N,N-dicarboxymethyl Perylene-diimide-modified CdV2O6 Nanorods for Colorimetric Sensing of H2O2 and Pyrogallol
The peroxidase-like activity of CdV 2 O 6 nanorods has been considerably improved by modification with N, N-dicarboxymethyl perylene-diimide (PDI) as a photosensitizer. The peroxidase-like behaviors are evaluated by virtue of the colorless chromogenic substrate 3,3',5,5'-tetramethylbenzidi...
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| Veröffentlicht in: | Mikrochimica acta (1966) 2023-07, Vol.190 (7), p.270-270, Article 270 |
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| container_title | Mikrochimica acta (1966) |
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| creator | Liu, Yaru Hao, Pingping Wang, Liming Li, Guijiang Fan, Gaochao Wu, Tao Zhu, Xixi Liu, Qingyun |
| description | The peroxidase-like activity of CdV
2
O
6
nanorods has been considerably improved by modification with N, N-dicarboxymethyl perylene-diimide (PDI) as a photosensitizer. The peroxidase-like behaviors are evaluated by virtue of the colorless chromogenic substrate 3,3',5,5'-tetramethylbenzidine (TMB), which is fast changed into blue oxTMB in the presence of H
2
O
2
in only 90 s. PDI-CdV
2
O
6
exhibits high stability at elevated temperatures and PDI-CdV
2
O
6
retains more than 70% of its catalytic activity over a wide range of 15 to 60 °C. The catalytic mechanism of PDI-CdV
2
O
6
is ascribed to the synergistic interaction between PDI and CdV
2
O
6
and the generation of •O
2
−
radicals. Based on the enhanced peroxidase-like activity of PDI-CdV
2
O
6
, a selective colorimetric sensor has been constructed for H
2
O
2
and pyrogallol (PG) with detection limits of 36.5 μM and 0.179 μM, respectively. The feasibility of the proposed sensing platform has been validated by detecting H
2
O
2
in milk and pyrogallol in tap water.
Graphical Abstract |
| doi_str_mv | 10.1007/s00604-023-05846-4 |
| format | Article |
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2
O
6
nanorods has been considerably improved by modification with N, N-dicarboxymethyl perylene-diimide (PDI) as a photosensitizer. The peroxidase-like behaviors are evaluated by virtue of the colorless chromogenic substrate 3,3',5,5'-tetramethylbenzidine (TMB), which is fast changed into blue oxTMB in the presence of H
2
O
2
in only 90 s. PDI-CdV
2
O
6
exhibits high stability at elevated temperatures and PDI-CdV
2
O
6
retains more than 70% of its catalytic activity over a wide range of 15 to 60 °C. The catalytic mechanism of PDI-CdV
2
O
6
is ascribed to the synergistic interaction between PDI and CdV
2
O
6
and the generation of •O
2
−
radicals. Based on the enhanced peroxidase-like activity of PDI-CdV
2
O
6
, a selective colorimetric sensor has been constructed for H
2
O
2
and pyrogallol (PG) with detection limits of 36.5 μM and 0.179 μM, respectively. The feasibility of the proposed sensing platform has been validated by detecting H
2
O
2
in milk and pyrogallol in tap water.
