Automated Laboratory Kilogram‐Scale Graphene Production from Coal
The flash Joule heating (FJH) method converts many carbon feedstocks into graphene in milliseconds to seconds using an electrical pulse. This opens an opportunity for processing low or negative value resources, such as coal and plastic waste, into high value graphene. Here, a lab‐scale automation FJ...
Gespeichert in:
| Veröffentlicht in: | Small methods 2024-03, Vol.8 (3), p.e2301144-n/a |
|---|---|
| Hauptverfasser: | , , , , , , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | n/a |
|---|---|
| container_issue | 3 |
| container_start_page | e2301144 |
| container_title | Small methods |
| container_volume | 8 |
| creator | Eddy, Lucas Luong, Duy Xuan Beckham, Jacob L. Wyss, Kevin M. Cooksey, Tyler J. Scotland, Phelecia Choi, Chi Hun Chen, Weiyin Advincula, Paul A. Zhang, Zhiyong Mancevski, Vladimir Kittrell, Carter Han, Yimo Tour, James M. |
| description | The flash Joule heating (FJH) method converts many carbon feedstocks into graphene in milliseconds to seconds using an electrical pulse. This opens an opportunity for processing low or negative value resources, such as coal and plastic waste, into high value graphene. Here, a lab‐scale automation FJH system that allows the synthesis of 1.1 kg of turbostratic flash graphene from coal‐based metallurgical coke (MC) in 1.5 h is demonstrated. The process is based on the automated conversion of 5.7 g of MC per batch using an electrical pulse width modulation system to conduct the bottom‐up upcycle of MC into flash graphene. This study then compare this method to two other scalable graphene synthesis techniques by both a life cycle assessment and a technoeconomic assessment.
Automated kilogram‐scale graphene production is achieved via flash Joule heating using an automated loading, flashing, and unloading apparatus. Pulse width modulation is used to increase graphene quality and uniformity in large batches. Life cycle and technoeconomic assessments demonstrate the energy and cost efficiency of this production method. |
| doi_str_mv | 10.1002/smtd.202301144 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2894722931</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2894722931</sourcerecordid><originalsourceid>FETCH-LOGICAL-c3454-57d303bb1d406a8f7d7074c28c3e62177c8ad9f968c4e30d83d04d4e4469f7783</originalsourceid><addsrcrecordid>eNqFkLtOwzAYRi0EolXpyogysqT4Vl_GKkBBFIHUMluO7UBQUhc7EerGI_CMPAmpWgob0_8P5zvDAeAUwRGCEF_EurEjDDGBCFF6APqYMJZKBsXhn78HhjG-wm4AERljdAx6REAoOZN9kE3axte6cTaZ6dwH3fiwTu7Kyj8HXX99fM6NrlwyDXr14pYueQzetqYp_TIpgq-TzOvqBBwVuopuuLsD8HR9tchu0tnD9DabzFJD6JimY24JJHmOLIVMi4JbDjk1WBjiGEacG6GtLCQThjoCrSAWUksdpUwWnAsyAOdb7yr4t9bFRtVlNK6q9NL5NiosJOUYS4I6dLRFTfAxBleoVShrHdYKQbVppzbt1L5dNzjbudu8dnaP_5TqALkF3svKrf_Rqfn94vJX_g0HHHr6</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2894722931</pqid></control><display><type>article</type><title>Automated Laboratory Kilogram‐Scale Graphene Production from Coal</title><source>Wiley Online Library Journals Frontfile Complete</source><creator>Eddy, Lucas ; Luong, Duy Xuan ; Beckham, Jacob L. ; Wyss, Kevin M. ; Cooksey, Tyler J. ; Scotland, Phelecia ; Choi, Chi Hun ; Chen, Weiyin ; Advincula, Paul A. ; Zhang, Zhiyong ; Mancevski, Vladimir ; Kittrell, Carter ; Han, Yimo ; Tour, James M.</creator><creatorcontrib>Eddy, Lucas ; Luong, Duy Xuan ; Beckham, Jacob L. ; Wyss, Kevin M. ; Cooksey, Tyler J. ; Scotland, Phelecia ; Choi, Chi Hun ; Chen, Weiyin ; Advincula, Paul A. ; Zhang, Zhiyong ; Mancevski, Vladimir ; Kittrell, Carter ; Han, Yimo ; Tour, James M.</creatorcontrib><description>The flash Joule heating (FJH) method converts many carbon feedstocks into graphene in milliseconds to seconds using an electrical pulse. This opens an opportunity for processing low or negative value resources, such as coal and plastic waste, into high value graphene. Here, a lab‐scale automation FJH system that allows the synthesis of 1.1 kg of turbostratic flash graphene from coal‐based metallurgical coke (MC) in 1.5 h is demonstrated. The process is based on the automated conversion of 5.7 g of MC per batch using an electrical pulse width modulation system to conduct the bottom‐up upcycle of MC into flash graphene. This study then compare this method to two other scalable graphene synthesis techniques by both a life cycle assessment and a technoeconomic assessment.
