Low-pressure CO2 sorption in ammonium-based poly(ionic liquid)s

Low-pressure CO2 sorption in ammonium-based poly(ionic liquid)s

Ammonium-based ionic liquid monomers and their corresponding polymers [poly(ionic liquid)s] are synthesized and characterized for CO2 sorption. The polymers have much higher CO2 sorption capacities than the room-temperature ionic liquids and imidazolium-based poly(ionic liquid)s. For example, P[VBTM...

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Veröffentlicht in:Polymer (Guilford) 2005-12, Vol.46 (26), p.12460-12467
Hauptverfasser: JIANBIN TANG, HUADONG TANG, WEILIN SUN, RADOSZ, Maciej, YOUQING SHEN
Format: Artikel
Sprache:eng
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Applied sciences
Exact sciences and technology
Organic polymers
Physicochemistry of polymers
Polymerization
Preparation, kinetics, thermodynamics, mechanism and catalysts
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container_end_page 12467
container_issue 26
container_start_page 12460
container_title Polymer (Guilford)
container_volume 46
creator JIANBIN TANG
HUADONG TANG
WEILIN SUN
RADOSZ, Maciej
YOUQING SHEN
description Ammonium-based ionic liquid monomers and their corresponding polymers [poly(ionic liquid)s] are synthesized and characterized for CO2 sorption. The polymers have much higher CO2 sorption capacities than the room-temperature ionic liquids and imidazolium-based poly(ionic liquid)s. For example, P[VBTMA][PF6] with polystyrene backbone has a CO2 sorption capacity of 10DDT67mol%. The CO2 sorption is selective over N2 and O2. The effects of cation, backbone, substituent, anion and crosslinking on CO2 sorption are discussed. The sorption mechanism study indicates that CO2 sorption by the poly(ionic liquid)s is a bulk and surface phenomenon.
doi_str_mv 10.1016/j.polymer.2005.10.082
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subjects Applied sciences
Exact sciences and technology
Organic polymers
Physicochemistry of polymers
Polymerization
Preparation, kinetics, thermodynamics, mechanism and catalysts
title Low-pressure CO2 sorption in ammonium-based poly(ionic liquid)s
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