Description of exciton transport in a TiO2/MEH-PPV heterojunction photovoltaic material

A model for exciton transport in conjugated polymers has been developed taking into account inhomogeneous broadening of exciton energy level. Time-resolved photoluminescence data were used to determine the parameters of the model, such as exciton lifetime, effective number of exciton energy levels w...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Solar energy materials and solar cells 2005-05, Vol.87 (1-4), p.715-724
Hauptverfasser: KAWATA, K, BURLAKOV, V. M, CAREY, M. J, ASSENDER, H. E, BRIGGS, G. A. D, RUSECKAS, A, SAMUEL, I. D. W
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 724
container_issue 1-4
container_start_page 715
container_title Solar energy materials and solar cells
container_volume 87
creator KAWATA, K
BURLAKOV, V. M
CAREY, M. J
ASSENDER, H. E
BRIGGS, G. A. D
RUSECKAS, A
SAMUEL, I. D. W
description A model for exciton transport in conjugated polymers has been developed taking into account inhomogeneous broadening of exciton energy level. Time-resolved photoluminescence data were used to determine the parameters of the model, such as exciton lifetime, effective number of exciton energy levels within inhomogeneously broadened density of states, hopping distance and hopping rate constants for excitons. Using the developed model a non-monoexponential decay of photoluminescence of the conjugated polymer deposited on TiO2 substrate was described, and the spectrum of internal quantum efficiency of the heterojunction photovoltaic device based on the conjugated polymer with a nanocrystalline TiO2 layer was predicted.
doi_str_mv 10.1016/j.solmat.2004.07.046
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_29200864</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>29200864</sourcerecordid><originalsourceid>FETCH-LOGICAL-c378t-8f91b937c0fd3dfa291ff0802f1d36a62f72fe5aab39a36270133f982a4fa9513</originalsourceid><addsrcrecordid>eNpFkLlOAzEURS0EEmH5A4ppoJvJsz3xUiJ2CQQFS2m9OLbiaDIebAfB3zMQJKp3i3uung4hJxQaClRMV02O3RpLwwDaBmQDrdghE6qkrjnXapdMQDNZA2vVPjnIeQUATPB2Qt4uXbYpDCXEvoq-cp82lDGWhH0eYipV6CusnsMjmz5c3dZPT6_V0hWX4mrT219qWMYSP2JXMNhq_MKlgN0R2fPYZXf8dw_Jy_XV88Vtff94c3dxfl9bLlWpldd0rrm04Bd84ZFp6j0oYJ4uuEDBvGTezRDnXCMXTALl3GvFsPWoZ5QfkrPt7pDi-8blYtYhW9d12Lu4yYbp0YkS7Vhst0WbYs7JeTOksMb0ZSiYH4tmZbYWzY9FA9KMFkfs9G8fs8XOj1psyP-skEqKlvFvzDN1dg</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>29200864</pqid></control><display><type>article</type><title>Description of exciton transport in a TiO2/MEH-PPV heterojunction photovoltaic material</title><source>Elsevier ScienceDirect Journals</source><creator>KAWATA, K ; BURLAKOV, V. M ; CAREY, M. J ; ASSENDER, H. E ; BRIGGS, G. A. D ; RUSECKAS, A ; SAMUEL, I. D. W</creator><creatorcontrib>KAWATA, K ; BURLAKOV, V. M ; CAREY, M. J ; ASSENDER, H. E ; BRIGGS, G. A. D ; RUSECKAS, A ; SAMUEL, I. D. W</creatorcontrib><description>A model for exciton transport in conjugated polymers has been developed taking into account inhomogeneous broadening of exciton energy level. Time-resolved photoluminescence data were used to determine the parameters of the model, such as exciton lifetime, effective number of exciton energy levels within inhomogeneously broadened density of states, hopping distance and hopping rate constants for excitons. Using the developed model a non-monoexponential decay of photoluminescence of the conjugated polymer deposited on TiO2 substrate was described, and the spectrum of internal quantum efficiency of the heterojunction photovoltaic device based on the conjugated polymer with a nanocrystalline TiO2 layer was predicted.