Automated kilogram‐scale graphene production is achieved via flash Joule heating using an automated loading, flashing, and unloading apparatus. Pulse width modulation is used to increase graphene quality and uniformity in large batches. Life cycle and technoeconomic assessments demonstrate the energy and cost efficiency of this production method.</description><identifier>ISSN: 2366-9608</identifier><identifier>EISSN: 2366-9608</identifier><identifier>DOI: 10.1002/smtd.202301144</identifier><identifier>PMID: 38009769</identifier><language>eng</language><publisher>Germany</publisher><subject>automation ; flash Joule heating ; graphene ; kilogram‐scale ; life cycle assessment</subject><ispartof>Small methods, 2024-03, Vol.8 (3), p.e2301144-n/a</ispartof><rights>2023 Wiley‐VCH GmbH</rights><rights>2023 Wiley-VCH GmbH.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c3454-57d303bb1d406a8f7d7074c28c3e62177c8ad9f968c4e30d83d04d4e4469f7783</citedby><cites>FETCH-LOGICAL-c3454-57d303bb1d406a8f7d7074c28c3e62177c8ad9f968c4e30d83d04d4e4469f7783</cites><orcidid>0000-0002-8449-4292 ; 0000-0003-4024-5814 ; 0000-0001-7089-3359 ; 0000-0002-8479-9328 ; 0000-0002-2787-3712 ; 0000-0001-8189-0081 ; 0000-0002-0208-6181 ; 0000-0001-8203-0788 ; 0000-0002-6427-4129 ; 0000-0003-0563-4611 ; 0000-0002-2838-0696</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fsmtd.202301144$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fsmtd.202301144$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27901,27902,45550,45551</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/38009769$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Eddy, Lucas</creatorcontrib><creatorcontrib>Luong, Duy Xuan</creatorcontrib><creatorcontrib>Beckham, Jacob L.</creatorcontrib><creatorcontrib>Wyss, Kevin M.</creatorcontrib><creatorcontrib>Cooksey, Tyler J.</creatorcontrib><creatorcontrib>Scotland, Phelecia</creatorcontrib><creatorcontrib>Choi, Chi Hun</creatorcontrib><creatorcontrib>Chen, Weiyin</creatorcontrib><creatorcontrib>Advincula, Paul A.</creatorcontrib><creatorcontrib>Zhang, Zhiyong</creatorcontrib><creatorcontrib>Mancevski, Vladimir</creatorcontrib><creatorcontrib>Kittrell, Carter</creatorcontrib><creatorcontrib>Han, Yimo</creatorcontrib><creatorcontrib>Tour, James M.</creatorcontrib><title>Automated Laboratory Kilogram‐Scale Graphene Production from Coal</title><title>Small methods</title><addtitle>Small Methods</addtitle><description>The flash Joule heating (FJH) method converts many carbon feedstocks into graphene in milliseconds to seconds using an electrical pulse. This opens an opportunity for processing low or negative value resources, such as coal and plastic waste, into high value graphene. Here, a lab‐scale automation FJH system that allows the synthesis of 1.1 kg of turbostratic flash graphene from coal‐based metallurgical coke (MC) in 1.5 h is demonstrated. The process is based on the automated conversion of 5.7 g of MC per batch using an electrical pulse width modulation system to conduct the bottom‐up upcycle of MC into flash graphene. This study then compare this method to two other scalable graphene synthesis techniques by both a life cycle assessment and a technoeconomic assessment.
