Arsenic sorption by carbonate-rich aquifer material, a control on arsenic mobility at Zimapán, México
Arsenic retention by carbonate-rich aquifer material at Zimapán, México, was studied to gain insight into the processes controlling arsenic mobility in natural systems. Batch experiments showed that retention of soluble As (V) on carbonate-rich aquifer material was 35.3-90% in the pH range of 7-9 fo...
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| Veröffentlicht in: | Archives of environmental contamination and toxicology 2004-07, Vol.47 (1), p.1-13 |
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| description | Arsenic retention by carbonate-rich aquifer material at Zimapán, México, was studied to gain insight into the processes controlling arsenic mobility in natural systems. Batch experiments showed that retention of soluble As (V) on carbonate-rich aquifer material was 35.3-90% in the pH range of 7-9 found in Zimapán natural water. Chemical and mineralogical compositions, point of zero charge (PZC), and experimental arsenic retention at various pH of three composite samples of limestone (M1, M2, M3) showed that sorption (adsorption and coprecipitation) may be one of the main processes controlling arsenic mobility in the Zimapán As-polluted aquifer. The PZC values approximately corresponded to the PZC reported for the main minerals present in each sample: hydrous ferric oxides (M1), calcite (M2), and the range from hydrous ferric oxides and calcite (M3). The chemical and mineralogical compositions of each sample explain the obtained PZC values. Experimental and modeled arsenic retention at various pH values on sample M1 corresponded to reported arsenic adsorption onto hydrous ferric oxides. Coprecipitacion of complex Ca arsenates or arsenic adsorption onto calcite or clay minerals could be the main processes of arsenic retention on samples M2 and M3. Groundwater flow through the granular, carbonate-rich, shallow aquifer may decrease the water As content as a result of these interactions. A remediation method based on the promotion of polluted water flow into the shallow aquifer could be developed from these results. |
| doi_str_mv | 10.1007/s00244-004-3009-1 |
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M ; ARMIENTA, M. A ; CARRILLO-CHAVEZ, A</creator><creatorcontrib>ROMERO, F. M ; ARMIENTA, M. A ; CARRILLO-CHAVEZ, A</creatorcontrib><description>Arsenic retention by carbonate-rich aquifer material at Zimapán, México, was studied to gain insight into the processes controlling arsenic mobility in natural systems. Batch experiments showed that retention of soluble As (V) on carbonate-rich aquifer material was 35.3-90% in the pH range of 7-9 found in Zimapán natural water. Chemical and mineralogical compositions, point of zero charge (PZC), and experimental arsenic retention at various pH of three composite samples of limestone (M1, M2, M3) showed that sorption (adsorption and coprecipitation) may be one of the main processes controlling arsenic mobility in the Zimapán As-polluted aquifer. The PZC values approximately corresponded to the PZC reported for the main minerals present in each sample: hydrous ferric oxides (M1), calcite (M2), and the range from hydrous ferric oxides and calcite (M3). The chemical and mineralogical compositions of each sample explain the obtained PZC values. Experimental and modeled arsenic retention at various pH values on sample M1 corresponded to reported arsenic adsorption onto hydrous ferric oxides. Coprecipitacion of complex Ca arsenates or arsenic adsorption onto calcite or clay minerals could be the main processes of arsenic retention on samples M2 and M3. Groundwater flow through the granular, carbonate-rich, shallow aquifer may decrease the water As content as a result of these interactions. A remediation method based on the promotion of polluted water flow into the shallow aquifer could be developed from these results.