Creating glassy states of dicarboxylate-bridged coordination polymers
We report the direct formation of dicarboxylate-based coordination polymer glasses through thermal dehydration. The rearrangement of the coordination networks caused by dehydration was monitored by in situ powder X-ray diffraction, infrared spectroscopy, and synchrotron X-ray characterizations. The...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2023-11, Vol.59 (96), p.14317-1432 |
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| container_title | Chemical communications (Cambridge, England) |
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| creator | Fan, Zeyu Wei, Yong-Sheng Das, Chinmoy Kanamori, Kazuyoshi Yamada, Hiroki Ohara, Koji Horike, Satoshi |
| description | We report the direct formation of dicarboxylate-based coordination polymer glasses through thermal dehydration. The rearrangement of the coordination networks caused by dehydration was monitored by
in situ
powder X-ray diffraction, infrared spectroscopy, and synchrotron X-ray characterizations. The microporosity and mechanical properties of these glasses were investigated.
A series of dicarboxylate-bridged networked glasses with tunable porosity and mechanical properties were obtained by dehydration of hydrated coordination polymer crystals. |
| doi_str_mv | 10.1039/d3cc04518h |
| format | Article |
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in situ
powder X-ray diffraction, infrared spectroscopy, and synchrotron X-ray characterizations. The microporosity and mechanical properties of these glasses were investigated.
A series of dicarboxylate-bridged networked glasses with tunable porosity and mechanical properties were obtained by dehydration of hydrated coordination polymer crystals.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/d3cc04518h</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Coordination polymers ; Dehydration ; Mechanical properties ; Microporosity ; Synchrotron radiation ; Synchrotrons ; X ray powder diffraction</subject><ispartof>Chemical communications (Cambridge, England), 2023-11, Vol.59 (96), p.14317-1432</ispartof><rights>Copyright Royal Society of Chemistry 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c314t-d1a6940e1ff630bc0eb80215eded3f7349957dd3b3a83a0ab7f65dc85f315d983</citedby><cites>FETCH-LOGICAL-c314t-d1a6940e1ff630bc0eb80215eded3f7349957dd3b3a83a0ab7f65dc85f315d983</cites><orcidid>0000-0003-3340-3626 ; 0009-0004-2431-6285 ; 0000-0001-8530-6364</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Fan, Zeyu</creatorcontrib><creatorcontrib>Wei, Yong-Sheng</creatorcontrib><creatorcontrib>Das, Chinmoy</creatorcontrib><creatorcontrib>Kanamori, Kazuyoshi</creatorcontrib><creatorcontrib>Yamada, Hiroki</creatorcontrib><creatorcontrib>Ohara, Koji</creatorcontrib><creatorcontrib>Horike, Satoshi</creatorcontrib><title>Creating glassy states of dicarboxylate-bridged coordination polymers</title><title>Chemical communications (Cambridge, England)</title><description>We report the direct formation of dicarboxylate-based coordination polymer glasses through thermal dehydration. The rearrangement of the coordination networks caused by dehydration was monitored by
in situ
powder X-ray diffraction, infrared spectroscopy, and synchrotron X-ray characterizations. The microporosity and mechanical properties of these glasses were investigated.
A series of dicarboxylate-bridged networked glasses with tunable porosity and mechanical properties were obtained by dehydration of hydrated coordination polymer crystals.</description><subject>Coordination polymers</subject><subject>Dehydration</subject><subject>Mechanical properties</subject><subject>Microporosity</subject><subject>Synchrotron radiation</subject><subject>Synchrotrons</subject><subject>X ray powder diffraction</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpd0E1LxDAQBuAgCq6rF-9CwYsI1aRJ2uQodXWFBS8K3kqaj9ql26yZLth_b-qKgrlMGJ4Zhhehc4JvCKby1lCtMeNEvB-gGaE5SzkTb4fTn8u0oIwfoxOANY6PcDFDizJYNbR9kzSdAhgTGNRgIfEuMa1WofafYxc7aR1a01iTaO-Dafs44_tk67txYwOcoiOnOrBnP3WOXh8WL-UyXT0_PpV3q1RTwobUEJVLhi1xLqe41tjWAmeEW2MNdfE6KXlhDK2pElRhVRcu50YL7ijhRgo6R1f7vdvgP3YWhmrTgrZdp3rrd1BlQpKC54xP9PIfXftd6ON1k-JZJkReRHW9Vzp4gGBdtQ3tRoWxIriaEq3uaVl-J7qM-GKPA-hf95c4_QJdt3Lc</recordid><startdate>20231130</startdate><enddate>20231130</enddate><creator>Fan, Zeyu</creator><creator>Wei, Yong-Sheng</creator><creator>Das, Chinmoy</creator><creator>Kanamori, Kazuyoshi</creator><creator>Yamada, Hiroki</creator><creator>Ohara, Koji</creator><creator>Horike, Satoshi</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-3340-3626</orcidid><orcidid>https://orcid.org/0009-0004-2431-6285</orcidid><orcidid>https://orcid.org/0000-0001-8530-6364</orcidid></search><sort><creationdate>20231130</creationdate><title>Creating glassy states of dicarboxylate-bridged coordination polymers</title><author>Fan, Zeyu ; Wei, Yong-Sheng ; Das, Chinmoy ; Kanamori, Kazuyoshi ; Yamada, Hiroki ; Ohara, Koji ; Horike, Satoshi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c314t-d1a6940e1ff630bc0eb80215eded3f7349957dd3b3a83a0ab7f65dc85f315d983</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Coordination polymers</topic><topic>Dehydration</topic><topic>Mechanical properties</topic><topic>Microporosity</topic><topic>Synchrotron radiation</topic><topic>Synchrotrons</topic><topic>X ray powder diffraction</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Fan, Zeyu</creatorcontrib><creatorcontrib>Wei, Yong-Sheng</creatorcontrib><creatorcontrib>Das, Chinmoy</creatorcontrib><creatorcontrib>Kanamori, Kazuyoshi</creatorcontrib><creatorcontrib>Yamada, Hiroki</creatorcontrib><creatorcontrib>Ohara, Koji</creatorcontrib><creatorcontrib>Horike, Satoshi</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Fan, Zeyu</au><au>Wei, Yong-Sheng</au><au>Das, Chinmoy</au><au>Kanamori, Kazuyoshi</au><au>Yamada, Hiroki</au><au>Ohara, Koji</au><au>Horike, Satoshi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Creating glassy states of dicarboxylate-bridged coordination polymers</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><date>2023-11-30</date><risdate>2023</risdate><volume>59</volume><issue>96</issue><spage>14317</spage><epage>1432</epage><pages>14317-1432</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>We report the direct formation of dicarboxylate-based coordination polymer glasses through thermal dehydration. The rearrangement of the coordination networks caused by dehydration was monitored by
in situ
powder X-ray diffraction, infrared spectroscopy, and synchrotron X-ray characterizations. The microporosity and mechanical properties of these glasses were investigated.
A series of dicarboxylate-bridged networked glasses with tunable porosity and mechanical properties were obtained by dehydration of hydrated coordination polymer crystals.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/d3cc04518h</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0003-3340-3626</orcidid><orcidid>https://orcid.org/0009-0004-2431-6285</orcidid><orcidid>https://orcid.org/0000-0001-8530-6364</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2023-11, Vol.59 (96), p.14317-1432 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2891756458 |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Coordination polymers Dehydration Mechanical properties Microporosity Synchrotron radiation Synchrotrons X ray powder diffraction |
| title | Creating glassy states of dicarboxylate-bridged coordination polymers |
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