Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region

We investigate the effects of combining growth interruption (GI) and InGaAs strain reducing matrix at low In content on the optical properties of Stanski–Krastanow InAs QDs grown by molecular beam epitaxy. Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three seri...

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Veröffentlicht in:Journal of crystal growth 2004-02, Vol.261 (4), p.458-465
Hauptverfasser: Convertino, Annalisa, Cerri, Luciana, Leo, Gabriella, Viticoli, Sesto
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creator Convertino, Annalisa
Cerri, Luciana
Leo, Gabriella
Viticoli, Sesto
description We investigate the effects of combining growth interruption (GI) and InGaAs strain reducing matrix at low In content on the optical properties of Stanski–Krastanow InAs QDs grown by molecular beam epitaxy. Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three series of uncapped and capped samples grown in different conditions: (a) low arsenic pressure (As BEP=4×10 −6 Torr) and relatively low InAs growth temperature ( T InAs=530°C); (b) low As BEP (4×10 −6 Torr) and high T InAs (545°C); (c) high As BEP (7×10 −6 Torr) and low T InAs (530°C). Our studies clearly show that in the three growth regimes, GI causes very different effects on the morphological and optical properties of InAs QDs embedded in InGaAs matrix (In=0.12), ruled by the In diffusion and desorption processes. In particular, for samples grown at 530°C and As BeP=4×10 −6 Torr (series a), the arrangment of GI and QD embedding in an InGaAs matrix at low In content is an effcient method to tune the InAs QD PL emission and to improve their optical quality. In this case, indeed, the increase of the interruption time up to 300 s introduces a strong redshift (∼110 meV) in the PL peak with a decreasing of the linewidths from 52 to 26 meV, obtaining room temperature emission characterized by a narrow peak close to 1.3 μm.
doi_str_mv 10.1016/j.jcrysgro.2003.09.034
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Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three series of uncapped and capped samples grown in different conditions: (a) low arsenic pressure (As BEP=4×10 −6 Torr) and relatively low InAs growth temperature ( T InAs=530°C); (b) low As BEP (4×10 −6 Torr) and high T InAs (545°C); (c) high As BEP (7×10 −6 Torr) and low T InAs (530°C). Our studies clearly show that in the three growth regimes, GI causes very different effects on the morphological and optical properties of InAs QDs embedded in InGaAs matrix (In=0.12), ruled by the In diffusion and desorption processes. In particular, for samples grown at 530°C and As BeP=4×10 −6 Torr (series a), the arrangment of GI and QD embedding in an InGaAs matrix at low In content is an effcient method to tune the InAs QD PL emission and to improve their optical quality. 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subjects A1. Surface processes
A3. Molecular beam epitaxy
B1. Nanomaterials
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Cross-disciplinary physics: materials science
rheology
Exact sciences and technology
Iii-v semiconductors
Materials science
Nanoscale materials and structures: fabrication and characterization
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Photoluminescence
Physics
Quantum dots
title Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region
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