</description><identifier>ISSN: 0090-4341</identifier><identifier>EISSN: 1432-0703</identifier><identifier>DOI: 10.1007/s00244-004-3009-1</identifier><identifier>PMID: 15346773</identifier><identifier>CODEN: AECTCV</identifier><language>eng</language><publisher>Heidelberg: Springer-Verlag</publisher><subject>Adsorption ; Animal, plant and microbial ecology ; Applied ecology ; Aquifers ; Arsenates ; Arsenic ; Arsenic - chemistry ; Biological and medical sciences ; Calcite ; Carbonates - chemistry ; Chemical Precipitation ; Clay minerals ; Ecotoxicology, biological effects of pollution ; Fundamental and applied biological sciences. Psychology ; General aspects ; Groundwater flow ; Hydrogen-Ion Concentration ; Limestone ; Mexico ; Mineralogy ; Minerals ; Oxides ; Retention ; Sorption ; Water flow ; Water Movements ; Water Pollutants - isolation & purification ; Water pollution ; Water Pollution - prevention & control ; Water Supply</subject><ispartof>Archives of environmental contamination and toxicology, 2004-07, Vol.47 (1), p.1-13</ispartof><rights>2004 INIST-CNRS</rights><rights>Springer-Verlag New York Inc. 2004</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=15837499$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/15346773$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>ROMERO, F. M</creatorcontrib><creatorcontrib>ARMIENTA, M. A</creatorcontrib><creatorcontrib>CARRILLO-CHAVEZ, A</creatorcontrib><title>Arsenic sorption by carbonate-rich aquifer material, a control on arsenic mobility at Zimapán, México</title><title>Archives of environmental contamination and toxicology</title><addtitle>Arch Environ Contam Toxicol</addtitle><description>Arsenic retention by carbonate-rich aquifer material at Zimapán, México, was studied to gain insight into the processes controlling arsenic mobility in natural systems. Batch experiments showed that retention of soluble As (V) on carbonate-rich aquifer material was 35.3-90% in the pH range of 7-9 found in Zimapán natural water. Chemical and mineralogical compositions, point of zero charge (PZC), and experimental arsenic retention at various pH of three composite samples of limestone (M1, M2, M3) showed that sorption (adsorption and coprecipitation) may be one of the main processes controlling arsenic mobility in the Zimapán As-polluted aquifer. The PZC values approximately corresponded to the PZC reported for the main minerals present in each sample: hydrous ferric oxides (M1), calcite (M2), and the range from hydrous ferric oxides and calcite (M3). The chemical and mineralogical compositions of each sample explain the obtained PZC values. Experimental and modeled arsenic retention at various pH values on sample M1 corresponded to reported arsenic adsorption onto hydrous ferric oxides. Coprecipitacion of complex Ca arsenates or arsenic adsorption onto calcite or clay minerals could be the main processes of arsenic retention on samples M2 and M3. Groundwater flow through the granular, carbonate-rich, shallow aquifer may decrease the water As content as a result of these interactions. A remediation method based on the promotion of polluted water flow into the shallow aquifer could be developed from these results.</description><subject>Adsorption</subject><subject>Animal, plant and microbial ecology</subject><subject>Applied ecology</subject><subject>Aquifers</subject><subject>Arsenates</subject><subject>Arsenic</subject><subject>Arsenic - chemistry</subject><subject>Biological and medical sciences</subject><subject>Calcite</subject><subject>Carbonates - chemistry</subject><subject>Chemical Precipitation</subject><subject>Clay minerals</subject><subject>Ecotoxicology, biological effects of pollution</subject><subject>Fundamental and applied biological sciences. Psychology</subject><subject>General aspects</subject><subject>Groundwater flow</subject><subject>Hydrogen-Ion Concentration</subject><subject>Limestone</subject><subject>Mexico</subject><subject>Mineralogy</subject><subject>Minerals</subject><subject>Oxides</subject><subject>Retention</subject><subject>Sorption</subject><subject>Water flow</subject><subject>Water Movements</subject><subject>Water Pollutants - isolation & purification</subject><subject>Water pollution</subject><subject>Water Pollution - prevention & control</subject><subject>Water Supply</subject><issn>0090-4341</issn><issn>1432-0703</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNqFkE9rFTEUxYMo9vn0A7iRIOiq0Zu5902SZSn-g5ZudONmSDIZTZmZvCYz0Pdxuuzn6Bcz4BPEjasLh9853HMYeynhnQRQ7wtAQyQASCCAEfIR20jCRoACfMw2VQNBSPKEPSvlGkA2WtNTdiJ3SK1SuGE_znIJc_S8pLxfYpq5O3Bvs0uzXYLI0f_k9maNQ8h8qkqOdjzllvs0LzmNvBrsMWFKLo5xOXC78O9xsvuHu_mUXz7c30afnrMngx1LeHG8W_bt44ev55_FxdWnL-dnF8IimUWoVpMxzpLW0IbWojG963sFmno5uAFNO1DrvGwUNKEnqV1QhoxE0I2WA27Z29-5-5xu1lCWborFh3G0c0hr6RqNLcKu-S8oDSGYutGWvf4HvE5rnmuJTqHc1U9JV-jVEVrdFPpun-sA-dD9GboCb46ALd6OQ7azj-UvTqOqzfEX2JuM-g</recordid><startdate>20040701</startdate><enddate>20040701</enddate><creator>ROMERO, F. 