Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region
We investigate the effects of combining growth interruption (GI) and InGaAs strain reducing matrix at low In content on the optical properties of Stanski–Krastanow InAs QDs grown by molecular beam epitaxy. Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three seri...
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creator | Convertino, Annalisa Cerri, Luciana Leo, Gabriella Viticoli, Sesto |
description | We investigate the effects of combining growth interruption (GI) and InGaAs strain reducing matrix at low In content on the optical properties of Stanski–Krastanow InAs QDs grown by molecular beam epitaxy. Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three series of uncapped and capped samples grown in different conditions: (a) low arsenic pressure (As BEP=4×10
−6
Torr) and relatively low InAs growth temperature (
T
InAs=530°C); (b) low As BEP (4×10
−6
Torr) and high
T
InAs (545°C); (c) high As BEP (7×10
−6
Torr) and low
T
InAs (530°C). Our studies clearly show that in the three growth regimes, GI causes very different effects on the morphological and optical properties of InAs QDs embedded in InGaAs matrix (In=0.12), ruled by the In diffusion and desorption processes. In particular, for samples grown at 530°C and As BeP=4×10
−6
Torr (series a), the arrangment of GI and QD embedding in an InGaAs matrix at low In content is an effcient method to tune the InAs QD PL emission and to improve their optical quality. In this case, indeed, the increase of the interruption time up to 300
s introduces a strong redshift (∼110
meV) in the PL peak with a decreasing of the linewidths from 52 to 26
meV, obtaining room temperature emission characterized by a narrow peak close to 1.3
μm. |
doi_str_mv | 10.1016/j.jcrysgro.2003.09.034 |
format | Article |
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−6
Torr) and relatively low InAs growth temperature (
T
InAs=530°C); (b) low As BEP (4×10
−6
Torr) and high
T
InAs (545°C); (c) high As BEP (7×10
−6
Torr) and low
T
InAs (530°C). Our studies clearly show that in the three growth regimes, GI causes very different effects on the morphological and optical properties of InAs QDs embedded in InGaAs matrix (In=0.12), ruled by the In diffusion and desorption processes. In particular, for samples grown at 530°C and As BeP=4×10
−6
Torr (series a), the arrangment of GI and QD embedding in an InGaAs matrix at low In content is an effcient method to tune the InAs QD PL emission and to improve their optical quality. In this case, indeed, the increase of the interruption time up to 300
s introduces a strong redshift (∼110
meV) in the PL peak with a decreasing of the linewidths from 52 to 26
meV, obtaining room temperature emission characterized by a narrow peak close to 1.3
μm.</description><identifier>ISSN: 0022-0248</identifier><identifier>EISSN: 1873-5002</identifier><identifier>DOI: 10.1016/j.jcrysgro.2003.09.034</identifier><identifier>CODEN: JCRGAE</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>A1. Surface processes ; A3. Molecular beam epitaxy ; B1. Nanomaterials ; Condensed matter: electronic structure, electrical, magnetic, and optical properties ; Cross-disciplinary physics: materials science; rheology ; Exact sciences and technology ; Iii-v semiconductors ; Materials science ; Nanoscale materials and structures: fabrication and characterization ; Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation ; Photoluminescence ; Physics ; Quantum dots</subject><ispartof>Journal of crystal growth, 2004-02, Vol.261 (4), p.458-465</ispartof><rights>2003 Elsevier B.V.</rights><rights>2004 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c437t-9a1a0c02d0259f93903990bbc445eff643bd7b3de562e7994c5e2324d22d97573</citedby><cites>FETCH-LOGICAL-c437t-9a1a0c02d0259f93903990bbc445eff643bd7b3de562e7994c5e2324d22d97573</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0022024803018189$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3536,27903,27904,65309</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=15494126$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Convertino, Annalisa</creatorcontrib><creatorcontrib>Cerri, Luciana</creatorcontrib><creatorcontrib>Leo, Gabriella</creatorcontrib><creatorcontrib>Viticoli, Sesto</creatorcontrib><title>Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region</title><title>Journal of crystal growth</title><description>We investigate the effects of combining growth interruption (GI) and InGaAs strain reducing matrix at low In content on the optical properties of Stanski–Krastanow InAs QDs grown by molecular beam epitaxy. Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three series of uncapped and capped samples grown in different conditions: (a) low arsenic pressure (As BEP=4×10
−6
Torr) and relatively low InAs growth temperature (
T
InAs=530°C); (b) low As BEP (4×10
−6
Torr) and high
T
InAs (545°C); (c) high As BEP (7×10
−6
Torr) and low
T
InAs (530°C). Our studies clearly show that in the three growth regimes, GI causes very different effects on the morphological and optical properties of InAs QDs embedded in InGaAs matrix (In=0.12), ruled by the In diffusion and desorption processes. In particular, for samples grown at 530°C and As BeP=4×10
−6
Torr (series a), the arrangment of GI and QD embedding in an InGaAs matrix at low In content is an effcient method to tune the InAs QD PL emission and to improve their optical quality. In this case, indeed, the increase of the interruption time up to 300
s introduces a strong redshift (∼110
