A wide-range ratiometric sensor mediating fluorescence and scattering based on carbon dots/metal–organic framework composites for the detection of bisulfite/sulfite in sugar
Bisulfite (HSO 3 − ) and sulfite (SO 3 2− ) are commonly employed in food preservatives and are also significant environmental pollutants. Thus, developing an effective method for detecting HSO 3 − /SO 3 2− is crucial for food safety and environment monitoring. In this work, based on carbon dots (CD...
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| Veröffentlicht in: | Analytical and bioanalytical chemistry 2023-08, Vol.415 (19), p.4639-4647 |
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| creator | Wang, Bing Jie Xu, Zi Yi Sun, Zhe Li, Zi Qing Luo, Yuan Hao Luo, Hong Qun Li, Nian Bing |
| description | Bisulfite (HSO
3
−
) and sulfite (SO
3
2−
) are commonly employed in food preservatives and are also significant environmental pollutants. Thus, developing an effective method for detecting HSO
3
−
/SO
3
2−
is crucial for food safety and environment monitoring. In this work, based on carbon dots (CDs) and zeolitic imidazolate framework‐90 (ZIF‐90), a composite probe (named CDs@ZIF-90) is constructed. The fluorescence signal and the second-order scattering signal of CDs@ZIF-90 are employed to ratiometricly detect HSO
3
−
/SO
3
2−
. This proposed strategy exhibits a broad linear range for HSO
3
−
/SO
3
2−
determination (10 µM to 8.5 mM) with a limit of detection of 2.74 μM. This strategy is successfully applied for evaluating HSO
3
−
/SO
3
2−
in sugar with satisfactory recoveries. Therefore, this work has uniquely combined the fluorescence and second-order scattering signals to establish a novel sensing system with a wide linear range, which is applicable for ratiometric sensing of HSO
3
−
/SO
3
2−
in actual samples.
Graphical Abstract |
| doi_str_mv | 10.1007/s00216-023-04763-y |
| format | Article |
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3
−
) and sulfite (SO
3
2−
) are commonly employed in food preservatives and are also significant environmental pollutants. Thus, developing an effective method for detecting HSO
3
−
/SO
3
2−
is crucial for food safety and environment monitoring. In this work, based on carbon dots (CDs) and zeolitic imidazolate framework‐90 (ZIF‐90), a composite probe (named CDs@ZIF-90) is constructed. The fluorescence signal and the second-order scattering signal of CDs@ZIF-90 are employed to ratiometricly detect HSO
3
−
/SO
3
2−
. This proposed strategy exhibits a broad linear range for HSO
3
−
/SO
3
2−
determination (10 µM to 8.5 mM) with a limit of detection of 2.74 μM. This strategy is successfully applied for evaluating HSO
3
−
/SO
3
2−
in sugar with satisfactory recoveries. Therefore, this work has uniquely combined the fluorescence and second-order scattering signals to establish a novel sensing system with a wide linear range, which is applicable for ratiometric sensing of HSO
3
−
/SO
3
2−
in actual samples.
