Target-regulated photoactivities of CdS/Ni-MOF heterojunction with [Ru(bpy)2dppz]2+ intercalator: a bisphenol A photoelectrochemical aptasensor
Bisphenol A (BPA), an important endocrine disrupting compound, has infiltrated human daily lives through electronic devices, food containers, and children’s toys. Developing of novel BPA assay methods with high sensitivity holds tremendous importance in valuing the pollution state. Here, we construc...
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Veröffentlicht in: | Mikrochimica acta (1966) 2024-03, Vol.191 (3), p.139-139, Article 139 |
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creator | Tanjung, Aisyah Protonia Yin, Ke Zhao, Lei Wu, Jiang-Zhou Wang, Ai-Jun Mei, Li-Ping Song, Pei Feng, Jiu-Ju |
description | Bisphenol A (BPA), an important endocrine disrupting compound, has infiltrated human daily lives through electronic devices, food containers, and children’s toys. Developing of novel BPA assay methods with high sensitivity holds tremendous importance in valuing the pollution state. Here, we constructed an ultrasensitive photoelectrochemical (PEC) aptasensor for BPA determination by regulating photoactivities of CdS/Ni-based metal–organic framework (CdS/Ni-MOF) with [Ru(bpy)
2
dppz]
2+
sensitizer. CdS/Ni-MOF spheres exhibited excellent photocatalytic performance, serving as a potential sensing platform for the construction of target recognition process. [Ru(bpy)
2
dppz]
2+
were embedded into DNA double-stranded structure, functioning as sensitizer for modulating the signal response of the developed PEC aptasensor. The proposed PEC sensor exhibited outstanding analytical performances, including a wide linear range (0.1 to 1000.0 nM), low detection limit (0.026 nM, at 3σ/m), excellent selectivity, and high stability. This work provides a perspective for the design of ideal photosensitive materials and signal amplification strategies and extends their application in environment analysis.
Graphical Abstract |
doi_str_mv | 10.1007/s00604-024-06230-6 |
format | Article |
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2
dppz]
2+
sensitizer. CdS/Ni-MOF spheres exhibited excellent photocatalytic performance, serving as a potential sensing platform for the construction of target recognition process. [Ru(bpy)
2
dppz]
2+
were embedded into DNA double-stranded structure, functioning as sensitizer for modulating the signal response of the developed PEC aptasensor. The proposed PEC sensor exhibited outstanding analytical performances, including a wide linear range (0.1 to 1000.0 nM), low detection limit (0.026 nM, at 3σ/m), excellent selectivity, and high stability. This work provides a perspective for the design of ideal photosensitive materials and signal amplification strategies and extends their application in environment analysis.
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2
dppz]
2+
sensitizer. CdS/Ni-MOF spheres exhibited excellent photocatalytic performance, serving as a potential sensing platform for the construction of target recognition process. [Ru(bpy)
2
dppz]
2+
were embedded into DNA double-stranded structure, functioning as sensitizer for modulating the signal response of the developed PEC aptasensor. The proposed PEC sensor exhibited outstanding analytical performances, including a wide linear range (0.1 to 1000.0 nM), low detection limit (0.026 nM, at 3σ/m), excellent selectivity, and high stability. This work provides a perspective for the design of ideal photosensitive materials and signal amplification strategies and extends their application in environment analysis.
Graphical Abstract</description><subject>Analytical Chemistry</subject><subject>Benzhydryl Compounds</subject><subject>Biosensing Techniques - methods</subject><subject>Bisphenol A</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Child</subject><subject>DNA</subject><subject>Heterojunctions</subject><subject>Humans</subject><subject>Intercalating Agents</subject><subject>Metal-Organic Frameworks</subject><subject>Microengineering</subject><subject>Nanochemistry</subject><subject>Nanotechnology</subject><subject>Original Paper</subject><subject>Phenols</subject><subject>Photosensitivity</subject><subject>Target recognition</subject><subject>Toys</subject><issn>0026-3672</issn><issn>1436-5073</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNp9kcFu1DAQhi0EosvCC3BAlrgUodCJ7djZ3qoVBaRCJSgnhCLHGW-8ysbBdkDlJXhlXFJA4sDBmoO_-WY0PyGPS3hRAqiTCCBBFMDyk4xDIe-QVSm4LCpQ_C5ZATBZcKnYEXkQ4x6gVJKJ--SI11zCpipX5MeVDjtMRcDdPOiEHZ16n7w2yX11yWGk3tJt9-HknSveXp7THhMGv5_HDPiRfnOpp5_ez8ftdP2MddP0_TN7Tt2YIaOzz4dTqmnr4tTj6Ad6tuhxQJOCNz0eXOaonpKOOEYfHpJ7Vg8RH93WNfl4_vJq-7q4uHz1Znt2URgOVSpsV7J8A13ZDe9Uqzsj63rDrJFMcSUQTWmkQm7q2lqtALu2FkKCsqK2otJ8TY4X7xT8lxljag4uGhwGPaKfY8M2rGZClfmua_L0H3Tv5zDm7W4oJQSISmWKLZQJPsaAtpmCO-hw3ZTQ3MTVLHE1Oa7mV1yNzE1PbtVze8DuT8vvfDLAFyDmr3GH4e_s_2h_AtOwofc</recordid><startdate>20240301</startdate><enddate>20240301</enddate><creator>Tanjung, Aisyah Protonia</creator><creator>Yin, Ke</creator><creator>Zhao, Lei</creator><creator>Wu, Jiang-Zhou</creator><creator>Wang, Ai-Jun</creator><creator>Mei, Li-Ping</creator><creator>Song, Pei</creator><creator>Feng, Jiu-Ju</creator><general>Springer Vienna</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>K9.