Calibration and Application of PUF Disk Passive Air Samplers To Assess Chlorinated Paraffins in Ambient Air in Australia, China, and Vietnam
Ambient air samples were collected in Brisbane (Australia), Dalian (China), and Hanoi (Vietnam) during Mar 2013–Feb 2018 using polyurethane foam based passive air samplers. A sampling rate calibration experiment was conducted for chlorinated paraffins (CPs, i.e., short-chain, medium-chain, and long-...
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| Veröffentlicht in: | Environmental science & technology 2023-12, Vol.57 (50), p.21061-21070 |
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| creator | He, Chang Thai, Phong K. Bertrand, Lidwina Jayarathne, Ayomi van Mourik, Louise Phuc, Dam Hoang Banks, Andrew Mueller, Jochen F. Wang, Xianyu Fisher |
| description | Ambient air samples were collected in Brisbane (Australia), Dalian (China), and Hanoi (Vietnam) during Mar 2013–Feb 2018 using polyurethane foam based passive air samplers. A sampling rate calibration experiment was conducted for chlorinated paraffins (CPs, i.e., short-chain, medium-chain, and long-chain CPs), where the sampling rates were 4.5 ± 0.7, 4.8 ± 0.3, and 4.8 ± 2.1 m3 day–1 for SCCPs, MCCPs, and LCCPs, respectively. The atmospheric concentration of CPs was then calculated and the medians of ∑CPs were 0.079, 1.0, and 0.89 ng m–3 in Brisbane, Dalian, and Hanoi, respectively. The concentration of CPs in Brisbane’s air remained at low levels, with no significant differences observed between the city background site and the city center site, indicating limited usage and production of CPs in this city. The highest concentration of MCCPs was detected in Dalian, while the highest concentration of SCCPs was detected in Hanoi. A decrease of SCCP concentration and an increase of MCCPs’ were found in Brisbane’s air from 2016 to 2018, while increasing trends for both SCCPs and MCCPs were observed in Dalian. These results indicated impacts from different sources of CPs in the investigated cities. |
| doi_str_mv | 10.1021/acs.est.3c06703 |
| format | Article |
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A sampling rate calibration experiment was conducted for chlorinated paraffins (CPs, i.e., short-chain, medium-chain, and long-chain CPs), where the sampling rates were 4.5 ± 0.7, 4.8 ± 0.3, and 4.8 ± 2.1 m3 day–1 for SCCPs, MCCPs, and LCCPs, respectively. The atmospheric concentration of CPs was then calculated and the medians of ∑CPs were 0.079, 1.0, and 0.89 ng m–3 in Brisbane, Dalian, and Hanoi, respectively. The concentration of CPs in Brisbane’s air remained at low levels, with no significant differences observed between the city background site and the city center site, indicating limited usage and production of CPs in this city. The highest concentration of MCCPs was detected in Dalian, while the highest concentration of SCCPs was detected in Hanoi. A decrease of SCCP concentration and an increase of MCCPs’ were found in Brisbane’s air from 2016 to 2018, while increasing trends for both SCCPs and MCCPs were observed in Dalian. These results indicated impacts from different sources of CPs in the investigated cities.</description><identifier>ISSN: 0013-936X</identifier><identifier>EISSN: 1520-5851</identifier><identifier>DOI: 10.1021/acs.est.3c06703</identifier><identifier>PMID: 37939218</identifier><language>eng</language><publisher>United States: American Chemical Society</publisher><subject>Air sampling ; Australia ; Calibration ; China ; Cities ; City centres ; Ecotoxicology and Public Health ; Environmental Monitoring - methods ; Hydrocarbons, Chlorinated - analysis ; Paraffin - analysis ; Paraffins ; Polyurethane ; Polyurethane foam ; Samplers ; Sampling ; Vietnam</subject><ispartof>Environmental science & technology, 2023-12, Vol.57 (50), p.21061-21070</ispartof><rights>2023 American Chemical Society</rights><rights>Copyright American Chemical Society Dec 19, 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-a315t-5ad555592cdc7bbbee6eb7d657389336045b7a629e2ce04bdbd461689838da6e3</cites><orcidid>0000-0002-5917-3366 ; 0000-0003-2345-5940 ; 0000-0003-3536-8895 ; 0000-0003-0042-3057</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acs.est.3c06703$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acs.est.3c06703$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,2763,27075,27923,27924,56737,56787</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/37939218$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>He, Chang</creatorcontrib><creatorcontrib>Thai, Phong K.