Kinetic magnetism in triangular moiré materials

Magnetic properties of materials ranging from conventional ferromagnetic metals to strongly correlated materials such as cuprates originate from Coulomb exchange interactions. The existence of alternate mechanisms for magnetism that could naturally facilitate electrical control has been discussed th...

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Veröffentlicht in:Nature (London) 2023-11, Vol.623 (7987), p.509-513
Hauptverfasser: Ciorciaro, L., Smoleński, T., Morera, I., Kiper, N., Hiestand, S., Kroner, M., Zhang, Y., Watanabe, K., Taniguchi, T., Demler, E., İmamoğlu, A.
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container_issue 7987
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container_title Nature (London)
container_volume 623
creator Ciorciaro, L.
Smoleński, T.
Morera, I.
Kiper, N.
Hiestand, S.
Kroner, M.
Zhang, Y.
Watanabe, K.
Taniguchi, T.
Demler, E.
İmamoğlu, A.
description Magnetic properties of materials ranging from conventional ferromagnetic metals to strongly correlated materials such as cuprates originate from Coulomb exchange interactions. The existence of alternate mechanisms for magnetism that could naturally facilitate electrical control has been discussed theoretically 1 – 7 , but an experimental demonstration 8 in an extended system has been missing. Here we investigate MoSe 2 /WS 2 van der Waals heterostructures in the vicinity of Mott insulator states of electrons forming a frustrated triangular lattice and observe direct evidence of magnetic correlations originating from a kinetic mechanism. By directly measuring electronic magnetization through the strength of the polarization-selective attractive polaron resonance 9 , 10 , we find that when the Mott state is electron-doped, the system exhibits ferromagnetic correlations in agreement with the Nagaoka mechanism. Minimization of kinetic energy leads to ferromagnetic correlations between itinerant electrons in MoSe 2 /WS 2 moiré lattices even in the absence of exchange interactions.
doi_str_mv 10.1038/s41586-023-06633-0
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subjects 140/125
639/766/119/1000/1018
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Correlation
Cuprates
Electrons
Ferromagnetic materials
Graphene
Heterostructures
Humanities and Social Sciences
Investigations
Magnetic fields
Magnetic properties
Magnetism
Material properties
Metals
multidisciplinary
Physics
Science
Science (multidisciplinary)
Temperature
title Kinetic magnetism in triangular moiré materials
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