
3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors.</description><identifier>ISSN: 0926-860X</identifier><identifier>EISSN: 1873-3875</identifier><identifier>DOI: 10.1016/j.apcata.2004.12.032</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Catalysis ; Chemistry ; Colloidal state and disperse state ; Exact sciences and technology ; Fischer–Tropsch ; General and physical chemistry ; Membrane reactor ; Membranes ; Monolith loop ; Natural gas conversion ; Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><ispartof>Applied catalysis. A, General, 2005-04, Vol.283 (1), p.39-46</ispartof><rights>2005 Elsevier B.V.</rights><rights>2005 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c404t-9f27b6c17091128027e3b48c01a24dbe358826cbaaa419e087286ef39d4269d83</citedby><cites>FETCH-LOGICAL-c404t-9f27b6c17091128027e3b48c01a24dbe358826cbaaa419e087286ef39d4269d83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.apcata.2004.12.032$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=16653200$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Bradford, Michael C.J.</creatorcontrib><creatorcontrib>Te, Mure</creatorcontrib><creatorcontrib>Pollack, Allen</creatorcontrib><title>Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis</title><title>Applied catalysis. A, General</title><description>A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al
2O
3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al
2O
3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors.</description><subject>Catalysis</subject><subject>Chemistry</subject><subject>Colloidal state and disperse state</subject><subject>Exact sciences and technology</subject><subject>Fischer–Tropsch</subject><subject>General and physical chemistry</subject><subject>Membrane reactor</subject><subject>Membranes</subject><subject>Monolith loop</subject><subject>Natural gas conversion</subject><subject>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><issn>0926-860X</issn><issn>1873-3875</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><recordid>eNp9kLFOwzAQhi0EEqXwBgxZYEuwHcexFyRUUYpUxFIkNstxLqqrpA52itSNd-ANeRJcpRIbg3Uevvvv7kPomuCMYMLvNpnujR50RjFmGaEZzukJmhBR5mkuyuIUTbCkPBUcv5-jixA2GGPKZDFBixe3da0d1knrXJ8cUtr9YE3SQVd5vYXEgzaD80kT39wGswb_8_W98q6P_yTst8Magg2X6KzRbYCrY52it_njarZIl69Pz7OHZWoYZkMqG1pW3JASS0KowLSEvGLCYKIpqyvICyEoN5XWmhEJWJRUcGhyWTPKZS3yKbodc3vvPnYQBtXFpaBt465uFxSVBZNCygiyETTeheChUb23nfZ7RbA6aFMbNWpTB22KUBW1xbabY74ORrdNdGBs-OvlvMgjH7n7kYN47KcFr4KxsDVQWw9mULWz_w_6Bal1hc8</recordid><startdate>20050408</startdate><enddate>20050408</enddate><creator>Bradford, Michael C.J.</creator><creator>Te, Mure</creator><creator>Pollack, Allen</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>20050408</creationdate><title>Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis</title><author>Bradford, Michael C.J. ; Te, Mure ; Pollack, Allen</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c404t-9f27b6c17091128027e3b48c01a24dbe358826cbaaa419e087286ef39d4269d83</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2005</creationdate><topic>Catalysis</topic><topic>Chemistry</topic><topic>Colloidal state and disperse state</topic><topic>Exact sciences and technology</topic><topic>Fischer–Tropsch</topic><topic>General and physical chemistry</topic><topic>Membrane reactor</topic><topic>Membranes</topic><topic>Monolith loop</topic><topic>Natural gas conversion</topic><topic>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Bradford, Michael C.J.</creatorcontrib><creatorcontrib>Te, Mure</creatorcontrib><creatorcontrib>Pollack, Allen</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied catalysis. A, General</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bradford, Michael C.J.</au><au>Te, Mure</au><au>Pollack, Allen</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis</atitle><jtitle>Applied catalysis. A, General</jtitle><date>2005-04-08</date><risdate>2005</risdate><volume>283</volume><issue>1</issue><spage>39</spage><epage>46</epage><pages>39-46</pages><issn>0926-860X</issn><eissn>1873-3875</eissn><abstract>A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al
2O
3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al
2O
3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.apcata.2004.12.032</doi><tpages>8</tpages></addata></record> |
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subjects | Catalysis Chemistry Colloidal state and disperse state Exact sciences and technology Fischer–Tropsch General and physical chemistry Membrane reactor Membranes Monolith loop Natural gas conversion Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry |
title | Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis |
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