Graphical Abstract</description><identifier>ISSN: 1618-2642</identifier><identifier>EISSN: 1618-2650</identifier><identifier>DOI: 10.1007/s00216-023-04763-y</identifier><identifier>PMID: 37268746</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Analysis ; Analytical Chemistry ; Biochemistry ; Bisulfite ; Carbon ; Carbon dots ; Characterization and Evaluation of Materials ; Chemistry ; Chemistry and Materials Science ; Composite materials ; Decomposition ; Fluorescence ; Food ; Food safety ; Food Science ; Laboratory Medicine ; Metal-organic frameworks ; Methods ; Monitoring/Environmental Analysis ; Organometallic compounds ; Paper in Forefront ; Preservatives ; Quantum dots ; Scattering ; Sensors ; Sugar ; Sulfite ; Sulfites ; Zeolites</subject><ispartof>Analytical and bioanalytical chemistry, 2023-08, Vol.415 (19), p.4639-4647</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>2023. Springer-Verlag GmbH Germany, part of Springer Nature.</rights><rights>COPYRIGHT 2023 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c414t-f2cf0e5488b6fb6d1280f5e437f618f721b7eebcdc9d3259ffe3a63ebabb808d3</citedby><cites>FETCH-LOGICAL-c414t-f2cf0e5488b6fb6d1280f5e437f618f721b7eebcdc9d3259ffe3a63ebabb808d3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00216-023-04763-y$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s00216-023-04763-y$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/37268746$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Wang, Bing Jie</creatorcontrib><creatorcontrib>Xu, Zi Yi</creatorcontrib><creatorcontrib>Sun, Zhe</creatorcontrib><creatorcontrib>Li, Zi Qing</creatorcontrib><creatorcontrib>Luo, Yuan Hao</creatorcontrib><creatorcontrib>Luo, Hong Qun</creatorcontrib><creatorcontrib>Li, Nian Bing</creatorcontrib><title>A wide-range ratiometric sensor mediating fluorescence and scattering based on carbon dots/metal–organic framework composites for the detection of bisulfite/sulfite in sugar</title><title>Analytical and bioanalytical chemistry</title><addtitle>Anal Bioanal Chem</addtitle><addtitle>Anal Bioanal Chem</addtitle><description>Bisulfite (HSO
3
−
) and sulfite (SO
3
2−
) are commonly employed in food preservatives and are also significant environmental pollutants. Thus, developing an effective method for detecting HSO
3
−
/SO
3
2−
is crucial for food safety and environment monitoring. In this work, based on carbon dots (CDs) and zeolitic imidazolate framework‐90 (ZIF‐90), a composite probe (named CDs@ZIF-90) is constructed. The fluorescence signal and the second-order scattering signal of CDs@ZIF-90 are employed to ratiometricly detect HSO
3
−
/SO
3
2−
. This proposed strategy exhibits a broad linear range for HSO
3
−
/SO
3
2−
determination (10 µM to 8.5 mM) with a limit of detection of 2.74 μM. This strategy is successfully applied for evaluating HSO
3
−
/SO
3
2−
in sugar with satisfactory recoveries. Therefore, this work has uniquely combined the fluorescence and second-order scattering signals to establish a novel sensing system with a wide linear range, which is applicable for ratiometric sensing of HSO
3
−
/SO
3
2−
in actual samples.
Graphical Abstract</description><subject>Analysis</subject><subject>Analytical Chemistry</subject><subject>Biochemistry</subject><subject>Bisulfite</subject><subject>Carbon</subject><subject>Carbon dots</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Composite materials</subject><subject>Decomposition</subject><subject>Fluorescence</subject><subject>Food</subject><subject>Food safety</subject><subject>Food Science</subject><subject>Laboratory Medicine</subject><subject>Metal-organic frameworks</subject><subject>Methods</subject><subject>Monitoring/Environmental Analysis</subject><subject>Organometallic compounds</subject><subject>Paper in Forefront</subject><subject>Preservatives</subject><subject>Quantum dots</subject><subject>Scattering</subject><subject>Sensors</subject><subject>Sugar</subject><subject>Sulfite</subject><subject>Sulfites</subject><subject>Zeolites</subject><issn>1618-2642</issn><issn>1618-2650</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9UUtuFDEQbSEQCYELsECW2LDpjD_dtmc5ivhJkdjAuuVPuXHotgfbrWh23IGDcKecJB56CBIL5EVZVe-9-rymeUnwJcFYbDLGlPAWU9biTnDWHh4154QT2VLe48cP_46eNc9yvsGY9JLwp80ZE5RL0fHz5tcO3XoLbVJhBJRU8XGGkrxBGUKOCc1gfc2GEblpiQmygWAAqWBRNqoUSMeaVhksigEZlXQNNpa8qUJquvvxM6ZRharokprhNqZvyMR5H7MvkJGrPcpXQBYKmNo9oOiQ9nmZXK1vThH5gPIyqvS8eeLUlOHFKV40X969_Xz1ob3-9P7j1e66NR3pSuuocRj6TkrNneaWUIldDx0Trt7ECUq0ANDGmq1ltN86B0xxBlppLbG07KJ5s-ruU_y-QC7D7Ovq06QCxCUPVFLKxLYet0Jf_wO9iUsKdbqKYrLrGee8oi5X1KgmGHxwsSRl6rMwexMDOF_zO9GLXrJe0EqgK8GkmHMCN-yTn1U6DAQPR_-H1f-h-j_89n84VNKr0yyLrs49UP4YXgFsBeT90ThIf4f9j-w9iGnBow</recordid><startdate>20230801</startdate><enddate>20230801</enddate><creator>Wang, 