</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-5067-3006</orcidid></search><sort><creationdate>20240301</creationdate><title>Target-regulated photoactivities of CdS/Ni-MOF heterojunction with [Ru(bpy)2dppz]2+ intercalator: a bisphenol A photoelectrochemical aptasensor</title><author>Tanjung, Aisyah Protonia ; Yin, Ke ; Zhao, Lei ; Wu, Jiang-Zhou ; Wang, Ai-Jun ; Mei, Li-Ping ; Song, Pei ; Feng, Jiu-Ju</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c305t-fd12100a5f93d7badc68892fc627374eec1c67e3c88ffa70edb844607f48f45a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Analytical Chemistry</topic><topic>Benzhydryl Compounds</topic><topic>Biosensing Techniques - methods</topic><topic>Bisphenol A</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Child</topic><topic>DNA</topic><topic>Heterojunctions</topic><topic>Humans</topic><topic>Intercalating Agents</topic><topic>Metal-Organic Frameworks</topic><topic>Microengineering</topic><topic>Nanochemistry</topic><topic>Nanotechnology</topic><topic>Original Paper</topic><topic>Phenols</topic><topic>Photosensitivity</topic><topic>Target recognition</topic><topic>Toys</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Tanjung, Aisyah Protonia</creatorcontrib><creatorcontrib>Yin, Ke</creatorcontrib><creatorcontrib>Zhao, Lei</creatorcontrib><creatorcontrib>Wu, Jiang-Zhou</creatorcontrib><creatorcontrib>Wang, Ai-Jun</creatorcontrib><creatorcontrib>Mei, Li-Ping</creatorcontrib><creatorcontrib>Song, Pei</creatorcontrib><creatorcontrib>Feng, Jiu-Ju</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>MEDLINE - Academic</collection><jtitle>Mikrochimica acta (1966)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tanjung, Aisyah Protonia</au><au>Yin, Ke</au><au>Zhao, Lei</au><au>Wu, Jiang-Zhou</au><au>Wang, Ai-Jun</au><au>Mei, Li-Ping</au><au>Song, Pei</au><au>Feng, Jiu-Ju</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Target-regulated photoactivities of CdS/Ni-MOF heterojunction with [Ru(bpy)2dppz]2+ intercalator: a bisphenol A photoelectrochemical aptasensor</atitle><jtitle>Mikrochimica acta (1966)</jtitle><stitle>Microchim Acta</stitle><addtitle>Mikrochim Acta</addtitle><date>2024-03-01</date><risdate>2024</risdate><volume>191</volume><issue>3</issue><spage>139</spage><epage>139</epage><pages>139-139</pages><artnum>139</artnum><issn>0026-3672</issn><eissn>1436-5073</eissn><abstract>Bisphenol A (BPA), an important endocrine disrupting compound, has infiltrated human daily lives through electronic devices, food containers, and children’s toys. Developing of novel BPA assay methods with high sensitivity holds tremendous importance in valuing the pollution state. Here, we constructed an ultrasensitive photoelectrochemical (PEC) aptasensor for BPA determination by regulating photoactivities of CdS/Ni-based metal–organic framework (CdS/Ni-MOF) with [Ru(bpy)
2
dppz]
2+
sensitizer. CdS/Ni-MOF spheres exhibited excellent photocatalytic performance, serving as a potential sensing platform for the construction of target recognition process. [Ru(bpy)
2
dppz]
2+
were embedded into DNA double-stranded structure, functioning as sensitizer for modulating the signal response of the developed PEC aptasensor. The proposed PEC sensor exhibited outstanding analytical performances, including a wide linear range (0.1 to 1000.0 nM), low detection limit (0.026 nM, at 3σ/m), excellent selectivity, and high stability. This work provides a perspective for the design of ideal photosensitive materials and signal amplification strategies and extends their application in environment analysis.
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subjects | Analytical Chemistry Benzhydryl Compounds Biosensing Techniques - methods Bisphenol A Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Child DNA Heterojunctions Humans Intercalating Agents Metal-Organic Frameworks Microengineering Nanochemistry Nanotechnology Original Paper Phenols Photosensitivity Target recognition Toys |
title | Target-regulated photoactivities of CdS/Ni-MOF heterojunction with [Ru(bpy)2dppz]2+ intercalator: a bisphenol A photoelectrochemical aptasensor |
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