Solar reforming as an emerging technology for circular chemical industries
The adverse environmental impacts of greenhouse gas emissions and persistent waste accumulation are driving the demand for sustainable approaches to clean-energy production and waste recycling. By coupling the thermodynamically favourable oxidation of waste-derived organic carbon streams with fuel-f...
Gespeichert in:
Veröffentlicht in: | Nature reviews. Chemistry 2024-02, Vol.8 (2), p.87-105 |
---|---|
Hauptverfasser: | , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | 105 |
---|---|
container_issue | 2 |
container_start_page | 87 |
container_title | Nature reviews. Chemistry |
container_volume | 8 |
creator | Bhattacharjee, Subhajit Linley, Stuart Reisner, Erwin |
description | The adverse environmental impacts of greenhouse gas emissions and persistent waste accumulation are driving the demand for sustainable approaches to clean-energy production and waste recycling. By coupling the thermodynamically favourable oxidation of waste-derived organic carbon streams with fuel-forming reduction reactions suitable for producing clean hydrogen or converting CO
2
to fuels, solar reforming simultaneously valorizes waste and generates useful chemical products. With appropriate light harvesting, catalyst design, device configurations and waste pre-treatment strategies, a range of sustainable fuels and value-added chemicals can already be selectively produced from diverse waste feedstocks, including biomass and plastics, demonstrating the potential of solar-powered upcycling plants. This Review highlights solar reforming as an emerging technology that is currently transitioning from fundamental research towards practical application. We investigate the chemistry and compatibility of waste pre-treatment, introduce process classifications, explore the mechanisms of different solar reforming technologies, and suggest appropriate concepts, metrics and pathways for various deployment scenarios in a net-zero-carbon future.
This Review introduces solar reforming as an emerging technology to produce sustainable fuels and chemicals from diverse waste feedstocks using sunlight. The chemistry and concept of solar reforming, suggestions of key metrics and proposed directions to realize solar-powered refineries for a future circular economy are discussed. |
doi_str_mv | 10.1038/s41570-023-00567-x |
format | Article |
fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2920573326</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2925317173</sourcerecordid><originalsourceid>FETCH-LOGICAL-c375t-f9f67de6466fdc0c7b08422bfc1f1d499ed726b7d9284683aa13074fc2ccbeed3</originalsourceid><addsrcrecordid>eNp9kMlOwzAURS0Eoqj0B1igSGzYBDwkdrxEFaMqsQDWluMhTZXExW6k9u9xSBnEgpWf9c69tg4AZwheIUiK65ChnMEUYpJCmFOWbg_ACSacpYTkxeGveQJmIawghIiTjDN-DCakwBwhgk_A04trpE-8sc63dVclMiSyS0xrfDVcN0YtO9e4apdEIlG1V_0QUEvT1ko2Sd3pPmx8bcIpOLKyCWa2P6fg7e72df6QLp7vH-c3i1QRlm9Syy1l2tCMUqsVVKyERYZxaRWySGecG80wLZnmuMhoQaREBLLMKqxUaYwmU3A59q69e-9N2Ii2Dso0jeyM64PAHMOcEYJpRC_-oCvX-y7-bqByghiK4BTgkVLehRBViLWvW-l3AkExyBajbBFli0_ZYhtD5_vqvmyN_o58qY0AGYEQV11l_M_b_9R-AGRHirE</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2925317173</pqid></control><display><type>article</type><title>Solar reforming as an emerging technology for circular chemical industries</title><source>Nature Journals Online</source><source>SpringerLink</source><creator>Bhattacharjee, Subhajit ; Linley, Stuart ; Reisner, Erwin</creator><creatorcontrib>Bhattacharjee, Subhajit ; Linley, Stuart ; Reisner, Erwin</creatorcontrib><description>The adverse environmental impacts of greenhouse gas emissions and persistent waste accumulation are driving the demand for sustainable approaches to clean-energy production and waste recycling. By coupling the thermodynamically favourable oxidation of waste-derived organic carbon streams with fuel-forming reduction reactions suitable for producing clean hydrogen or converting CO
2
to fuels, solar reforming simultaneously valorizes waste and generates useful chemical products. With appropriate light harvesting, catalyst design, device configurations and waste pre-treatment strategies, a range of sustainable fuels and value-added chemicals can already be selectively produced from diverse waste feedstocks, including biomass and plastics, demonstrating the potential of solar-powered upcycling plants. This Review highlights solar reforming as an emerging technology that is currently transitioning from fundamental research towards practical application. We investigate the chemistry and compatibility of waste pre-treatment, introduce process classifications, explore the mechanisms of different solar reforming technologies, and suggest appropriate concepts, metrics and pathways for various deployment scenarios in a net-zero-carbon future.
