Enhanced fluorescence transduction properties of metallic nanocavity arrays
We studied fluorescence enhancement of molecular species bound within metallic nanocavities. These nanostructures possess a number of desirable properties for real-time microarrays, such as localization of excitation light within the nanocavities, strong isolation from fluorescence produced by unbou...
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Veröffentlicht in: | IEEE journal of selected topics in quantum electronics 2005-07, Vol.11 (4), p.778-784 |
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creator | Yongdong Liu Mahdavi, F. Blair, S. |
description | We studied fluorescence enhancement of molecular species bound within metallic nanocavities. These nanostructures possess a number of desirable properties for real-time microarrays, such as localization of excitation light within the nanocavities, strong isolation from fluorescence produced by unbound species, and an apparent increase in fluorescence yield for bound species. Experimental measurements show nearly a factor of two increase in excitation intensity within the nanocavities, and factor of six increase in yield. A simple electromagnetic model of a dipole within a nanocavity shows an increase in radiative output consistent with our yield estimates, and also verifies the strong fluorescence isolation from species lying outside the nanocavity. |
doi_str_mv | 10.1109/JSTQE.2005.857688 |
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These nanostructures possess a number of desirable properties for real-time microarrays, such as localization of excitation light within the nanocavities, strong isolation from fluorescence produced by unbound species, and an apparent increase in fluorescence yield for bound species. Experimental measurements show nearly a factor of two increase in excitation intensity within the nanocavities, and factor of six increase in yield. A simple electromagnetic model of a dipole within a nanocavity shows an increase in radiative output consistent with our yield estimates, and also verifies the strong fluorescence isolation from species lying outside the nanocavity.</description><identifier>ISSN: 1077-260X</identifier><identifier>EISSN: 1558-4542</identifier><identifier>DOI: 10.1109/JSTQE.2005.857688</identifier><identifier>CODEN: IJSQEN</identifier><language>eng</language><publisher>New York: IEEE</publisher><subject>Arrays ; Biotechnology ; Cities and towns ; Excitation ; Fluorescence ; Kinetic theory ; Mathematical models ; molecular detection ; Nanocomposites ; Nanomaterials ; Nanoparticles ; Nanostructure ; Nanostructures ; Optical arrays ; plasmonics ; Plasmons ; Quantum electronics ; Semiconductor device measurement ; Yield estimation</subject><ispartof>IEEE journal of selected topics in quantum electronics, 2005-07, Vol.11 (4), p.778-784</ispartof><rights>Copyright The Institute of Electrical and Electronics Engineers, Inc. (IEEE) 2005</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c355t-4ee28bcd64604cfc0140ce9bd2bb344a9e3b183f98916c6e2cd59dca0ddad4f63</citedby><cites>FETCH-LOGICAL-c355t-4ee28bcd64604cfc0140ce9bd2bb344a9e3b183f98916c6e2cd59dca0ddad4f63</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://ieeexplore.ieee.org/document/1545976$$EHTML$$P50$$Gieee$$H</linktohtml><link.rule.ids>314,776,780,792,27901,27902,54733</link.rule.ids><linktorsrc>$$Uhttps://ieeexplore.ieee.org/document/1545976$$EView_record_in_IEEE$$FView_record_in_$$GIEEE</linktorsrc></links><search><creatorcontrib>Yongdong Liu</creatorcontrib><creatorcontrib>Mahdavi, F.</creatorcontrib><creatorcontrib>Blair, S.</creatorcontrib><title>Enhanced fluorescence transduction properties of metallic nanocavity arrays</title><title>IEEE journal of selected topics in quantum electronics</title><addtitle>JSTQE</addtitle><description>We studied fluorescence enhancement of molecular species bound within metallic nanocavities. These nanostructures possess a number of desirable properties for real-time microarrays, such as localization of excitation light within the nanocavities, strong isolation from fluorescence produced by unbound species, and an apparent increase in fluorescence yield for bound species. Experimental measurements show nearly a factor of two increase in excitation intensity within the nanocavities, and factor of six increase in yield. A simple electromagnetic model of a dipole within a nanocavity shows an increase in radiative output consistent with our yield estimates, and also verifies the strong fluorescence isolation from species lying outside the nanocavity.</description><subject>Arrays</subject><subject>Biotechnology</subject><subject>Cities and towns</subject><subject>Excitation</subject><subject>Fluorescence</subject><subject>Kinetic theory</subject><subject>Mathematical models</subject><subject>molecular detection</subject><subject>Nanocomposites</subject><subject>Nanomaterials</subject><subject>Nanoparticles</subject><subject>Nanostructure</subject><subject>Nanostructures</subject><subject>Optical arrays</subject><subject>plasmonics</subject><subject>Plasmons</subject><subject>Quantum electronics</subject><subject>Semiconductor device measurement</subject><subject>Yield estimation</subject><issn>1077-260X</issn><issn>1558-4542</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><sourceid>RIE</sourceid><recordid>eNp9kU9LxDAQxYsouK5-APFSPOip6yRN0uQoy_p3QcQVvIU0mWKXbrsmrbDf3qwrCB48zQz83swbXpKcEpgQAurq4WXxPJtQAD6RvBBS7iUjwrnMGGd0P_ZQFBkV8HaYHIWwBADJJIySx1n7blqLLq2aofMYLMYp7b1pgxtsX3dtuvbdGn1fY0i7Kl1hb5qmtmlr2s6az7rfpMZ7swnHyUFlmoAnP3WcvN7MFtO7bP50ez-9nmc257zPGCKVpXWCCWC2skAYWFSlo2WZM2YU5iWReaWkIsIKpNZx5awB54xjlcjHyeVubzT2MWDo9aqOvpvGtNgNQUslaNwNNJIX_5JUAqVEQATP_4DLbvBt_EIrQlQhCWzvkh1kfReCx0qvfb0yfqMJ6G0K-jsFvU1B71KImrOdpkbEX54zrgqRfwFyL4UV</recordid><startdate>20050701</startdate><enddate>20050701</enddate><creator>Yongdong Liu</creator><creator>Mahdavi, F.</creator><creator>Blair, S.</creator><general>IEEE</general><general>The Institute of Electrical and Electronics Engineers, Inc. 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These nanostructures possess a number of desirable properties for real-time microarrays, such as localization of excitation light within the nanocavities, strong isolation from fluorescence produced by unbound species, and an apparent increase in fluorescence yield for bound species. Experimental measurements show nearly a factor of two increase in excitation intensity within the nanocavities, and factor of six increase in yield. A simple electromagnetic model of a dipole within a nanocavity shows an increase in radiative output consistent with our yield estimates, and also verifies the strong fluorescence isolation from species lying outside the nanocavity.</abstract><cop>New York</cop><pub>IEEE</pub><doi>10.1109/JSTQE.2005.857688</doi><tpages>7</tpages></addata></record> |
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subjects | Arrays Biotechnology Cities and towns Excitation Fluorescence Kinetic theory Mathematical models molecular detection Nanocomposites Nanomaterials Nanoparticles Nanostructure Nanostructures Optical arrays plasmonics Plasmons Quantum electronics Semiconductor device measurement Yield estimation |
title | Enhanced fluorescence transduction properties of metallic nanocavity arrays |
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