meV) in the PL peak with a decreasing of the linewidths from 52 to 26
meV, obtaining room temperature emission characterized by a narrow peak close to 1.3
μm.</description><subject>A1. Surface processes</subject><subject>A3. Molecular beam epitaxy</subject><subject>B1. Nanomaterials</subject><subject>Condensed matter: electronic structure, electrical, magnetic, and optical properties</subject><subject>Cross-disciplinary physics: materials science; rheology</subject><subject>Exact sciences and technology</subject><subject>Iii-v semiconductors</subject><subject>Materials science</subject><subject>Nanoscale materials and structures: fabrication and characterization</subject><subject>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</subject><subject>Photoluminescence</subject><subject>Physics</subject><subject>Quantum dots</subject><issn>0022-0248</issn><issn>1873-5002</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><recordid>eNqFkE9v1DAQxS0EEkvhKyBf4JZ0_CfJ-kZVwVKpEhc4W4492XqVtbe209JvX0dbxLEXW5r3fvM0j5DPDFoGrL88tAebnvI-xZYDiBZUC0K-IRu2HUTTAfC3ZFNf3gCX2_fkQ84HgEoy2JBll-JjuaM-FExpORUfAy2RliUgLXdI8ehzXodxojfhKtP7xYSyHKmLJVd1ROfQVb6qO1P1oynJ_10HKz7HsKeP5gFnDPuak3Bfl30k7yYzZ_z08l-QPz--_77-2dz-2t1cX902VoqhNMowAxa4A96pSQkFQikYRytlh9PUSzG6YRQOu57joJS0HXLBpePcqaEbxAX5et57SvF-wVx0vcbiPJuAccmab5lisuursT8bbYo5J5z0KfmjSU-agV5b1gf9r2W9tqxB6dpyBb-8JJhszTwlE6zP_-lOKsn4GvDt7MN67oPHpLP1GCw6n9AW7aJ_LeoZWWyX0Q</recordid><startdate>20040201</startdate><enddate>20040201</enddate><creator>Convertino, Annalisa</creator><creator>Cerri, Luciana</creator><creator>Leo, Gabriella</creator><creator>Viticoli, Sesto</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20040201</creationdate><title>Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region</title><author>Convertino, Annalisa ; Cerri, Luciana ; Leo, Gabriella ; Viticoli, Sesto</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c437t-9a1a0c02d0259f93903990bbc445eff643bd7b3de562e7994c5e2324d22d97573</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2004</creationdate><topic>A1. Surface processes</topic><topic>A3. Molecular beam epitaxy</topic><topic>B1. Nanomaterials</topic><topic>Condensed matter: electronic structure, electrical, magnetic, and optical properties</topic><topic>Cross-disciplinary physics: materials science; rheology</topic><topic>Exact sciences and technology</topic><topic>Iii-v semiconductors</topic><topic>Materials science</topic><topic>Nanoscale materials and structures: fabrication and characterization</topic><topic>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</topic><topic>Photoluminescence</topic><topic>Physics</topic><topic>Quantum dots</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Convertino, Annalisa</creatorcontrib><creatorcontrib>Cerri, Luciana</creatorcontrib><creatorcontrib>Leo, Gabriella</creatorcontrib><creatorcontrib>Viticoli, Sesto</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Journal of crystal growth</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Convertino, Annalisa</au><au>Cerri, Luciana</au><au>Leo, Gabriella</au><au>Viticoli, Sesto</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region</atitle><jtitle>Journal of crystal growth</jtitle><date>2004-02-01</date><risdate>2004</risdate><volume>261</volume><issue>4</issue><spage>458</spage><epage>465</epage><pages>458-465</pages><issn>0022-0248</issn><eissn>1873-5002</eissn><coden>JCRGAE</coden><abstract>We investigate the effects of combining growth interruption (GI) and InGaAs strain reducing matrix at low In content on the optical properties of Stanski–Krastanow InAs QDs grown by molecular beam epitaxy. Atomic force microscopy and Photoluminescence (PL) measurements were carried out on three series of uncapped and capped samples grown in different conditions: (a) low arsenic pressure (As BEP=4×10
−6
Torr) and relatively low InAs growth temperature (
T
InAs=530°C); (b) low As BEP (4×10
−6
Torr) and high
T
InAs (545°C); (c) high As BEP (7×10
−6
Torr) and low
T
InAs (530°C). Our studies clearly show that in the three growth regimes, GI causes very different effects on the morphological and optical properties of InAs QDs embedded in InGaAs matrix (In=0.12), ruled by the In diffusion and desorption processes. In particular, for samples grown at 530°C and As BeP=4×10
−6
Torr (series a), the arrangment of GI and QD embedding in an InGaAs matrix at low In content is an effcient method to tune the InAs QD PL emission and to improve their optical quality. In this case, indeed, the increase of the interruption time up to 300
s introduces a strong redshift (∼110
meV) in the PL peak with a decreasing of the linewidths from 52 to 26
meV, obtaining room temperature emission characterized by a narrow peak close to 1.3
μm.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.jcrysgro.2003.09.034</doi><tpages>8</tpages></addata></record> |
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subjects | A1. Surface processes A3. Molecular beam epitaxy B1. Nanomaterials Condensed matter: electronic structure, electrical, magnetic, and optical properties Cross-disciplinary physics: materials science rheology Exact sciences and technology Iii-v semiconductors Materials science Nanoscale materials and structures: fabrication and characterization Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation Photoluminescence Physics Quantum dots |
title | Growth interruption to tune the emission of InAs quantum dots embedded in InGaAs matrix in the long wavelength region |
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