Automated kilogram‐scale graphene production is achieved via flash Joule heating using an automated loading, flashing, and unloading apparatus. Pulse width modulation is used to increase graphene quality and uniformity in large batches. Life cycle and technoeconomic assessments demonstrate the energy and cost efficiency of this production method.</description><subject>automation</subject><subject>flash Joule heating</subject><subject>graphene</subject><subject>kilogram‐scale</subject><subject>life cycle assessment</subject><issn>2366-9608</issn><issn>2366-9608</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNqFkLtOwzAYRi0EolXpyogysqT4Vl_GKkBBFIHUMluO7UBQUhc7EerGI_CMPAmpWgob0_8P5zvDAeAUwRGCEF_EurEjDDGBCFF6APqYMJZKBsXhn78HhjG-wm4AERljdAx6REAoOZN9kE3axte6cTaZ6dwH3fiwTu7Kyj8HXX99fM6NrlwyDXr14pYueQzetqYp_TIpgq-TzOvqBBwVuopuuLsD8HR9tchu0tnD9DabzFJD6JimY24JJHmOLIVMi4JbDjk1WBjiGEacG6GtLCQThjoCrSAWUksdpUwWnAsyAOdb7yr4t9bFRtVlNK6q9NL5NiosJOUYS4I6dLRFTfAxBleoVShrHdYKQbVppzbt1L5dNzjbudu8dnaP_5TqALkF3svKrf_Rqfn94vJX_g0HHHr6</recordid><startdate>20240301</startdate><enddate>20240301</enddate><creator>Eddy, Lucas</creator><creator>Luong, Duy Xuan</creator><creator>Beckham, Jacob L.</creator><creator>Wyss, Kevin M.</creator><creator>Cooksey, Tyler J.</creator><creator>Scotland, Phelecia</creator><creator>Choi, Chi Hun</creator><creator>Chen, Weiyin</creator><creator>Advincula, Paul A.</creator><creator>Zhang, Zhiyong</creator><creator>Mancevski, Vladimir</creator><creator>Kittrell, Carter</creator><creator>Han, Yimo</creator><creator>Tour, James M.</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-8449-4292</orcidid><orcidid>https://orcid.org/0000-0003-4024-5814</orcidid><orcidid>https://orcid.org/0000-0001-7089-3359</orcidid><orcidid>https://orcid.org/0000-0002-8479-9328</orcidid><orcidid>https://orcid.org/0000-0002-2787-3712</orcidid><orcidid>https://orcid.org/0000-0001-8189-0081</orcidid><orcidid>https://orcid.org/0000-0002-0208-6181</orcidid><orcidid>https://orcid.org/0000-0001-8203-0788</orcidid><orcidid>https://orcid.org/0000-0002-6427-4129</orcidid><orcidid>https://orcid.org/0000-0003-0563-4611</orcidid><orcidid>https://orcid.org/0000-0002-2838-0696</orcidid></search><sort><creationdate>20240301</creationdate><title>Automated Laboratory Kilogram‐Scale Graphene Production from Coal</title><author>Eddy, Lucas ; Luong, Duy Xuan ; Beckham, Jacob L. ; Wyss, Kevin M. ; Cooksey, Tyler J. ; Scotland, Phelecia ; Choi, Chi Hun ; Chen, Weiyin ; Advincula, Paul A. ; Zhang, Zhiyong ; Mancevski, Vladimir ; Kittrell, Carter ; Han, Yimo ; Tour, James M.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c3454-57d303bb1d406a8f7d7074c28c3e62177c8ad9f968c4e30d83d04d4e4469f7783</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>automation</topic><topic>flash Joule heating</topic><topic>graphene</topic><topic>kilogram‐scale</topic><topic>life cycle assessment</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Eddy, Lucas</creatorcontrib><creatorcontrib>Luong, Duy Xuan</creatorcontrib><creatorcontrib>Beckham, Jacob L.</creatorcontrib><creatorcontrib>Wyss, Kevin M.</creatorcontrib><creatorcontrib>Cooksey, Tyler J.</creatorcontrib><creatorcontrib>Scotland, Phelecia</creatorcontrib><creatorcontrib>Choi, Chi Hun</creatorcontrib><creatorcontrib>Chen, Weiyin</creatorcontrib><creatorcontrib>Advincula, Paul A.</creatorcontrib><creatorcontrib>Zhang, Zhiyong</creatorcontrib><creatorcontrib>Mancevski, Vladimir</creatorcontrib><creatorcontrib>Kittrell, Carter</creatorcontrib><creatorcontrib>Han, Yimo</creatorcontrib><creatorcontrib>Tour, James M.