Surface plasmon assisted preparation of X1-type Y2SiO5:Eu3+-Au luminescent crystals
Rare-earth doped yttrium orthosilicate (Y2SiO5) crystals have many important applications due to their unique optical and luminescence properties. However, the indispensable high temperature treatment and long period reaction tend to greatly reduce the preparation efficiency. Here, the plasmonic pho...
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Veröffentlicht in: | Nanoscale 2023-07, Vol.15 (29), p.12333-12339 |
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creator | Xi, Lei Zhang, Chengyun Tuxun, Hairegu Zhang, Baobao Ji, Min Zhou, Xilin Liang, Wanqiu Li, Jinyu Chen, Huan Li, Jinping Fu, Zhengkun Zhang, Zhenglong Zheng, Hairong |
description | Rare-earth doped yttrium orthosilicate (Y2SiO5) crystals have many important applications due to their unique optical and luminescence properties. However, the indispensable high temperature treatment and long period reaction tend to greatly reduce the preparation efficiency. Here, the plasmonic photothermal effect of Au nanoparticles has been properly applied to realize in situ transformation from a composite structure NaYF4:Eu3+@SiO2@Au into a single monoclinic X1-type Y2SiO5:Eu3+-Au particle. It is worth mentioning that the X1-type Y2SiO5-Au particle can be well obtained within about 10 seconds when the thickness of the SiO2 shell is about 15 nm, which is unattainable with conventional approaches. Moreover, the particle turns out to possess good crystallinity, controllable morphology, and significantly improved luminescence performance. This study not only provides a brand-new path for the preparation of yttrium silicate crystals but also further extends the application of surface plasmons in the field of catalytic luminescent materials. |
doi_str_mv | 10.1039/d3nr01813j |
format | Article |
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However, the indispensable high temperature treatment and long period reaction tend to greatly reduce the preparation efficiency. Here, the plasmonic photothermal effect of Au nanoparticles has been properly applied to realize in situ transformation from a composite structure NaYF4:Eu3+@SiO2@Au into a single monoclinic X1-type Y2SiO5:Eu3+-Au particle. It is worth mentioning that the X1-type Y2SiO5-Au particle can be well obtained within about 10 seconds when the thickness of the SiO2 shell is about 15 nm, which is unattainable with conventional approaches. Moreover, the particle turns out to possess good crystallinity, controllable morphology, and significantly improved luminescence performance. This study not only provides a brand-new path for the preparation of yttrium silicate crystals but also further extends the application of surface plasmons in the field of catalytic luminescent materials.</description><identifier>ISSN: 2040-3364</identifier><identifier>EISSN: 2040-3372</identifier><identifier>DOI: 10.1039/d3nr01813j</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Composite structures ; Controllability ; Crystals ; Europium ; Gold ; High temperature ; Luminescence ; Nanoparticles ; Optical properties ; Plasmons ; Rare earth elements ; Silicon dioxide ; Yttrium</subject><ispartof>Nanoscale, 2023-07, Vol.15 (29), p.12333-12339</ispartof><rights>Copyright Royal Society of Chemistry 2023</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Xi, Lei</creatorcontrib><creatorcontrib>Zhang, Chengyun</creatorcontrib><creatorcontrib>Tuxun, Hairegu</creatorcontrib><creatorcontrib>Zhang, Baobao</creatorcontrib><creatorcontrib>Ji, Min</creatorcontrib><creatorcontrib>Zhou, Xilin</creatorcontrib><creatorcontrib>Liang, Wanqiu</creatorcontrib><creatorcontrib>Li, Jinyu</creatorcontrib><creatorcontrib>Chen, Huan</creatorcontrib><creatorcontrib>Li, Jinping</creatorcontrib><creatorcontrib>Fu, Zhengkun</creatorcontrib><creatorcontrib>Zhang, Zhenglong</creatorcontrib><creatorcontrib>Zheng, Hairong</creatorcontrib><title>Surface plasmon assisted preparation of X1-type Y2SiO5:Eu3+-Au luminescent crystals</title><title>Nanoscale</title><description>Rare-earth doped yttrium orthosilicate (Y2SiO5) crystals have many important applications due to their unique optical and luminescence properties. However, the indispensable high temperature treatment and long period reaction tend to greatly reduce the preparation efficiency. Here, the plasmonic photothermal effect of Au nanoparticles has been properly applied to realize in situ transformation from a composite structure NaYF4:Eu3+@SiO2@Au into a single monoclinic X1-type Y2SiO5:Eu3+-Au particle. It is worth mentioning that the X1-type Y2SiO5-Au particle can be well obtained within about 10 seconds when the thickness of the SiO2 shell is about 15 nm, which is unattainable with conventional approaches. Moreover, the particle turns out to possess good crystallinity, controllable morphology, and significantly improved luminescence performance. This study not only provides a brand-new path for the preparation of yttrium silicate crystals but also further extends the application of surface plasmons in the field of catalytic luminescent materials.