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M ; ARMIENTA, M. A ; CARRILLO-CHAVEZ, A</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a349t-768499ba48806e6a399dbdd7084d1fbf396f46bc12702ed418be79491308281f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2004</creationdate><topic>Adsorption</topic><topic>Animal, plant and microbial ecology</topic><topic>Applied ecology</topic><topic>Aquifers</topic><topic>Arsenates</topic><topic>Arsenic</topic><topic>Arsenic - chemistry</topic><topic>Biological and medical sciences</topic><topic>Calcite</topic><topic>Carbonates - chemistry</topic><topic>Chemical Precipitation</topic><topic>Clay minerals</topic><topic>Ecotoxicology, biological effects of pollution</topic><topic>Fundamental and applied biological sciences. 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M</au><au>ARMIENTA, M. A</au><au>CARRILLO-CHAVEZ, A</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Arsenic sorption by carbonate-rich aquifer material, a control on arsenic mobility at Zimapán, México</atitle><jtitle>Archives of environmental contamination and toxicology</jtitle><addtitle>Arch Environ Contam Toxicol</addtitle><date>2004-07-01</date><risdate>2004</risdate><volume>47</volume><issue>1</issue><spage>1</spage><epage>13</epage><pages>1-13</pages><issn>0090-4341</issn><eissn>1432-0703</eissn><coden>AECTCV</coden><abstract>Arsenic retention by carbonate-rich aquifer material at Zimapán, México, was studied to gain insight into the processes controlling arsenic mobility in natural systems. Batch experiments showed that retention of soluble As (V) on carbonate-rich aquifer material was 35.3-90% in the pH range of 7-9 found in Zimapán natural water. Chemical and mineralogical compositions, point of zero charge (PZC), and experimental arsenic retention at various pH of three composite samples of limestone (M1, M2, M3) showed that sorption (adsorption and coprecipitation) may be one of the main processes controlling arsenic mobility in the Zimapán As-polluted aquifer. The PZC values approximately corresponded to the PZC reported for the main minerals present in each sample: hydrous ferric oxides (M1), calcite (M2), and the range from hydrous ferric oxides and calcite (M3). The chemical and mineralogical compositions of each sample explain the obtained PZC values. Experimental and modeled arsenic retention at various pH values on sample M1 corresponded to reported arsenic adsorption onto hydrous ferric oxides. Coprecipitacion of complex Ca arsenates or arsenic adsorption onto calcite or clay minerals could be the main processes of arsenic retention on samples M2 and M3. Groundwater flow through the granular, carbonate-rich, shallow aquifer may decrease the water As content as a result of these interactions. A remediation method based on the promotion of polluted water flow into the shallow aquifer could be developed from these results.</abstract><cop>Heidelberg</cop><cop>Berlin</cop><cop>New York, NY</cop><pub>Springer-Verlag</pub><pmid>15346773</pmid><doi>10.1007/s00244-004-3009-1</doi><tpages>13</tpages></addata></record> |
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| ispartof | Archives of environmental contamination and toxicology, 2004-07, Vol.47 (1), p.1-13 |
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| subjects | Adsorption Animal, plant and microbial ecology Applied ecology Aquifers Arsenates Arsenic Arsenic - chemistry Biological and medical sciences Calcite Carbonates - chemistry Chemical Precipitation Clay minerals Ecotoxicology, biological effects of pollution Fundamental and applied biological sciences. Psychology General aspects Groundwater flow Hydrogen-Ion Concentration Limestone Mexico Mineralogy Minerals Oxides Retention Sorption Water flow Water Movements Water Pollutants - isolation & purification Water pollution Water Pollution - prevention & control Water Supply |
| title | Arsenic sorption by carbonate-rich aquifer material, a control on arsenic mobility at Zimapán, México |
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