Graphical Abstract</description><identifier>ISSN: 0026-3672</identifier><identifier>EISSN: 1436-5073</identifier><identifier>DOI: 10.1007/s00604-023-05846-4</identifier><language>eng</language><publisher>Vienna: Springer Vienna</publisher><subject>Analytical Chemistry ; Catalytic activity ; Characterization and Evaluation of Materials ; Chemistry ; Chemistry and Materials Science ; Colorimetry ; Diimide ; Drinking water ; High temperature ; Hydrogen peroxide ; Microengineering ; Nanochemistry ; Nanorods ; Nanotechnology ; Original Paper ; Peroxidase ; Substrates</subject><ispartof>Mikrochimica acta (1966), 2023-07, Vol.190 (7), p.270-270, Article 270</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Austria, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c352t-be255faaf61716ce4ae573487c572c96cba9fa8af0dea34f0ebcfe7b765ab6b3</citedby><cites>FETCH-LOGICAL-c352t-be255faaf61716ce4ae573487c572c96cba9fa8af0dea34f0ebcfe7b765ab6b3</cites><orcidid>0000-0003-1178-6232</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00604-023-05846-4$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s00604-023-05846-4$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Liu, Yaru</creatorcontrib><creatorcontrib>Hao, Pingping</creatorcontrib><creatorcontrib>Wang, Liming</creatorcontrib><creatorcontrib>Li, Guijiang</creatorcontrib><creatorcontrib>Fan, Gaochao</creatorcontrib><creatorcontrib>Wu, Tao</creatorcontrib><creatorcontrib>Zhu, Xixi</creatorcontrib><creatorcontrib>Liu, Qingyun</creatorcontrib><title>N,N-dicarboxymethyl Perylene-diimide-modified CdV2O6 Nanorods for Colorimetric Sensing of H2O2 and Pyrogallol</title><title>Mikrochimica acta (1966)</title><addtitle>Microchim Acta</addtitle><description>The peroxidase-like activity of CdV
2
O
6
nanorods has been considerably improved by modification with N, N-dicarboxymethyl perylene-diimide (PDI) as a photosensitizer. The peroxidase-like behaviors are evaluated by virtue of the colorless chromogenic substrate 3,3',5,5'-tetramethylbenzidine (TMB), which is fast changed into blue oxTMB in the presence of H
2
O
2
in only 90 s. PDI-CdV
2
O
6
exhibits high stability at elevated temperatures and PDI-CdV
2
O
6
retains more than 70% of its catalytic activity over a wide range of 15 to 60 °C. The catalytic mechanism of PDI-CdV
2
O
6
is ascribed to the synergistic interaction between PDI and CdV
2
O
6
and the generation of •O
2
−
radicals. Based on the enhanced peroxidase-like activity of PDI-CdV
2
O
6
, a selective colorimetric sensor has been constructed for H
2
O
2
and pyrogallol (PG) with detection limits of 36.5 μM and 0.179 μM, respectively. The feasibility of the proposed sensing platform has been validated by detecting H
2
O
2
in milk and pyrogallol in tap water.
Graphical Abstract</description><subject>Analytical Chemistry</subject><subject>Catalytic activity</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Colorimetry</subject><subject>Diimide</subject><subject>Drinking water</subject><subject>High temperature</subject><subject>Hydrogen peroxide</subject><subject>Microengineering</subject><subject>Nanochemistry</subject><subject>Nanorods</subject><subject>Nanotechnology</subject><subject>Original Paper</subject><subject>Peroxidase</subject><subject>Substrates</subject><issn>0026-3672</issn><issn>1436-5073</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kcFqGzEQhkVJoI6TF-hJ0EsPVaKVtNL6GExbB4wdiMlVaLUjV0a7ciQbsm9ftRso5JDTHOb7fmb4EfpS0duKUnWXKZVUEMo4oXUjJBGf0KwSXJKaKn6BZpQySbhU7DO6yvlAaaUkEzPUb75vSOetSW18HXs4_R4DfoQ0BhigLHzvOyB97Lzz0OFl98y2Em_MEFPsMnYx4WUMMfmiJm_xEwzZD3scHV6xLcNm6PDjmOLehBDDNbp0JmS4eZtztPv5Y7dckfX218Pyfk0sr9mJtMDq2hnjZKUqaUEYqBUXjbK1YnYhbWsWzjTG0Q4MF45Cax2oVsnatLLlc_Rtij2m-HKGfNK9zxZCMAPEc9asYQ2XlRBNQb--Qw_xnIZy3EQtFpyzQrGJsinmnMDpY_nYpFFXVP8tQE8F6FKA_leAFkXik5QLPOwh_Y_-wPoDphOJeQ</recordid><startdate>20230701</startdate><enddate>20230701</enddate><creator>Liu, Yaru</creator><creator>Hao, Pingping</creator><creator>Wang, Liming</creator><creator>Li, Guijiang</creator><creator>Fan, Gaochao</creator><creator>Wu, Tao</creator><creator>Zhu, Xixi</creator><creator>Liu, Qingyun</creator><general>Springer Vienna</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>K9.