</description><identifier>ISSN: 0927-0248</identifier><identifier>EISSN: 1879-3398</identifier><identifier>DOI: 10.1016/j.solmat.2004.07.046</identifier><language>eng</language><publisher>Amsterdam: Elsevier</publisher><subject>Applied sciences ; Energy ; Equipments, installations and applications ; Exact sciences and technology ; Natural energy ; Photovoltaic conversion ; Solar cells. Photoelectrochemical cells ; Solar energy</subject><ispartof>Solar energy materials and solar cells, 2005-05, Vol.87 (1-4), p.715-724</ispartof><rights>2005 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c378t-8f91b937c0fd3dfa291ff0802f1d36a62f72fe5aab39a36270133f982a4fa9513</citedby><cites>FETCH-LOGICAL-c378t-8f91b937c0fd3dfa291ff0802f1d36a62f72fe5aab39a36270133f982a4fa9513</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>309,310,314,777,781,786,787,23911,23912,25121,27905,27906</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&amp;idt=16787642$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>KAWATA, K</creatorcontrib><creatorcontrib>BURLAKOV, V. M</creatorcontrib><creatorcontrib>CAREY, M. J</creatorcontrib><creatorcontrib>ASSENDER, H. E</creatorcontrib><creatorcontrib>BRIGGS, G. A. D</creatorcontrib><creatorcontrib>RUSECKAS, A</creatorcontrib><creatorcontrib>SAMUEL, I. D. W</creatorcontrib><title>Description of exciton transport in a TiO2/MEH-PPV heterojunction photovoltaic material</title><title>Solar energy materials and solar cells</title><description>A model for exciton transport in conjugated polymers has been developed taking into account inhomogeneous broadening of exciton energy level. Time-resolved photoluminescence data were used to determine the parameters of the model, such as exciton lifetime, effective number of exciton energy levels within inhomogeneously broadened density of states, hopping distance and hopping rate constants for excitons. Using the developed model a non-monoexponential decay of photoluminescence of the conjugated polymer deposited on TiO2 substrate was described, and the spectrum of internal quantum efficiency of the heterojunction photovoltaic device based on the conjugated polymer with a nanocrystalline TiO2 layer was predicted.</description><subject>Applied sciences</subject><subject>Energy</subject><subject>Equipments, installations and applications</subject><subject>Exact sciences and technology</subject><subject>Natural energy</subject><subject>Photovoltaic conversion</subject><subject>Solar cells. Photoelectrochemical cells</subject><subject>Solar energy</subject><issn>0927-0248</issn><issn>1879-3398</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><recordid>eNpFkLlOAzEURS0EEmH5A4ppoJvJsz3xUiJ2CQQFS2m9OLbiaDIebAfB3zMQJKp3i3uung4hJxQaClRMV02O3RpLwwDaBmQDrdghE6qkrjnXapdMQDNZA2vVPjnIeQUATPB2Qt4uXbYpDCXEvoq-cp82lDGWhH0eYipV6CusnsMjmz5c3dZPT6_V0hWX4mrT219qWMYSP2JXMNhq_MKlgN0R2fPYZXf8dw_Jy_XV88Vtff94c3dxfl9bLlWpldd0rrm04Bd84ZFp6j0oYJ4uuEDBvGTezRDnXCMXTALl3GvFsPWoZ5QfkrPt7pDi-8blYtYhW9d12Lu4yYbp0YkS7Vhst0WbYs7JeTOksMb0ZSiYH4tmZbYWzY9FA9KMFkfs9G8fs8XOj1psyP-skEqKlvFvzDN1dg</recordid><startdate>20050501</startdate><enddate>20050501</enddate><creator>KAWATA, K</creator><creator>BURLAKOV, V. M</creator><creator>CAREY, M. J</creator><creator>ASSENDER, H. E</creator><creator>BRIGGS, G. A. D</creator><creator>RUSECKAS, A</creator><creator>SAMUEL, I. D. W</creator><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7TB</scope><scope>7U5</scope><scope>8FD</scope><scope>FR3</scope><scope>L7M</scope></search><sort><creationdate>20050501</creationdate><title>Description of exciton transport in a TiO2/MEH-PPV heterojunction photovoltaic material</title><author>KAWATA, K ; BURLAKOV, V. M ; CAREY, M. J ; ASSENDER, H. E ; BRIGGS, G. A. D ; RUSECKAS, A ; SAMUEL, I. D. W</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c378t-8f91b937c0fd3dfa291ff0802f1d36a62f72fe5aab39a36270133f982a4fa9513</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2005</creationdate><topic>Applied sciences</topic><topic>Energy</topic><topic>Equipments, installations and applications</topic><topic>Exact sciences and technology</topic><topic>Natural energy</topic><topic>Photovoltaic conversion</topic><topic>Solar cells. Photoelectrochemical cells</topic><topic>Solar energy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>KAWATA, K</creatorcontrib><creatorcontrib>BURLAKOV, V. M</creatorcontrib><creatorcontrib>CAREY, M. J</creatorcontrib><creatorcontrib>ASSENDER, H. E</creatorcontrib><creatorcontrib>BRIGGS, G. A. D</creatorcontrib><creatorcontrib>RUSECKAS, A</creatorcontrib><creatorcontrib>SAMUEL, I. D. W</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Electronics &amp; Communications Abstracts</collection><collection>Mechanical &amp; Transportation Engineering Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Solar energy materials and solar cells</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>KAWATA, K</au><au>BURLAKOV, V. M</au><au>CAREY, M. J</au><au>ASSENDER, H. E</au><au>BRIGGS, G. A. D</au><au>RUSECKAS, A</au><au>SAMUEL, I. D. W</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Description of exciton transport in a TiO2/MEH-PPV heterojunction photovoltaic material</atitle><jtitle>Solar energy materials and solar cells</jtitle><date>2005-05-01</date><risdate>2005</risdate><volume>87</volume><issue>1-4</issue><spage>715</spage><epage>724</epage><pages>715-724</pages><issn>0927-0248</issn><eissn>1879-3398</eissn><abstract>A model for exciton transport in conjugated polymers has been developed taking into account inhomogeneous broadening of exciton energy level. Time-resolved photoluminescence data were used to determine the parameters of the model, such as exciton lifetime, effective number of exciton energy levels within inhomogeneously broadened density of states, hopping distance and hopping rate constants for excitons. Using the developed model a non-monoexponential decay of photoluminescence of the conjugated polymer deposited on TiO2 substrate was described, and the spectrum of internal quantum efficiency of the heterojunction photovoltaic device based on the conjugated polymer with a nanocrystalline TiO2 layer was predicted.</abstract><cop>Amsterdam</cop><pub>Elsevier</pub><doi>10.1016/j.solmat.2004.07.046</doi><tpages>10</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0927-0248
ispartof Solar energy materials and solar cells, 2005-05, Vol.87 (1-4), p.715-724
issn 0927-0248
1879-3398
language eng
recordid cdi_proquest_miscellaneous_29200864
source Elsevier ScienceDirect Journals
subjects Applied sciences
Energy
Equipments, installations and applications
Exact sciences and technology
Natural energy
Photovoltaic conversion
Solar cells. Photoelectrochemical cells
Solar energy
title Description of exciton transport in a TiO2/MEH-PPV heterojunction photovoltaic material
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-18T16%3A47%3A28IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Description%20of%20exciton%20transport%20in%20a%20TiO2/MEH-PPV%20heterojunction%20photovoltaic%20material&rft.jtitle=Solar%20energy%20materials%20and%20solar%20cells&rft.au=KAWATA,%20K&rft.date=2005-05-01&rft.volume=87&rft.issue=1-4&rft.spage=715&rft.epage=724&rft.pages=715-724&rft.issn=0927-0248&rft.eissn=1879-3398&rft_id=info:doi/10.1016/j.solmat.2004.07.046&rft_dat=%3Cproquest_cross%3E29200864%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=29200864&rft_id=info:pmid/&rfr_iscdi=true