Entropy engineering of La-based perovskite for simultaneous photocatalytic CO2 reduction and biomass oxidation
Herein, the high-entropy perovskite, i.e. La(FeCoNiCrMn)O3, was prepared for simultaneous CO2 reduction and biomass upgrading. Based on the synergistic effect between the elements in the high-entropy material, an excellent CO evolution rate of 131.8 μmol g−1 h−1 and a xylonic acid yield of 63.9% wer...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2023-12, Vol.59 (99), p.14673-14676 |
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| container_issue | 99 |
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| container_title | Chemical communications (Cambridge, England) |
| container_volume | 59 |
| creator | Wang, Mengchen Li, Liming Li, Yong Shi, Xuxia Ren, Hangxing Sun, Yuetao Liu, Kangning Song, Wei Li, Huamin Wang, Haibin Han, Mei Wang, Xi Momo, Christopher Dorma Chen, Songhua Liu, Lihua Liang, Hongyan |
| description | Herein, the high-entropy perovskite, i.e. La(FeCoNiCrMn)O3, was prepared for simultaneous CO2 reduction and biomass upgrading. Based on the synergistic effect between the elements in the high-entropy material, an excellent CO evolution rate of 131.8 μmol g−1 h−1 and a xylonic acid yield of 63.9% were gained. |
| doi_str_mv | 10.1039/d3cc04393b |
| format | Article |
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Based on the synergistic effect between the elements in the high-entropy material, an excellent CO evolution rate of 131.8 μmol g−1 h−1 and a xylonic acid yield of 63.9% were gained.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d3cc04393b</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Biomass ; Carbon dioxide ; Entropy ; Oxidation ; Perovskites ; Reduction ; Synergistic effect</subject><ispartof>Chemical communications (Cambridge, England), 2023-12, Vol.59 (99), p.14673-14676</ispartof><rights>Copyright Royal Society of Chemistry 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Wang, Mengchen</creatorcontrib><creatorcontrib>Li, Liming</creatorcontrib><creatorcontrib>Li, Yong</creatorcontrib><creatorcontrib>Shi, Xuxia</creatorcontrib><creatorcontrib>Ren, Hangxing</creatorcontrib><creatorcontrib>Sun, Yuetao</creatorcontrib><creatorcontrib>Liu, Kangning</creatorcontrib><creatorcontrib>Song, Wei</creatorcontrib><creatorcontrib>Li, Huamin</creatorcontrib><creatorcontrib>Wang, Haibin</creatorcontrib><creatorcontrib>Han, Mei</creatorcontrib><creatorcontrib>Wang, Xi</creatorcontrib><creatorcontrib>Momo, Christopher Dorma</creatorcontrib><creatorcontrib>Chen, Songhua</creatorcontrib><creatorcontrib>Liu, Lihua</creatorcontrib><creatorcontrib>Liang, Hongyan</creatorcontrib><title>Entropy engineering of La-based perovskite for simultaneous photocatalytic CO2 reduction and biomass oxidation</title><title>Chemical communications (Cambridge, England)</title><description>Herein, the high-entropy perovskite, i.e. La(FeCoNiCrMn)O3, was prepared for simultaneous CO2 reduction and biomass upgrading. Based on the synergistic effect between the elements in the high-entropy material, an excellent CO evolution rate of 131.8 μmol g−1 h−1 and a xylonic acid yield of 63.9% were gained.</description><subject>Biomass</subject><subject>Carbon dioxide</subject><subject>Entropy</subject><subject>Oxidation</subject><subject>Perovskites</subject><subject>Reduction</subject><subject>Synergistic