Interacting Phonons between Layers in Raman Spectra of Carbon Nanotubes inside Boron Nitride Nanotubes

We present the resonant Raman spectra of a single-wall carbon nanotube inside a multiwall boron nitride nanotube (SWNT@BNNT). At E L = 1.58 eV, SWNT@BNNT exhibited resonant Raman spectra at 807 (ωBN) and 804 cm–1 (ωGr). Their intensities almost disappeared at E L = 2.33 eV. We assigned ωBN to the ou...

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Veröffentlicht in:	The journal of physical chemistry letters 2023-11, Vol.14 (45), p.10263-10270
Hauptverfasser:	Gulo, Desman Perdamaian, Hung, Nguyen Tuan, Chen, Wei-Liang, Wang, Shuhui, Liu, Ming, Kauppinen, Esko I., Maruyama, Shigeo, Chang, Yu-Ming, Saito, Riichiro, Liu, Hsiang-Lin
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container_title	The journal of physical chemistry letters
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creator	Gulo, Desman Perdamaian Hung, Nguyen Tuan Chen, Wei-Liang Wang, Shuhui Liu, Ming Kauppinen, Esko I. Maruyama, Shigeo Chang, Yu-Ming Saito, Riichiro Liu, Hsiang-Lin
description	We present the resonant Raman spectra of a single-wall carbon nanotube inside a multiwall boron nitride nanotube (SWNT@BNNT). At E L = 1.58 eV, SWNT@BNNT exhibited resonant Raman spectra at 807 (ωBN) and 804 cm–1 (ωGr). Their intensities almost disappeared at E L = 2.33 eV. We assigned ωBN to the out-of-plane BN phonon mode that coupled with ωGr. At E L = 4.66 eV, the G+ and G– bands of the SWNT@BNNT red-shifted 3.8 cm–1 compared with the SWNT, suggesting the interwall interactions between the in-plane modes of SWNT and BNNT. Moreover, the E 2g mode of the BNNT in SWNT@BNNT appeared at 1370.3 ± 0.1 cm–1, which is undistinguishable for E L < 3 eV because of the overlap with the D band frequency. The assignment of the present Raman spectra was confirmed through the first-principles calculations.
doi_str_mv	10.1021/acs.jpclett.3c02528
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At E L = 1.58 eV, SWNT@BNNT exhibited resonant Raman spectra at 807 (ωBN) and 804 cm–1 (ωGr). Their intensities almost disappeared at E L = 2.33 eV. We assigned ωBN to the out-of-plane BN phonon mode that coupled with ωGr. At E L = 4.66 eV, the G+ and G– bands of the SWNT@BNNT red-shifted 3.8 cm–1 compared with the SWNT, suggesting the interwall interactions between the in-plane modes of SWNT and BNNT. Moreover, the E 2g mode of the BNNT in SWNT@BNNT appeared at 1370.3 ± 0.1 cm–1, which is undistinguishable for E L < 3 eV because of the overlap with the D band frequency. The assignment of the present Raman spectra was confirmed through the first-principles calculations.</description><identifier>ISSN: 1948-7185</identifier><identifier>EISSN: 1948-7185</identifier><identifier>DOI: 10.1021/acs.jpclett.3c02528</identifier><identifier>PMID: 37939010</identifier><language>eng</language><publisher>United States: American Chemical Society</publisher><subject>Physical Insights into Light Interacting with Matter</subject><ispartof>The journal of physical chemistry letters, 2023-11, Vol.14 (45), p.10263-10270</ispartof><rights>2023 American Chemical Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a345t-a7043e9076dcbc4944bdaafe50f0100cf64acbb272f7da96089c7c48e451695b3</citedby><cites>FETCH-LOGICAL-a345t-a7043e9076dcbc4944bdaafe50f0100cf64acbb272f7da96089c7c48e451695b3</cites><orcidid>0000-0003-3694-3070 ; 0000-0003-1960-2776 ; 0000-0002-5630-3874 ; 0000-0003-1727-8810 ; 0000-0002-3336-9985 ; 0000-0003-4156-6230</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acs.jpclett.3c02528$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acs.jpclett.3c02528$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,778,782,2754,27063,27911,27912,56725,56775</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/37939010$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Gulo, Desman Perdamaian</creatorcontrib><creatorcontrib>Hung, Nguyen Tuan</creatorcontrib><creatorcontrib>Chen, Wei-Liang</creatorcontrib><creatorcontrib>Wang, Shuhui</creatorcontrib><creatorcontrib>Liu, Ming</creatorcontrib><creatorcontrib>Kauppinen, Esko I.</creatorcontrib><creatorcontrib>Maruyama, Shigeo</creatorcontrib><creatorcontrib>Chang, Yu-Ming</creatorcontrib><creatorcontrib>Saito, Riichiro</creatorcontrib><creatorcontrib>Liu, Hsiang-Lin</creatorcontrib><title>Interacting Phonons between Layers in Raman Spectra of Carbon Nanotubes inside Boron Nitride Nanotubes</title><title>The journal of physical chemistry letters</title><addtitle>J. Phys. Chem. Lett</addtitle><description>We present the resonant Raman spectra of a single-wall carbon nanotube inside a multiwall boron nitride nanotube (SWNT@BNNT). At E L = 1.58 eV, SWNT@BNNT exhibited resonant Raman spectra at 807 (ωBN) and 804 cm–1 (ωGr). Their intensities almost disappeared at E L = 2.33 eV. We assigned ωBN to the out-of-plane BN phonon mode that coupled with ωGr. At E L = 4.66 eV, the G+ and G– bands of the SWNT@BNNT red-shifted 3.8 cm–1 compared with the SWNT, suggesting the interwall interactions between the in-plane modes of SWNT and BNNT. Moreover, the E 2g mode of the BNNT in SWNT@BNNT appeared at 1370.3 ± 0.1 cm–1, which is undistinguishable for E L < 3 eV because of the overlap with the D band frequency. 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Phys. Chem. Lett</addtitle><date>2023-11-16</date><risdate>2023</risdate><volume>14</volume><issue>45</issue><spage>10263</spage><epage>10270</epage><pages>10263-10270</pages><issn>1948-7185</issn><eissn>1948-7185</eissn><abstract>We present the resonant Raman spectra of a single-wall carbon nanotube inside a multiwall boron nitride nanotube (SWNT@BNNT). At E L = 1.58 eV, SWNT@BNNT exhibited resonant Raman spectra at 807 (ωBN) and 804 cm–1 (ωGr). Their intensities almost disappeared at E L = 2.33 eV. We assigned ωBN to the out-of-plane BN phonon mode that coupled with ωGr. At E L = 4.66 eV, the G+ and G– bands of the SWNT@BNNT red-shifted 3.8 cm–1 compared with the SWNT, suggesting the interwall interactions between the in-plane modes of SWNT and BNNT. Moreover, the E 2g mode of the BNNT in SWNT@BNNT appeared at 1370.3 ± 0.1 cm–1, which is undistinguishable for E L < 3 eV because of the overlap with the D band frequency. 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title	Interacting Phonons between Layers in Raman Spectra of Carbon Nanotubes inside Boron Nitride Nanotubes
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