</creatorcontrib><creatorcontrib>Bertrand, Lidwina</creatorcontrib><creatorcontrib>Jayarathne, Ayomi</creatorcontrib><creatorcontrib>van Mourik, Louise</creatorcontrib><creatorcontrib>Phuc, Dam Hoang</creatorcontrib><creatorcontrib>Banks, Andrew</creatorcontrib><creatorcontrib>Mueller, Jochen F.</creatorcontrib><creatorcontrib>Wang, Xianyu Fisher</creatorcontrib><title>Calibration and Application of PUF Disk Passive Air Samplers To Assess Chlorinated Paraffins in Ambient Air in Australia, China, and Vietnam</title><title>Environmental science & technology</title><addtitle>Environ. Sci. Technol</addtitle><description>Ambient air samples were collected in Brisbane (Australia), Dalian (China), and Hanoi (Vietnam) during Mar 2013–Feb 2018 using polyurethane foam based passive air samplers. A sampling rate calibration experiment was conducted for chlorinated paraffins (CPs, i.e., short-chain, medium-chain, and long-chain CPs), where the sampling rates were 4.5 ± 0.7, 4.8 ± 0.3, and 4.8 ± 2.1 m3 day–1 for SCCPs, MCCPs, and LCCPs, respectively. The atmospheric concentration of CPs was then calculated and the medians of ∑CPs were 0.079, 1.0, and 0.89 ng m–3 in Brisbane, Dalian, and Hanoi, respectively. The concentration of CPs in Brisbane’s air remained at low levels, with no significant differences observed between the city background site and the city center site, indicating limited usage and production of CPs in this city. The highest concentration of MCCPs was detected in Dalian, while the highest concentration of SCCPs was detected in Hanoi. A decrease of SCCP concentration and an increase of MCCPs’ were found in Brisbane’s air from 2016 to 2018, while increasing trends for both SCCPs and MCCPs were observed in Dalian. These results indicated impacts from different sources of CPs in the investigated cities.</description><subject>Air sampling</subject><subject>Australia</subject><subject>Calibration</subject><subject>China</subject><subject>Cities</subject><subject>City centres</subject><subject>Ecotoxicology and Public Health</subject><subject>Environmental Monitoring - methods</subject><subject>Hydrocarbons, Chlorinated - analysis</subject><subject>Paraffin - analysis</subject><subject>Paraffins</subject><subject>Polyurethane</subject><subject>Polyurethane foam</subject><subject>Samplers</subject><subject>Sampling</subject><subject>Vietnam</subject><issn>0013-936X</issn><issn>1520-5851</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNp1kU-L1TAUxYMoznN07U4CbgSnb_KnSZNleToqDDjgjLgrSXuLGdu0k9sKfgc_tHnznrMQvJvLhd85J-QQ8pKzLWeCn7sWt4DLVrZMV0w-IhuuBCuUUfwx2TDGZWGl_nZCniHeMsaEZOYpOZGVlVZwsyG_d24IPrklTJG62NF6nofQHu6pp1c3F_RdwB_0yiGGn0DrkOgXN84DJKTXE60RAZHuvg9TCtEt0GU0ub4PEWmItB59gLjc6_bnikvKke4sSzJ_dh_6NcAS3ficPOndgPDiuE_JzcX7693H4vLzh0-7-rJwkqulUK5Teaxou7by3gNo8FWnVSWNlVKzUvnKaWFBtMBK3_mu1Fwba6TpnAZ5St4cfOc03a35_5oxYAvD4CJMKzbCGMMkL3mZ0df_oLfTmmJ-XSMsU1ZWpeKZOj9QbZoQE_TNnMLo0q-Gs2ZfVJOLavbqY1FZ8erou_oRugf-bzMZeHsA9sqHzP_Z_QFSDJ3s</recordid><startdate>20231219</startdate><enddate>20231219</enddate><creator>He, Chang</creator><creator>Thai, Phong K.</creator><creator>Bertrand, Lidwina</creator><creator>Jayarathne, Ayomi</creator><creator>van Mourik, Louise</creator><creator>Phuc, Dam Hoang</creator><creator>Banks, Andrew</creator><creator>Mueller, Jochen F.</creator><creator>Wang, Xianyu Fisher</creator><general>American Chemical Society</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QO</scope><scope>7ST</scope><scope>7T7</scope><scope>7U7</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>P64</scope><scope>SOI</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-5917-3366</orcidid><orcidid>https://orcid.org/0000-0003-2345-5940</orcidid><orcidid>https://orcid.org/0000-0003-3536-8895</orcidid><orcidid>https://orcid.org/0000-0003-0042-3057</orcidid></search><sort><creationdate>20231219</creationdate><title>Calibration and Application of PUF Disk Passive Air Samplers To Assess Chlorinated Paraffins in Ambient Air in Australia, China, and Vietnam</title><author>He, Chang ; Thai, Phong K. ; Bertrand, Lidwina ; Jayarathne, Ayomi ; van Mourik, Louise ; Phuc, Dam Hoang ; Banks, Andrew ; Mueller, Jochen F. ; Wang, Xianyu Fisher</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a315t-5ad555592cdc7bbbee6eb7d657389336045b7a629e2ce04bdbd461689838da6e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Air sampling</topic><topic>Australia</topic><topic>Calibration</topic><topic>China</topic><topic>Cities</topic><topic>City centres</topic><topic>Ecotoxicology and Public Health</topic><topic>Environmental Monitoring - methods</topic><topic>Hydrocarbons, Chlorinated - analysis</topic><topic>Paraffin - analysis</topic><topic>Paraffins</topic><topic>Polyurethane</topic><topic>Polyurethane foam</topic><topic>Samplers</topic><topic>Sampling</topic><topic>Vietnam</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>He, Chang</creatorcontrib><creatorcontrib>Thai, Phong K.</creatorcontrib><creatorcontrib>Bertrand, Lidwina</creatorcontrib><creatorcontrib>Jayarathne, Ayomi</creatorcontrib><creatorcontrib>van Mourik, Louise</creatorcontrib><creatorcontrib>Phuc, Dam Hoang</creatorcontrib><creatorcontrib>Banks, Andrew</creatorcontrib><creatorcontrib>Mueller, Jochen F.</creatorcontrib><creatorcontrib>Wang, Xianyu Fisher</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Biotechnology Research Abstracts</collection><collection>Environment Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Toxicology Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environment Abstracts</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science & technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>He, Chang</au><au>Thai, Phong K.</au><au>Bertrand, Lidwina</au><au>Jayarathne, Ayomi</au><au>van Mourik, Louise</au><au>Phuc, Dam Hoang</au><au>Banks, Andrew</au><au>Mueller, Jochen F.</au><au>Wang, Xianyu Fisher</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Calibration and Application of PUF Disk Passive Air Samplers To Assess Chlorinated Paraffins in Ambient Air in Australia, China, and Vietnam</atitle><jtitle>Environmental science & technology</jtitle><addtitle>Environ. Sci. Technol</addtitle><date>2023-12-19</date><risdate>2023</risdate><volume>57</volume><issue>50</issue><spage>21061</spage><epage>21070</epage><pages>21061-21070</pages><issn>0013-936X</issn><eissn>1520-5851</eissn><abstract>Ambient air samples were collected in Brisbane (Australia), Dalian (China), and Hanoi (Vietnam) during Mar 2013–Feb 2018 using polyurethane foam based passive air samplers. A sampling rate calibration experiment was conducted for chlorinated paraffins (CPs, i.e., short-chain, medium-chain, and long-chain CPs), where the sampling rates were 4.5 ± 0.7, 4.8 ± 0.3, and 4.8 ± 2.1 m3 day–1 for SCCPs, MCCPs, and LCCPs, respectively. The atmospheric concentration of CPs was then calculated and the medians of ∑CPs were 0.079, 1.0, and 0.89 ng m–3 in Brisbane, Dalian, and Hanoi, respectively. The concentration of CPs in Brisbane’s air remained at low levels, with no significant differences observed between the city background site and the city center site, indicating limited usage and production of CPs in this city. The highest concentration of MCCPs was detected in Dalian, while the highest concentration of SCCPs was detected in Hanoi. A decrease of SCCP concentration and an increase of MCCPs’ were found in Brisbane’s air from 2016 to 2018, while increasing trends for both SCCPs and MCCPs were observed in Dalian. These results indicated impacts from different sources of CPs in the investigated cities.</abstract><cop>United States</cop><pub>American Chemical Society</pub><pmid>37939218</pmid><doi>10.1021/acs.est.3c06703</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-5917-3366</orcidid><orcidid>https://orcid.org/0000-0003-2345-5940</orcidid><orcidid>https://orcid.org/0000-0003-3536-8895</orcidid><orcidid>https://orcid.org/0000-0003-0042-3057</orcidid></addata></record> |
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| subjects | Air sampling Australia Calibration China Cities City centres Ecotoxicology and Public Health Environmental Monitoring - methods Hydrocarbons, Chlorinated - analysis Paraffin - analysis Paraffins Polyurethane Polyurethane foam Samplers Sampling Vietnam |
| title | Calibration and Application of PUF Disk Passive Air Samplers To Assess Chlorinated Paraffins in Ambient Air in Australia, China, and Vietnam |
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