</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Small methods</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Eddy, Lucas</au><au>Luong, Duy Xuan</au><au>Beckham, Jacob L.</au><au>Wyss, Kevin M.</au><au>Cooksey, Tyler J.</au><au>Scotland, Phelecia</au><au>Choi, Chi Hun</au><au>Chen, Weiyin</au><au>Advincula, Paul A.</au><au>Zhang, Zhiyong</au><au>Mancevski, Vladimir</au><au>Kittrell, Carter</au><au>Han, Yimo</au><au>Tour, James M.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Automated Laboratory Kilogram‐Scale Graphene Production from Coal</atitle><jtitle>Small methods</jtitle><addtitle>Small Methods</addtitle><date>2024-03-01</date><risdate>2024</risdate><volume>8</volume><issue>3</issue><spage>e2301144</spage><epage>n/a</epage><pages>e2301144-n/a</pages><issn>2366-9608</issn><eissn>2366-9608</eissn><abstract>The flash Joule heating (FJH) method converts many carbon feedstocks into graphene in milliseconds to seconds using an electrical pulse. This opens an opportunity for processing low or negative value resources, such as coal and plastic waste, into high value graphene. Here, a lab‐scale automation FJH system that allows the synthesis of 1.1 kg of turbostratic flash graphene from coal‐based metallurgical coke (MC) in 1.5 h is demonstrated. The process is based on the automated conversion of 5.7 g of MC per batch using an electrical pulse width modulation system to conduct the bottom‐up upcycle of MC into flash graphene. This study then compare this method to two other scalable graphene synthesis techniques by both a life cycle assessment and a technoeconomic assessment.
Automated kilogram‐scale graphene production is achieved via flash Joule heating using an automated loading, flashing, and unloading apparatus. Pulse width modulation is used to increase graphene quality and uniformity in large batches. Life cycle and technoeconomic assessments demonstrate the energy and cost efficiency of this production method.</abstract><cop>Germany</cop><pmid>38009769</pmid><doi>10.1002/smtd.202301144</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0002-8449-4292</orcidid><orcidid>https://orcid.org/0000-0003-4024-5814</orcidid><orcidid>https://orcid.org/0000-0001-7089-3359</orcidid><orcidid>https://orcid.org/0000-0002-8479-9328</orcidid><orcidid>https://orcid.org/0000-0002-2787-3712</orcidid><orcidid>https://orcid.org/0000-0001-8189-0081</orcidid><orcidid>https://orcid.org/0000-0002-0208-6181</orcidid><orcidid>https://orcid.org/0000-0001-8203-0788</orcidid><orcidid>https://orcid.org/0000-0002-6427-4129</orcidid><orcidid>https://orcid.org/0000-0003-0563-4611</orcidid><orcidid>https://orcid.org/0000-0002-2838-0696</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 2366-9608 |
| ispartof | Small methods, 2024-03, Vol.8 (3), p.e2301144-n/a |
| issn | 2366-9608 2366-9608 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2894722931 |
| source | Wiley Online Library Journals Frontfile Complete |
| subjects | automation flash Joule heating graphene kilogram‐scale life cycle assessment |
| title | Automated Laboratory Kilogram‐Scale Graphene Production from Coal |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-02T17%3A39%3A22IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Automated%20Laboratory%20Kilogram%E2%80%90Scale%20Graphene%20Production%20from%20Coal&rft.jtitle=Small%20methods&rft.au=Eddy,%20Lucas&rft.date=2024-03-01&rft.volume=8&rft.issue=3&rft.spage=e2301144&rft.epage=n/a&rft.pages=e2301144-n/a&rft.issn=2366-9608&rft.eissn=2366-9608&rft_id=info:doi/10.1002/smtd.202301144&rft_dat=%3Cproquest_cross%3E2894722931%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2894722931&rft_id=info:pmid/38009769&rfr_iscdi=true |