</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-1178-6232</orcidid></search><sort><creationdate>20230701</creationdate><title>N,N-dicarboxymethyl Perylene-diimide-modified CdV2O6 Nanorods for Colorimetric Sensing of H2O2 and Pyrogallol</title><author>Liu, Yaru ; Hao, Pingping ; Wang, Liming ; Li, Guijiang ; Fan, Gaochao ; Wu, Tao ; Zhu, Xixi ; Liu, Qingyun</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c352t-be255faaf61716ce4ae573487c572c96cba9fa8af0dea34f0ebcfe7b765ab6b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Analytical Chemistry</topic><topic>Catalytic activity</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Colorimetry</topic><topic>Diimide</topic><topic>Drinking water</topic><topic>High temperature</topic><topic>Hydrogen peroxide</topic><topic>Microengineering</topic><topic>Nanochemistry</topic><topic>Nanorods</topic><topic>Nanotechnology</topic><topic>Original Paper</topic><topic>Peroxidase</topic><topic>Substrates</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Liu, Yaru</creatorcontrib><creatorcontrib>Hao, Pingping</creatorcontrib><creatorcontrib>Wang, Liming</creatorcontrib><creatorcontrib>Li, Guijiang</creatorcontrib><creatorcontrib>Fan, Gaochao</creatorcontrib><creatorcontrib>Wu, Tao</creatorcontrib><creatorcontrib>Zhu, Xixi</creatorcontrib><creatorcontrib>Liu, Qingyun</creatorcontrib><collection>CrossRef</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>MEDLINE - Academic</collection><jtitle>Mikrochimica acta (1966)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, Yaru</au><au>Hao, Pingping</au><au>Wang, Liming</au><au>Li, Guijiang</au><au>Fan, Gaochao</au><au>Wu, Tao</au><au>Zhu, Xixi</au><au>Liu, Qingyun</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>N,N-dicarboxymethyl Perylene-diimide-modified CdV2O6 Nanorods for Colorimetric Sensing of H2O2 and Pyrogallol</atitle><jtitle>Mikrochimica acta (1966)</jtitle><stitle>Microchim Acta</stitle><date>2023-07-01</date><risdate>2023</risdate><volume>190</volume><issue>7</issue><spage>270</spage><epage>270</epage><pages>270-270</pages><artnum>270</artnum><issn>0026-3672</issn><eissn>1436-5073</eissn><abstract>The peroxidase-like activity of CdV
2
O
6
nanorods has been considerably improved by modification with N, N-dicarboxymethyl perylene-diimide (PDI) as a photosensitizer. The peroxidase-like behaviors are evaluated by virtue of the colorless chromogenic substrate 3,3',5,5'-tetramethylbenzidine (TMB), which is fast changed into blue oxTMB in the presence of H
2
O
2
in only 90 s. PDI-CdV
2
O
6
exhibits high stability at elevated temperatures and PDI-CdV
2
O
6
retains more than 70% of its catalytic activity over a wide range of 15 to 60 °C. The catalytic mechanism of PDI-CdV
2
O
6
is ascribed to the synergistic interaction between PDI and CdV
2
O
6
and the generation of •O
2
−
radicals. Based on the enhanced peroxidase-like activity of PDI-CdV
2
O
6
, a selective colorimetric sensor has been constructed for H
2
O
2
and pyrogallol (PG) with detection limits of 36.5 μM and 0.179 μM, respectively. The feasibility of the proposed sensing platform has been validated by detecting H
2
O
2
in milk and pyrogallol in tap water.
Graphical Abstract</abstract><cop>Vienna</cop><pub>Springer Vienna</pub><doi>10.1007/s00604-023-05846-4</doi><tpages>1</tpages><orcidid>https://orcid.org/0000-0003-1178-6232</orcidid></addata></record> |
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| subjects | Analytical Chemistry Catalytic activity Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Colorimetry Diimide Drinking water High temperature Hydrogen peroxide Microengineering Nanochemistry Nanorods Nanotechnology Original Paper Peroxidase Substrates |
| title | N,N-dicarboxymethyl Perylene-diimide-modified CdV2O6 Nanorods for Colorimetric Sensing of H2O2 and Pyrogallol |
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