Quantum dynamics of laser-induced desorption from metal and semiconductor surfaces, and related phenomena

Quantum dynamics of laser-induced desorption from metal and semiconductor surfaces, and related phenomena

Recent progress towards a quantum theory of laser-induced desorption and related phenomena is reviewed, for specific examples. These comprise the photodesorption of NO from Pt(111), the scanning tunnelling microscope and laser-induced desorption and switching of H at Si(100), and the electron stimul...

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Veröffentlicht in:Journal of physics. Condensed matter 2006-08, Vol.18 (30), p.S1425-S1459
Hauptverfasser: Saalfrank, Peter, Nest, Mathias, Andrianov, Ivan, Klamroth, Tillmann, Kröner, Dominik, Beyvers, Stephanie
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container_issue 30
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container_title Journal of physics. Condensed matter
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creator Saalfrank, Peter
Nest, Mathias
Andrianov, Ivan
Klamroth, Tillmann
Kröner, Dominik
Beyvers, Stephanie
description Recent progress towards a quantum theory of laser-induced desorption and related phenomena is reviewed, for specific examples. These comprise the photodesorption of NO from Pt(111), the scanning tunnelling microscope and laser-induced desorption and switching of H at Si(100), and the electron stimulated desorption and dissociation of CO at Ru(0001). The theoretical methods used for nuclear dynamics range from open-system density matrix theory over nonadiabatically coupled multi-state models to electron-nuclear wavepackets. Also, aspects of time-dependent spectroscopy to probe ultrafast nonadiabatic processes at surfaces will be considered for the example of two-photon photoemission of solvated electrons in ice layers on Cu(111).
doi_str_mv 10.1088/0953-8984/18/30/S05
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title Quantum dynamics of laser-induced desorption from metal and semiconductor surfaces, and related phenomena
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