Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis

A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al 2O 3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the select...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Applied catalysis. A, General General, 2005-04, Vol.283 (1), p.39-46
Hauptverfasser: Bradford, Michael C.J., Te, Mure, Pollack, Allen
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 46
container_issue 1
container_start_page 39
container_title Applied catalysis. A, General
container_volume 283
creator Bradford, Michael C.J.
Te, Mure
Pollack, Allen
description A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al 2O 3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al 2O 3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors.
doi_str_mv 10.1016/j.apcata.2004.12.032
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_29549899</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S0926860X04010191</els_id><sourcerecordid>29549899</sourcerecordid><originalsourceid>FETCH-LOGICAL-c404t-9f27b6c17091128027e3b48c01a24dbe358826cbaaa419e087286ef39d4269d83</originalsourceid><addsrcrecordid>eNp9kLFOwzAQhi0EEqXwBgxZYEuwHcexFyRUUYpUxFIkNstxLqqrpA52itSNd-ANeRJcpRIbg3Uevvvv7kPomuCMYMLvNpnujR50RjFmGaEZzukJmhBR5mkuyuIUTbCkPBUcv5-jixA2GGPKZDFBixe3da0d1knrXJ8cUtr9YE3SQVd5vYXEgzaD80kT39wGswb_8_W98q6P_yTst8Magg2X6KzRbYCrY52it_njarZIl69Pz7OHZWoYZkMqG1pW3JASS0KowLSEvGLCYKIpqyvICyEoN5XWmhEJWJRUcGhyWTPKZS3yKbodc3vvPnYQBtXFpaBt465uFxSVBZNCygiyETTeheChUb23nfZ7RbA6aFMbNWpTB22KUBW1xbabY74ORrdNdGBs-OvlvMgjH7n7kYN47KcFr4KxsDVQWw9mULWz_w_6Bal1hc8</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>29549899</pqid></control><display><type>article</type><title>Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis</title><source>Access via ScienceDirect (Elsevier)</source><creator>Bradford, Michael C.J. ; Te, Mure ; Pollack, Allen</creator><creatorcontrib>Bradford, Michael C.J. ; Te, Mure ; Pollack, Allen</creatorcontrib><description>A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al 2O 3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al 2O 3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors.</description><identifier>ISSN: 0926-860X</identifier><identifier>EISSN: 1873-3875</identifier><identifier>DOI: 10.1016/j.apcata.2004.12.032</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Catalysis ; Chemistry ; Colloidal state and disperse state ; Exact sciences and technology ; Fischer–Tropsch ; General and physical chemistry ; Membrane reactor ; Membranes ; Monolith loop ; Natural gas conversion ; Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><ispartof>Applied catalysis. A, General, 2005-04, Vol.283 (1), p.39-46</ispartof><rights>2005 Elsevier B.V.</rights><rights>2005 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c404t-9f27b6c17091128027e3b48c01a24dbe358826cbaaa419e087286ef39d4269d83</citedby><cites>FETCH-LOGICAL-c404t-9f27b6c17091128027e3b48c01a24dbe358826cbaaa419e087286ef39d4269d83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.apcata.2004.12.032$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&amp;idt=16653200$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Bradford, Michael C.J.</creatorcontrib><creatorcontrib>Te, Mure</creatorcontrib><creatorcontrib>Pollack, Allen</creatorcontrib><title>Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis</title><title>Applied catalysis. A, General</title><description>A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al 2O 3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al 2O 3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors.</description><subject>Catalysis</subject><subject>Chemistry</subject><subject>Colloidal state and disperse state</subject><subject>Exact sciences and technology</subject><subject>Fischer–Tropsch</subject><subject>General and physical chemistry</subject><subject>Membrane reactor</subject><subject>Membranes</subject><subject>Monolith loop</subject><subject>Natural gas conversion</subject><subject>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><issn>0926-860X</issn><issn>1873-3875</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><recordid>eNp9kLFOwzAQhi0EEqXwBgxZYEuwHcexFyRUUYpUxFIkNstxLqqrpA52itSNd-ANeRJcpRIbg3Uevvvv7kPomuCMYMLvNpnujR50RjFmGaEZzukJmhBR5mkuyuIUTbCkPBUcv5-jixA2GGPKZDFBixe3da0d1knrXJ8cUtr9YE3SQVd5vYXEgzaD80kT39wGswb_8_W98q6P_yTst8Magg2X6KzRbYCrY52it_njarZIl69Pz7OHZWoYZkMqG1pW3JASS0KowLSEvGLCYKIpqyvICyEoN5XWmhEJWJRUcGhyWTPKZS3yKbodc3vvPnYQBtXFpaBt465uFxSVBZNCygiyETTeheChUb23nfZ7RbA6aFMbNWpTB22KUBW1xbabY74ORrdNdGBs-OvlvMgjH7n7kYN47KcFr4KxsDVQWw9mULWz_w_6Bal1hc8</recordid><startdate>20050408</startdate><enddate>20050408</enddate><creator>Bradford, Michael C.J.</creator><creator>Te, Mure</creator><creator>Pollack, Allen</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>20050408</creationdate><title>Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis</title><author>Bradford, Michael C.J. ; Te, Mure ; Pollack, Allen</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c404t-9f27b6c17091128027e3b48c01a24dbe358826cbaaa419e087286ef39d4269d83</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2005</creationdate><topic>Catalysis</topic><topic>Chemistry</topic><topic>Colloidal state and disperse state</topic><topic>Exact sciences and technology</topic><topic>Fischer–Tropsch</topic><topic>General and physical chemistry</topic><topic>Membrane reactor</topic><topic>Membranes</topic><topic>Monolith loop</topic><topic>Natural gas conversion</topic><topic>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Bradford, Michael C.J.</creatorcontrib><creatorcontrib>Te, Mure</creatorcontrib><creatorcontrib>Pollack, Allen</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Applied catalysis. A, General</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bradford, Michael C.J.</au><au>Te, Mure</au><au>Pollack, Allen</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis</atitle><jtitle>Applied catalysis. A, General</jtitle><date>2005-04-08</date><risdate>2005</risdate><volume>283</volume><issue>1</issue><spage>39</spage><epage>46</epage><pages>39-46</pages><issn>0926-860X</issn><eissn>1873-3875</eissn><abstract>A monolith loop catalytic membrane reactor (ML-CMR) concept for Fischer–Tropsch synthesis (FTS) was investigated by evaluating the performance of a P/Pt–Co/γ-Al 2O 3 catalyst in a prototype, tubular CMR and in a tubular, fixed-bed reactor (FBR). Although experimental data demonstrate that the selectivity to paraffins and the product yield per unit catalyst mass exhibited by the P/Pt–Co/γ-Al 2O 3 catalyst in the tubular CMR exceed those observed by the same catalyst in a tubular FBR, simple model calculations indicate that the ML-CMR product yield per unit reactor volume, at its present stage of development, is less than that for state-of-the-art multi-tubular fixed-bed and slurry-bubble column reactors.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.apcata.2004.12.032</doi><tpages>8</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0926-860X
ispartof Applied catalysis. A, General, 2005-04, Vol.283 (1), p.39-46
issn 0926-860X
1873-3875
language eng
recordid cdi_proquest_miscellaneous_29549899
source Access via ScienceDirect (Elsevier)
subjects Catalysis
Chemistry
Colloidal state and disperse state
Exact sciences and technology
Fischer–Tropsch
General and physical chemistry
Membrane reactor
Membranes
Monolith loop
Natural gas conversion
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
title Monolith loop catalytic membrane reactor for Fischer–Tropsch synthesis
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-26T00%3A00%3A47IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Monolith%20loop%20catalytic%20membrane%20reactor%20for%20Fischer%E2%80%93Tropsch%20synthesis&rft.jtitle=Applied%20catalysis.%20A,%20General&rft.au=Bradford,%20Michael%20C.J.&rft.date=2005-04-08&rft.volume=283&rft.issue=1&rft.spage=39&rft.epage=46&rft.pages=39-46&rft.issn=0926-860X&rft.eissn=1873-3875&rft_id=info:doi/10.1016/j.apcata.2004.12.032&rft_dat=%3Cproquest_cross%3E29549899%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=29549899&rft_id=info:pmid/&rft_els_id=S0926860X04010191&rfr_iscdi=true