Extinction by plasmonic nanoparticles in dispersive and dissipative media

Extinction of small metallic spheres has been well understood through the classical Mie theory when the host medium is dispersive and transparent. However, the role of host dissipation on the particulate extinction remains a competition between the enhancing and reducing effects on the localized sur...

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Veröffentlicht in:Optics letters 2022-11, Vol.47 (21), p.5577-5580
Hauptverfasser: Zhang, Shangyu, Dong, Jian, Zhang, Wenjie, Luo, Minggang, Liu, Linhua
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creator Zhang, Shangyu
Dong, Jian
Zhang, Wenjie
Luo, Minggang
Liu, Linhua
description Extinction of small metallic spheres has been well understood through the classical Mie theory when the host medium is dispersive and transparent. However, the role of host dissipation on the particulate extinction remains a competition between the enhancing and reducing effects on the localized surface plasmonic resonance (LSPR). Here, using a generalized Mie theory, we elaborate on the specific influence mechanisms of host dissipation on the extinction efficiency factors of a plasmonic nanosphere. To this end, we isolate the dissipative effects by comparing the dispersive and dissipative host with its dissipationless counterpart. As a result, we identify the damping effects of host dissipation on the LSPR including the resonance widening and amplitude reducing. The resonance positions are shifted by host dissipation, which cannot be predicted by the classical Fröhlich condition. Finally, we demonstrate that a wideband extinction enhancement due to host dissipation can be realized away from the positions of the LSPR.
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subjects Damping
Dispersion
Dissipation
Extinction
Mie scattering
Nanoparticles
Nanospheres
Plasmonics
Surface plasmon resonance
title Extinction by plasmonic nanoparticles in dispersive and dissipative media
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