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wide-range ratiometric sensor mediating fluorescence and scattering based on carbon dots/metal–organic framework composites for the detection of bisulfite/sulfite in sugar</title><author>Wang, Bing Jie ; Xu, Zi Yi ; Sun, Zhe ; Li, Zi Qing ; Luo, Yuan Hao ; Luo, Hong Qun ; Li, Nian Bing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c414t-f2cf0e5488b6fb6d1280f5e437f618f721b7eebcdc9d3259ffe3a63ebabb808d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Analysis</topic><topic>Analytical Chemistry</topic><topic>Biochemistry</topic><topic>Bisulfite</topic><topic>Carbon</topic><topic>Carbon dots</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Composite materials</topic><topic>Decomposition</topic><topic>Fluorescence</topic><topic>Food</topic><topic>Food safety</topic><topic>Food Science</topic><topic>Laboratory Medicine</topic><topic>Metal-organic frameworks</topic><topic>Methods</topic><topic>Monitoring/Environmental Analysis</topic><topic>Organometallic compounds</topic><topic>Paper in Forefront</topic><topic>Preservatives</topic><topic>Quantum dots</topic><topic>Scattering</topic><topic>Sensors</topic><topic>Sugar</topic><topic>Sulfite</topic><topic>Sulfites</topic><topic>Zeolites</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Bing Jie</creatorcontrib><creatorcontrib>Xu, Zi Yi</creatorcontrib><creatorcontrib>Sun, Zhe</creatorcontrib><creatorcontrib>Li, Zi Qing</creatorcontrib><creatorcontrib>Luo, Yuan Hao</creatorcontrib><creatorcontrib>Luo, Hong Qun</creatorcontrib><creatorcontrib>Li, Nian Bing</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Aluminium Industry Abstracts</collection><collection>Biotechnology 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chemistry</jtitle><stitle>Anal Bioanal Chem</stitle><addtitle>Anal Bioanal Chem</addtitle><date>2023-08-01</date><risdate>2023</risdate><volume>415</volume><issue>19</issue><spage>4639</spage><epage>4647</epage><pages>4639-4647</pages><issn>1618-2642</issn><eissn>1618-2650</eissn><abstract>Bisulfite (HSO
3
−
) and sulfite (SO
3
2−
) are commonly employed in food preservatives and are also significant environmental pollutants. Thus, developing an effective method for detecting HSO
3
−
/SO
3
2−
is crucial for food safety and environment monitoring. In this work, based on carbon dots (CDs) and zeolitic imidazolate framework‐90 (ZIF‐90), a composite probe (named CDs@ZIF-90) is constructed. The fluorescence signal and the second-order scattering signal of CDs@ZIF-90 are employed to ratiometricly detect HSO
3
−
/SO
3
2−
. This proposed strategy exhibits a broad linear range for HSO
3
−
/SO
3
2−
determination (10 µM to 8.5 mM) with a limit of detection of 2.74 μM. This strategy is successfully applied for evaluating HSO
3
−
/SO
3
2−
in sugar with satisfactory recoveries. Therefore, this work has uniquely combined the fluorescence and second-order scattering signals to establish a novel sensing system with a wide linear range, which is applicable for ratiometric sensing of HSO
3
−
/SO
3
2−
in actual samples.
Graphical Abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>37268746</pmid><doi>10.1007/s00216-023-04763-y</doi><tpages>9</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1618-2642 |
| ispartof | Analytical and bioanalytical chemistry, 2023-08, Vol.415 (19), p.4639-4647 |
| issn | 1618-2642 1618-2650 |
| language | eng |
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| source | SpringerLink Journals - AutoHoldings |
| subjects | Analysis Analytical Chemistry Biochemistry Bisulfite Carbon Carbon dots Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Composite materials Decomposition Fluorescence Food Food safety Food Science Laboratory Medicine Metal-organic frameworks Methods Monitoring/Environmental Analysis Organometallic compounds Paper in Forefront Preservatives Quantum dots Scattering Sensors Sugar Sulfite Sulfites Zeolites |
| title | A wide-range ratiometric sensor mediating fluorescence and scattering based on carbon dots/metal–organic framework composites for the detection of bisulfite/sulfite in sugar |
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