effect</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpdjk1LAzEQhoMoWKsXf0HAi5fVfG12c5RSP6DQi4K3JZtMauo2WTdZsf_eLfXkwDAvLw_Dg9A1JXeUcHVvuTFEcMXbEzSjXIqiFPX76SGXqqi4KM_RRUpbMg0t6xkKy5CH2O8xhI0PAIMPGxwdXumi1Qks7mGI3-nTZ8AuDjj53dhlHSCOCfcfMUejs-722Ru8WDM8gB1N9jFgHSxufdzplHD88VYf2kt05nSX4OrvztHb4_J18Vys1k8vi4dV0TMqc2G1dFQba6GkxElRQ6lryUFXk7QjUomWM6HAGKuEVZK5moHjlTGccKCSz9Ht8W8_xK8RUm52PhnouqN5w2rFlJj2gN78Q7dxHMJk1zBFiBSSVJz_ApYTauY</recordid><startdate>20231212</startdate><enddate>20231212</enddate><creator>Wang, Mengchen</creator><creator>Li, Liming</creator><creator>Li, Yong</creator><creator>Shi, Xuxia</creator><creator>Ren, Hangxing</creator><creator>Sun, Yuetao</creator><creator>Liu, Kangning</creator><creator>Song, Wei</creator><creator>Li, Huamin</creator><creator>Wang, Haibin</creator><creator>Han, Mei</creator><creator>Wang, Xi</creator><creator>Momo, Christopher Dorma</creator><creator>Chen, Songhua</creator><creator>Liu, Lihua</creator><creator>Liang, Hongyan</creator><general>Royal Society of Chemistry</general><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope></search><sort><creationdate>20231212</creationdate><title>Entropy engineering of La-based perovskite for simultaneous photocatalytic CO2 reduction and biomass oxidation</title><author>Wang, Mengchen ; Li, Liming ; Li, Yong ; Shi, Xuxia ; Ren, Hangxing ; Sun, Yuetao ; Liu, Kangning ; Song, Wei ; Li, Huamin ; Wang, Haibin ; Han, Mei ; Wang, Xi ; Momo, Christopher Dorma ; Chen, Songhua ; Liu, Lihua ; Liang, Hongyan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-p216t-da6f1acdde510f648e5a863ea7158f0694b3249eccd94d962f82ef37cc303e163</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Biomass</topic><topic>Carbon dioxide</topic><topic>Entropy</topic><topic>Oxidation</topic><topic>Perovskites</topic><topic>Reduction</topic><topic>Synergistic effect</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Mengchen</creatorcontrib><creatorcontrib>Li, Liming</creatorcontrib><creatorcontrib>Li, Yong</creatorcontrib><creatorcontrib>Shi, Xuxia</creatorcontrib><creatorcontrib>Ren, Hangxing</creatorcontrib><creatorcontrib>Sun, Yuetao</creatorcontrib><creatorcontrib>Liu, Kangning</creatorcontrib><creatorcontrib>Song, Wei</creatorcontrib><creatorcontrib>Li, Huamin</creatorcontrib><creatorcontrib>Wang, Haibin</creatorcontrib><creatorcontrib>Han, Mei</creatorcontrib><creatorcontrib>Wang, Xi</creatorcontrib><creatorcontrib>Momo, Christopher Dorma</creatorcontrib><creatorcontrib>Chen, Songhua</creatorcontrib><creatorcontrib>Liu, Lihua</creatorcontrib><creatorcontrib>Liang, Hongyan</creatorcontrib><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Mengchen</au><au>Li, Liming</au><au>Li, Yong</au><au>Shi, Xuxia</au><au>Ren, Hangxing</au><au>Sun, Yuetao</au><au>Liu, Kangning</au><au>Song, Wei</au><au>Li, Huamin</au><au>Wang, Haibin</au><au>Han, Mei</au><au>Wang, Xi</au><au>Momo, Christopher Dorma</au><au>Chen, Songhua</au><au>Liu, Lihua</au><au>Liang, Hongyan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Entropy engineering of La-based perovskite for simultaneous photocatalytic CO2 reduction and biomass oxidation</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><date>2023-12-12</date><risdate>2023</risdate><volume>59</volume><issue>99</issue><spage>14673</spage><epage>14676</epage><pages>14673-14676</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>Herein, the high-entropy perovskite, i.e. La(FeCoNiCrMn)O3, was prepared for simultaneous CO2 reduction and biomass upgrading. Based on the synergistic effect between the elements in the high-entropy material, an excellent CO evolution rate of 131.8 μmol g−1 h−1 and a xylonic acid yield of 63.9% were gained.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/d3cc04393b</doi><tpages>4</tpages></addata></record> |
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| ispartof | Chemical communications (Cambridge, England), 2023-12, Vol.59 (99), p.14673-14676 |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Biomass Carbon dioxide Entropy Oxidation Perovskites Reduction Synergistic effect |
| title | Entropy engineering of La-based perovskite for simultaneous photocatalytic CO2 reduction and biomass oxidation |
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