Disclosing the origin of the reduced magnetoresistance in electron-doped double perovskites

Electron doping in A2-xLxFeMoO6 (where L is a trivalent lanthanide and A is a divalent cation) double perovskites has been established as a suitable technique for increasing their Curie temperature. However, it was found that the magnetoresistance gradually decreases with increasing lanthanide subst...

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Veröffentlicht in:Journal of physics. Condensed matter 2006-08, Vol.18 (34), p.7991-7998
Hauptverfasser: Rubi, D, Fontcuberta, J
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Fontcuberta, J
description Electron doping in A2-xLxFeMoO6 (where L is a trivalent lanthanide and A is a divalent cation) double perovskites has been established as a suitable technique for increasing their Curie temperature. However, it was found that the magnetoresistance gradually decreases with increasing lanthanide substitution. Here we analyse in detail the magnetoresistance as a function of the magnetic field for several series of ceramic A2-xLxFeMoO6 oxides, showing that the data can be well described by assuming a gradual loss of spin polarization of the conduction band upon electron doping. This observation introduces some constraints to models of ferromagnetic coupling in double perovskites.
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subjects Condensed matter: electronic structure, electrical, magnetic, and optical properties
Electronic transport in condensed matter
Exact sciences and technology
Physics
Spin polarized transport
title Disclosing the origin of the reduced magnetoresistance in electron-doped double perovskites
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