This Review introduces solar reforming as an emerging technology to produce sustainable fuels and chemicals from diverse waste feedstocks using sunlight. The chemistry and concept of solar reforming, suggestions of key metrics and proposed directions to realize solar-powered refineries for a future circular economy are discussed.</description><identifier>ISSN: 2397-3358</identifier><identifier>EISSN: 2397-3358</identifier><identifier>DOI: 10.1038/s41570-023-00567-x</identifier><identifier>PMID: 38291132</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/638/675 ; 639/638/77/890 ; 639/638/905 ; Analytical Chemistry ; Biochemistry ; Chemical reduction ; Chemistry ; Chemistry and Materials Science ; Chemistry/Food Science ; Clean energy ; Configuration management ; Emissions ; Fuels ; Greenhouse gases ; Inorganic Chemistry ; New technology ; Organic carbon ; Organic Chemistry ; Oxidation ; Physical Chemistry ; Pretreatment ; Raw materials ; Refineries ; Reforming ; Review Article ; Solar energy</subject><ispartof>Nature reviews. Chemistry, 2024-02, Vol.8 (2), p.87-105</ispartof><rights>Springer Nature Limited 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>2024. Springer Nature Limited.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c375t-f9f67de6466fdc0c7b08422bfc1f1d499ed726b7d9284683aa13074fc2ccbeed3</citedby><cites>FETCH-LOGICAL-c375t-f9f67de6466fdc0c7b08422bfc1f1d499ed726b7d9284683aa13074fc2ccbeed3</cites><orcidid>0000-0002-7781-1616 ; 0000-0003-0596-1073</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1038/s41570-023-00567-x$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1038/s41570-023-00567-x$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38291132$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Bhattacharjee, Subhajit</creatorcontrib><creatorcontrib>Linley, Stuart</creatorcontrib><creatorcontrib>Reisner, Erwin</creatorcontrib><title>Solar reforming as an emerging technology for circular chemical industries</title><title>Nature reviews. Chemistry</title><addtitle>Nat Rev Chem</addtitle><addtitle>Nat Rev Chem</addtitle><description>The adverse environmental impacts of greenhouse gas emissions and persistent waste accumulation are driving the demand for sustainable approaches to clean-energy production and waste recycling. By coupling the thermodynamically favourable oxidation of waste-derived organic carbon streams with fuel-forming reduction reactions suitable for producing clean hydrogen or converting CO
2
to fuels, solar reforming simultaneously valorizes waste and generates useful chemical products. With appropriate light harvesting, catalyst design, device configurations and waste pre-treatment strategies, a range of sustainable fuels and value-added chemicals can already be selectively produced from diverse waste feedstocks, including biomass and plastics, demonstrating the potential of solar-powered upcycling plants. This Review highlights solar reforming as an emerging technology that is currently transitioning from fundamental research towards practical application. We investigate the chemistry and compatibility of waste pre-treatment, introduce process classifications, explore the mechanisms of different solar reforming technologies, and suggest appropriate concepts, metrics and pathways for various deployment scenarios in a net-zero-carbon future.
This Review introduces solar reforming as an emerging technology to produce sustainable fuels and chemicals from diverse waste feedstocks using sunlight. The chemistry and concept of solar reforming, suggestions of key metrics and proposed directions to realize solar-powered refineries for a future circular economy are discussed.</description><subject>639/638/675</subject><subject>639/638/77/890</subject><subject>639/638/905</subject><subject>Analytical Chemistry</subject><subject>Biochemistry</subject><subject>Chemical reduction</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Chemistry/Food Science</subject><subject>Clean energy</subject><subject>Configuration management</subject><subject>Emissions</subject><subject>Fuels</subject><subject>Greenhouse gases</subject><subject>Inorganic Chemistry</subject><subject>New technology</subject><subject>Organic carbon</subject><subject>Organic Chemistry</subject><subject>Oxidation</subject><subject>Physical Chemistry</subject><subject>Pretreatment</subject><subject>Raw materials</subject><subject>Refineries</subject><subject>Reforming</subject><subject>Review Article</subject><subject>Solar energy</subject><issn>2397-3358</issn><issn>2397-3358</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kMlOwzAURS0Eoqj0B1igSGzYBDwkdrxEFaMqsQDWluMhTZXExW6k9u9xSBnEgpWf9c69tg4AZwheIUiK65ChnMEUYpJCmFOWbg_ACSacpYTkxeGveQJmIawghIiTjDN-DCakwBwhgk_A04trpE-8sc63dVclMiSyS0xrfDVcN0YtO9e4apdEIlG1V_0QUEvT1ko2Sd3pPmx8bcIpOLKyCWa2P6fg7e72df6QLp7vH-c3i1QRlm9Syy1l2tCMUqsVVKyERYZxaRWySGecG80wLZnmuMhoQaREBLLMKqxUaYwmU3A59q69e-9N2Ii2Dso0jeyM64PAHMOcEYJpRC_-oCvX-y7-bqByghiK4BTgkVLehRBViLWvW-l3AkExyBajbBFli0_ZYhtD5_vqvmyN_o58qY0AGYEQV11l_M_b_9R-AGRHirE</recordid><startdate>20240201</startdate><enddate>20240201</enddate><creator>Bhattacharjee, Subhajit</creator><creator>Linley, Stuart</creator><creator>Reisner, Erwin</creator><general>Nature Publishing Group