</description><subject>Composite structures</subject><subject>Controllability</subject><subject>Crystals</subject><subject>Europium</subject><subject>Gold</subject><subject>High temperature</subject><subject>Luminescence</subject><subject>Nanoparticles</subject><subject>Optical properties</subject><subject>Plasmons</subject><subject>Rare earth elements</subject><subject>Silicon dioxide</subject><subject>Yttrium</subject><issn>2040-3364</issn><issn>2040-3372</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNpdkE1LAzEYhIMoWKsXf0HAiyCrSd5NNvFWSv2AQg9V0FNJ0zewZbu75uPQf29A8eBphuFhGIaQa87uOQPzsIM-MK457E_IRLCaVQCNOP3zqj4nFzHuGVMGFEzIep2Dtw7p2Nl4GHpqY2xjwh0dA4422NSWcPD0g1fpOCL9FOt2JR8XGe6qWaZdPrQ9Rod9oi4cY7JdvCRnvghe_eqUvD8t3uYv1XL1_DqfLauR1ypVStZaeAe4RbQNb7RWxnkB0mxds224FlpK1zDmQKLUXKD13lijrEetRA1TcvvTO4bhK2NMm0NblnSd7XHIcSM0KGG0VLKgN__Q_ZBDX9YVqi5dQpVDvgFuLl6f</recordid><startdate>20230727</startdate><enddate>20230727</enddate><creator>Xi, Lei</creator><creator>Zhang, Chengyun</creator><creator>Tuxun, Hairegu</creator><creator>Zhang, Baobao</creator><creator>Ji, Min</creator><creator>Zhou, Xilin</creator><creator>Liang, Wanqiu</creator><creator>Li, Jinyu</creator><creator>Chen, Huan</creator><creator>Li, Jinping</creator><creator>Fu, Zhengkun</creator><creator>Zhang, Zhenglong</creator><creator>Zheng, Hairong</creator><general>Royal Society of Chemistry</general><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>F28</scope><scope>FR3</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope></search><sort><creationdate>20230727</creationdate><title>Surface plasmon assisted preparation of X1-type Y2SiO5:Eu3+-Au luminescent crystals</title><author>Xi, Lei ; Zhang, Chengyun ; Tuxun, Hairegu ; Zhang, Baobao ; Ji, Min ; Zhou, Xilin ; Liang, Wanqiu ; Li, Jinyu ; Chen, Huan ; Li, Jinping ; Fu, Zhengkun ; Zhang, Zhenglong ; Zheng, Hairong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-p146t-65482fc3ebeea7178869cf2359bc7b7182855c700c35e5812eaff9a96afe86243</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Composite structures</topic><topic>Controllability</topic><topic>Crystals</topic><topic>Europium</topic><topic>Gold</topic><topic>High temperature</topic><topic>Luminescence</topic><topic>Nanoparticles</topic><topic>Optical properties</topic><topic>Plasmons</topic><topic>Rare earth elements</topic><topic>Silicon dioxide</topic><topic>Yttrium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Xi, Lei</creatorcontrib><creatorcontrib>Zhang, Chengyun</creatorcontrib><creatorcontrib>Tuxun, Hairegu</creatorcontrib><creatorcontrib>Zhang, Baobao</creatorcontrib><creatorcontrib>Ji, Min</creatorcontrib><creatorcontrib>Zhou, Xilin</creatorcontrib><creatorcontrib>Liang, Wanqiu</creatorcontrib><creatorcontrib>Li, Jinyu</creatorcontrib><creatorcontrib>Chen, Huan</creatorcontrib><creatorcontrib>Li, Jinping</creatorcontrib><creatorcontrib>Fu, Zhengkun</creatorcontrib><creatorcontrib>Zhang, Zhenglong</creatorcontrib><creatorcontrib>Zheng, Hairong</creatorcontrib><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Nanoscale</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Xi, Lei</au><au>Zhang, Chengyun</au><au>Tuxun, Hairegu</au><au>Zhang, Baobao</au><au>Ji, Min</au><au>Zhou, Xilin</au><au>Liang, Wanqiu</au><au>Li, Jinyu</au><au>Chen, Huan</au><au>Li, Jinping</au><au>Fu, Zhengkun</au><au>Zhang, Zhenglong</au><au>Zheng, Hairong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Surface plasmon assisted preparation of X1-type Y2SiO5:Eu3+-Au luminescent crystals</atitle><jtitle>Nanoscale</jtitle><date>2023-07-27</date><risdate>2023</risdate><volume>15</volume><issue>29</issue><spage>12333</spage><epage>12339</epage><pages>12333-12339</pages><issn>2040-3364</issn><eissn>2040-3372</eissn><abstract>Rare-earth doped yttrium orthosilicate (Y2SiO5) crystals have many important applications due to their unique optical and luminescence properties. However, the indispensable high temperature treatment and long period reaction tend to greatly reduce the preparation efficiency. Here, the plasmonic photothermal effect of Au nanoparticles has been properly applied to realize in situ transformation from a composite structure NaYF4:Eu3+@SiO2@Au into a single monoclinic X1-type Y2SiO5:Eu3+-Au particle. It is worth mentioning that the X1-type Y2SiO5-Au particle can be well obtained within about 10 seconds when the thickness of the SiO2 shell is about 15 nm, which is unattainable with conventional approaches. Moreover, the particle turns out to possess good crystallinity, controllable morphology, and significantly improved luminescence performance. This study not only provides a brand-new path for the preparation of yttrium silicate crystals but also further extends the application of surface plasmons in the field of catalytic luminescent materials.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/d3nr01813j</doi><tpages>7</tpages></addata></record> |
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subjects | Composite structures Controllability Crystals Europium Gold High temperature Luminescence Nanoparticles Optical properties Plasmons Rare earth elements Silicon dioxide Yttrium |
title | Surface plasmon assisted preparation of X1-type Y2SiO5:Eu3+-Au luminescent crystals |
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