UK</general><general>Nature Publishing Group</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-7781-1616</orcidid><orcidid>https://orcid.org/0000-0003-0596-1073</orcidid></search><sort><creationdate>20240201</creationdate><title>Solar reforming as an emerging technology for circular chemical industries</title><author>Bhattacharjee, Subhajit ; Linley, Stuart ; Reisner, Erwin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c375t-f9f67de6466fdc0c7b08422bfc1f1d499ed726b7d9284683aa13074fc2ccbeed3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>639/638/675</topic><topic>639/638/77/890</topic><topic>639/638/905</topic><topic>Analytical Chemistry</topic><topic>Biochemistry</topic><topic>Chemical reduction</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Chemistry/Food Science</topic><topic>Clean energy</topic><topic>Configuration management</topic><topic>Emissions</topic><topic>Fuels</topic><topic>Greenhouse gases</topic><topic>Inorganic Chemistry</topic><topic>New technology</topic><topic>Organic carbon</topic><topic>Organic Chemistry</topic><topic>Oxidation</topic><topic>Physical Chemistry</topic><topic>Pretreatment</topic><topic>Raw materials</topic><topic>Refineries</topic><topic>Reforming</topic><topic>Review Article</topic><topic>Solar energy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Bhattacharjee, Subhajit</creatorcontrib><creatorcontrib>Linley, Stuart</creatorcontrib><creatorcontrib>Reisner, Erwin</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Nature reviews. Chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Bhattacharjee, Subhajit</au><au>Linley, Stuart</au><au>Reisner, Erwin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Solar reforming as an emerging technology for circular chemical industries</atitle><jtitle>Nature reviews. Chemistry</jtitle><stitle>Nat Rev Chem</stitle><addtitle>Nat Rev Chem</addtitle><date>2024-02-01</date><risdate>2024</risdate><volume>8</volume><issue>2</issue><spage>87</spage><epage>105</epage><pages>87-105</pages><issn>2397-3358</issn><eissn>2397-3358</eissn><abstract>The adverse environmental impacts of greenhouse gas emissions and persistent waste accumulation are driving the demand for sustainable approaches to clean-energy production and waste recycling. By coupling the thermodynamically favourable oxidation of waste-derived organic carbon streams with fuel-forming reduction reactions suitable for producing clean hydrogen or converting CO
2
to fuels, solar reforming simultaneously valorizes waste and generates useful chemical products. With appropriate light harvesting, catalyst design, device configurations and waste pre-treatment strategies, a range of sustainable fuels and value-added chemicals can already be selectively produced from diverse waste feedstocks, including biomass and plastics, demonstrating the potential of solar-powered upcycling plants. This Review highlights solar reforming as an emerging technology that is currently transitioning from fundamental research towards practical application. We investigate the chemistry and compatibility of waste pre-treatment, introduce process classifications, explore the mechanisms of different solar reforming technologies, and suggest appropriate concepts, metrics and pathways for various deployment scenarios in a net-zero-carbon future.
This Review introduces solar reforming as an emerging technology to produce sustainable fuels and chemicals from diverse waste feedstocks using sunlight. The chemistry and concept of solar reforming, suggestions of key metrics and proposed directions to realize solar-powered refineries for a future circular economy are discussed.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>38291132</pmid><doi>10.1038/s41570-023-00567-x</doi><tpages>19</tpages><orcidid>https://orcid.org/0000-0002-7781-1616</orcidid><orcidid>https://orcid.org/0000-0003-0596-1073</orcidid></addata></record> |
fulltext | fulltext |
identifier | ISSN: 2397-3358 |
ispartof | Nature reviews. Chemistry, 2024-02, Vol.8 (2), p.87-105 |
issn | 2397-3358 2397-3358 |
language | eng |
recordid | cdi_proquest_miscellaneous_2920573326 |
source | Nature Journals Online; SpringerLink |
subjects | 639/638/675 639/638/77/890 639/638/905 Analytical Chemistry Biochemistry Chemical reduction Chemistry Chemistry and Materials Science Chemistry/Food Science Clean energy Configuration management Emissions Fuels Greenhouse gases Inorganic Chemistry New technology Organic carbon Organic Chemistry Oxidation Physical Chemistry Pretreatment Raw materials Refineries Reforming Review Article Solar energy |
title | Solar reforming as an emerging technology for circular chemical industries |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-29T10%3A09%3A16IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Solar%20reforming%20as%20an%20emerging%20technology%20for%20circular%20chemical%20industries&rft.jtitle=Nature%20reviews.%20Chemistry&rft.au=Bhattacharjee,%20Subhajit&rft.date=2024-02-01&rft.volume=8&rft.issue=2&rft.spage=87&rft.epage=105&rft.pages=87-105&rft.issn=2397-3358&rft.eissn=2397-3358&rft_id=info:doi/10.1038/s41570-023-00567-x&rft_dat=%3Cproquest_cross%3E2925317173%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2925317173&rft_id=info:pmid/38291132&rfr_iscdi=true |